scholarly journals Exploring Relations between Cloud Morphology, Cloud Phase, and Cloud Radiative Properties in Southern Ocean Stratocumulus Clouds

2021 ◽  
Author(s):  
Jessica Danker ◽  
Odran Sourdeval ◽  
Isabel L. McCoy ◽  
Robert Wood ◽  
Anna Possner
Keyword(s):  
Southern Ocean ◽  
Austral Summer ◽  
Supercooled Liquid ◽  
Mixed Phase ◽  
Radiative Properties ◽  
Radiative Effect ◽  
Open Cell ◽  
Cloud Albedo ◽  
Organizational Patterns ◽  
Cloud Radiative Properties

Abstract. Marine stratocumuli are the most dominant cloud type by area coverage in the Southern Ocean (SO). They can be divided into different self-organized cellular morphological regimes known as open and closed mesoscale-cellular convec- tive (MCC) clouds. Open and closed cells are the two most frequent types of organizational regimes in the SO. Using the liDAR- raDAR (DARDAR) version 2 retrievals, we quantify 59 % of all MCC clouds in this region as mixed-phase clouds (MPCs) during a 4-year time period from 2007 to 2010. The net radiative effect of SO MCC clouds is governed by changes in cloud albedo. Both, cloud morphology and phase, have previously been shown to impact cloud albedo individually, but their interac- tions and their combined impact on cloud albedo remain unclear. Here, we investigate the relationships between cloud phase, organizational patterns, and their differences regarding their cloud radiative properties in the SO. The mixed-phase fraction, which is defined as the number of MPCs divided by the sum of MPC and supercooled liquid cloud (SLC) pixels, of all MCC clouds at a given cloud-top temperature (CTT) varies considerably between austral summer and winter. We further find that seasonal changes in cloud phase at a given CTT across all latitudes are largely independent of cloud morphology and are thus seemingly constrained by other external factors. Overall, our results show a stronger dependence of cloud phase on cloud-top height (CTH) than CTT for clouds below 2.5 km in altitude. Preconditioning through ice-phase processes in MPCs has been observed to accelerate individual closed to open cell transitions in extratropical stratocumuli. The hypothesis of preconditioning has been further substantiated in large-eddy simulations of open and closed MPCs. In this study, we do not find preconditioning to primarily impact climatological SO cloud mor- phology statistics. Meanwhile, in-cloud albedo analysis reveals stronger changes in open and closed cell albedo in SLCs than MPCs. In particular few optically thick (cloud optical thickness > 10) open cell stratocumuli are characterized as ice-free SLCs. Theses differences in in-cloud albedo are found to alter the cloud radiative effect in the SO by 12 W m−2 to 39 W m−2 depending on season and cloud phase.

scholarly journals The efficacy of aerosol–cloud radiative perturbations from near-surface emissions in deep open-cell stratocumuli

2018 ◽  
Vol 18 (23) ◽  
pp. 17475-17488 ◽  
Author(s):  
Anna Possner ◽  
Hailong Wang ◽  
Robert Wood ◽  
Ken Caldeira ◽  
Thomas P. Ackerman
Keyword(s):  
Emission Line ◽  
Radiative Properties ◽  
Radiative Effect ◽  
Radiative Effects ◽  
Near Surface ◽  
Open Cell ◽  
Detection And Attribution ◽  
Cloud Radiative Effects ◽  
Ship Tracks ◽  
Cloud Radiative Properties

Abstract. Aerosol–cloud radiative effects are determined and quantified in simulations of deep open-cell stratocumuli observed during the VAMOS Ocean-Cloud-Atmosphere-Land Study Regional Experiment (VOCALS-REx) campaign off the west coast of Chile. The cloud deck forms in a boundary layer 1.5 km deep, with cell sizes reaching 50 km in diameter. Global databases of ship tracks suggest that these linear structures are seldom found in boundary layers this deep. Here, we quantify the changes in cloud radiative properties to a continuous aerosol point source moving along a fixed emission line releasing 1017 particles per second. We show that a spatially coherent cloud perturbation is not evident along the emission line. Yet our model simulates an increase in domain-mean all-sky albedo of 0.05, corresponding to a diurnally averaged cloud radiative effect of 20 W m−2, given the annual mean solar insolation at the VOCALS-REx site. Therefore, marked changes in cloud radiative properties in precipitating deep open cells may be driven by anthropogenic near-surface aerosol perturbations, such as those generated by ships. Furthermore, we demonstrate that these changes in cloud radiative properties are masked by the naturally occurring variability within the organised cloud field. A clear detection and attribution of cloud radiative effects to a perturbation in aerosol concentrations becomes possible when sub-filtering of the cloud field is applied, using the spatio-temporal distribution of the aerosol perturbation. Therefore, this work has implications for the detection and attribution of effective cloud radiative forcing in marine stratocumuli, which constitutes one of the major physical uncertainties within the climate system. Our results suggest that ships may sometimes have a substantial radiative effect on marine clouds and albedo, even when ship tracks are not readily visible.

