Enhanced thermoelectric performance via carrier energy filtering effect in β-Zn4Sb3 alloy bulk embedded with (Bi2Te3)0.2(Sb2Te3)0.8

2014 ◽  
Vol 115 (5) ◽  
pp. 053710 ◽  
Author(s):  
T. H. Zou ◽  
X. Y. Qin ◽  
D. Li ◽  
B. J. Ren ◽  
G. L. Sun ◽  
...  
2018 ◽  
Vol 6 (43) ◽  
pp. 21341-21349 ◽  
Author(s):  
Amir Pakdel ◽  
Quansheng Guo ◽  
Valeria Nicolosi ◽  
Takao Mori

24 month high-ZT stability of Bi0.5Sb1.5Te3/Sb2O3 nanocomposites that demonstrate simultaneous Seebeck coefficient enhancement and thermal conductivity decline through energy filtering effect.


2015 ◽  
Vol 08 (06) ◽  
pp. 1550070
Author(s):  
Boyu Zhang ◽  
Jun Wang ◽  
Xinba Yaer ◽  
Zhenzhen Huo ◽  
Yin Wu ◽  
...  

Effect of crystal size distribution on thermoelectric performance of Lanthanum-doped strontium titanate ( La - SrTiO 3) ceramics are investigated in this study. Thermoelectric performance measurement, coupled with microstructure studies, shows that the electrical conductivity strongly depends on the crystal size, potential barrier on the grain boundary and porosity. Meantime, because the average potential barriers height are increased along with the reduction of crystal size, the Seebeck coefficients are increased by energy filtering effect at the large number of grain boundaries. As a result, by controlling of crystal size distribution, ZT value of La - SrTiO 3 is improved.


2021 ◽  
Vol 5 (1) ◽  
pp. 267-273
Author(s):  
Hyeonseok Hwang ◽  
Kwang-Suk Jang

High-performance thermoelectric all-carbon heterostructures are investigated. The carbon nanoparticle barrier between carbon nanotubes can enhance the thermoelectric performance due to the energy filtering effect.


Materials ◽  
2021 ◽  
Vol 15 (1) ◽  
pp. 148
Author(s):  
Hong-Ju Ahn ◽  
Seil Kim ◽  
Kwang Ho Kim ◽  
Joo-Yul Lee

In this study, we prepared Te nanorod arrays via a galvanic displacement reaction (GDR) on a Si wafer, and their composite with poly(3,4-ethylenedioxythiophene) (PEDOT) were successfully synthesized by electrochemical polymerization with lithium perchlorate (LiClO4) as a counter ion. The thermoelectric performance of the composite film was optimized by adjusting the polymerization time. As a result, a maximum power factor (PF) of 235 µW/mK2 was obtained from a PEDOT/Te composite film electrochemically polymerized for 15 s at room temperature, which was 11.7 times higher than that of the PEDOT film, corresponding to a Seebeck coefficient (S) of 290 µV/K and electrical conductivity (σ) of 28 S/cm. This outstanding PF was due to the enhanced interface interaction and carrier energy filtering effect at the interfacial potential barrier between the PEDOT and Te nanorods. This study demonstrates that the combination of an inorganic Te nanorod array with electrodeposited PEDOT is a promising strategy for developing high-performance thermoelectric materials.


2019 ◽  
Vol 7 (26) ◽  
pp. 15757-15765 ◽  
Author(s):  
Rui Xu ◽  
Lulu Huang ◽  
Jian Zhang ◽  
Di Li ◽  
Jizi Liu ◽  
...  

Through magnetic field-assisted hydrothermal synthesis, high thermoelectric performance of SnSe is obtained due to Se quantum dots and smaller nano grains, leading to enhanced density of states and energy filtering effect.


2018 ◽  
Vol 11 (04) ◽  
pp. 1850069 ◽  
Author(s):  
Xuerui Liu ◽  
Shuankui Li ◽  
Tinyang Liu ◽  
Weiming Zhu ◽  
Rui Wang ◽  
...  

With the development of nanotechnology, thermoelectric materials with complex heterogeneous nanostructure offer a promising approach to improve the thermoelectric performance. In this work, SnSe/SnS hetero-nanosheet was tuned by the epitaxial growth of SnSe on the few layers of SnS nanosheets. The heterojunction interface can optimize the carrier/phonon transport behavior by energy filtering effect and scattering the phonon in multiple scales. Compared with pristine SnSe, the power factor of SnSe/SnS hetero-nanosheet increases from 2.2[Formula: see text][Formula: see text]V/cmK2 to 3.21[Formula: see text][Formula: see text]V/cmK2 at 773[Formula: see text]K, whereas the thermal conductivity decreases significantly from 0.65[Formula: see text]W[Formula: see text][Formula: see text][Formula: see text]m[Formula: see text] to 0.48[Formula: see text]W[Formula: see text][Formula: see text][Formula: see text]m[Formula: see text] at 773[Formula: see text]K. The maximum ZT of 0.5 is obtained at 773[Formula: see text]K in the SnSe/SnS hetero-nanosheets, which is 89% higher than pristine SnSe. This approach is proved to be a promising strategy to design high performance thermoelectric materials.


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