scholarly journals The efficacy of aerosol-cloud-radiative perturbations from near-surface emissions in deep open-cell stratocumulus

2018 ◽  
Author(s):  
Anna Possner ◽  
Hailong Wang ◽  
Robert Wood ◽  
Ken Caldeira ◽  
Thomas Ackerman
Keyword(s):  
Emission Line ◽  
Radiative Properties ◽  
Radiative Effect ◽  
Radiative Effects ◽  
Near Surface ◽  
Open Cell ◽  
Detection And Attribution ◽  
Cloud Radiative Effects ◽  
Ship Tracks ◽  
Cloud Radiative Properties

Abstract. Aerosol-cloud-radiative effects are determined and quantified in simulations of deep open-cell stratocumuli observed during the VOCALS-REx campaign off the West coast of Chile. The cloud deck forms in a 1.5 km deep boundary layer with cell sizes reaching 50 km in diameter. Global data bases of ship tracks suggest that these linear structures are seldom found in boundary layers this deep. Here, we quantify the changes in cloud-radiative properties to a continuous aerosol point source moving along a fixed emission line releasing 1017 particles per second. We show that a spatially coherent cloud perturbation is not evident along the emission line. Yet, our models simulates an increase in domain-mean all-sky albedo of 0.05 corresponding to a diurnally-averaged cloud-radiative effect of 20 W m−2 given the annual mean solar insolation at the VOCALS-REx site. Therefore, marked changes in cloud-radiative properties in precipitating deep open cells may be driven by anthropogenic near-surface aerosol perturbations such as ships. Furthermore, we demonstrate that these changes in cloud-radiative properties are masked by the natural variability within the organised cloud field. A clear detection and attribution of cloud-radiative effects to a perturbation in aerosol concentrations becomes possible when sub-filtering of the cloud field is applied utilising the spatio-temporal distribution of the aerosol perturbation. Therefore, this work has implications for the detection and attribution of effective cloud-radiative forcing in marine stratocumuli, which constitutes one of the major physical uncertainties within the climate system. Our results suggest that ships may sometimes have a substantial radiative effect on marine clouds and albedo even when ship tracks are not readily visible.

scholarly journals A Modeling Case Study of Mixed-Phase Clouds over the Southern Ocean and Tasmania

2010 ◽  
Vol 138 (3) ◽  
pp. 839-862 ◽  
Author(s):  
Anthony E. Morrison ◽  
Steven T. Siems ◽  
Michael J. Manton ◽  
Alex Nazarov
Keyword(s):  
Southern Ocean ◽  
Supercooled Liquid ◽  
Mixed Phase ◽  
Weather Research And Forecasting ◽  
Marine Stratocumulus ◽  
Cloud Structure ◽  
In Situ Observations ◽  
Cloud Tops ◽  
Mixed Phase Clouds

Abstract The cloud structure associated with two frontal passages over the Southern Ocean and Tasmania is investigated. The first event, during August 2006, is characterized by large quantities of supercooled liquid water and little ice. The second case, during October 2007, is more mixed phase. The Weather Research and Forecasting model (WRFV2.2.1) is evaluated using remote sensed and in situ observations within the post frontal air mass. The Thompson microphysics module is used to describe in-cloud processes, where ice is initiated using the Cooper parameterization at temperatures lower than −8°C or at ice supersaturations greater than 8%. The evaluated cases are then used to numerically investigate the prevalence of supercooled and mixed-phase clouds over Tasmania and the ocean to the west. The simulations produce marine stratocumulus-like clouds with maximum heights of between 3 and 5 km. These are capped by weak temperature and strong moisture inversions. When the inversion is at temperatures warmer than −10°C, WRF produces widespread supercooled cloud fields with little glaciation. This is consistent with the limited in situ observations. When the inversion is at higher altitudes, allowing cooler cloud tops, glaciated (and to a lesser extent mixed phase) clouds are more common. The simulations are further explored to evaluate any orographic signature within the cloud structure over Tasmania. No consistent signature is found between the two cases.

scholarly journals Evaluation of Southern Ocean cloud in the HadGEM3 general circulation model and MERRA-2 reanalysis using ship-based observations

2020 ◽  
Vol 20 (11) ◽  
pp. 6607-6630 ◽  
Author(s):  
Peter Kuma ◽  
Adrian J. McDonald ◽  
Olaf Morgenstern ◽  
Simon P. Alexander ◽  
John J. Cassano ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Southern Ocean ◽  
General Circulation ◽  
Cloud Cover ◽  
Atmospheric Stability ◽  
Austral Summer ◽  
Circulation Model ◽  
Radiation Budget ◽  
Cloud Albedo ◽  
Low Cloud

Abstract. Southern Ocean (SO) shortwave (SW) radiation biases are a common problem in contemporary general circulation models (GCMs), with most models exhibiting a tendency to absorb too much incoming SW radiation. These biases have been attributed to deficiencies in the representation of clouds during the austral summer months, either due to cloud cover or cloud albedo being too low. The problem has been the focus of many studies, most of which utilised satellite datasets for model evaluation. We use multi-year ship-based observations and the CERES spaceborne radiation budget measurements to contrast cloud representation and SW radiation in the atmospheric component Global Atmosphere (GA) version 7.1 of the HadGEM3 GCM and the MERRA-2 reanalysis. We find that the prevailing bias is negative in GA7.1 and positive in MERRA-2. GA7.1 performs better than MERRA-2 in terms of absolute SW bias. Significant errors of up to 21 W m−2 (GA7.1) and 39 W m−2 (MERRA-2) are present in both models in the austral summer. Using ship-based ceilometer observations, we find low cloud below 2 km to be predominant in the Ross Sea and the Indian Ocean sectors of the SO. Utilising a novel surface lidar simulator developed for this study, derived from an existing Cloud Feedback Model Intercomparison Project (CFMIP) Observation Simulator Package (COSP) – active remote sensing simulator (ACTSIM) spaceborne lidar simulator, we find that GA7.1 and MERRA-2 both underestimate low cloud and fog occurrence relative to the ship observations on average by 4 %–9 % (GA7.1) and 18 % (MERRA-2). Based on radiosonde observations, we also find the low cloud to be strongly linked to boundary layer atmospheric stability and the sea surface temperature. GA7.1 and MERRA-2 do not represent the observed relationship between boundary layer stability and clouds well. We find that MERRA-2 has a much greater proportion of cloud liquid water in the SO in austral summer than GA7.1, a likely key contributor to the difference in the SW radiation bias. Our results suggest that subgrid-scale processes (cloud and boundary layer parameterisations) are responsible for the bias and that in GA7.1 a major part of the SW radiation bias can be explained by cloud cover underestimation, relative to underestimation of cloud albedo.

scholarly journals The importance of mixed-phase clouds for climate sensitivity in the global aerosol-climate model ECHAM6-HAM2

2018 ◽  
Author(s):  
Ulrike Lohmann ◽  
David Neubauer
Keyword(s):  
Southern Ocean ◽  
Climate Sensitivity ◽  
Liquid Water ◽  
Climate Model ◽  
Global Climate Model ◽  
Supercooled Liquid ◽  
Mixed Phase ◽  
Radiation Budget ◽  
Shortwave Radiation ◽  
Mixed Phase Clouds

Abstract. Clouds are important in the climate system because of their large influence on the radiation budget. On the one hand, they scatter solar radiation and with that cool the climate. On the other hand, they absorb and re-emit terrestrial radiation, which causes a warming. How clouds change in a warmer climate is one of the largest uncertainties for the equilibrium climate sensitivity (ECS). While a large spread in the cloud feedback arises from low-level clouds, it was recently shown that also mixed-phase clouds are important for ECS. If mixed-phase clouds in the current climate contain too few supercooled cloud droplets, too much ice will change to liquid water in a warmer climate. As shown by Tan et al. (2016), this overestimates the negative cloud phase feedback and underestimates ECS in the CAM global climate model (GCM). Here we are using the newest version of the ECHAM6-HAM2 GCM to investigate the importance of mixed-phase clouds for ECS. Although we also considerably underestimate the fraction of supercooled liquid water globally in the reference version of ECHAM6-HAM2 GCM, we do not obtain increases in ECS in simulations with more supercooled liquid water in the present-day climate, contrary to the findings by Tan et al. (2016). We hypothesize that it is not the global supercooled liquid water fraction that matters, but only how well low- and mid-level mixed-phase clouds with cloud top temperatures in the mixed-phase temperature range between 0 and −35 ºC are simulated. These occur most frequent in mid-latitudes, in particular over the Southern Ocean where they determine the amount of absorbed shortwave radiation. In ECHAM6-HAM2 the amount of absorbed shortwave radiation over the Southern Ocean is only overestimated if all clouds below 0 ºC consist exclusively of ice and only in this simulation is ECS is significantly smaller than in all other simulations. Hence, the negative cloud phase feedback seems to be important only if the optically thin low- and mid-level mid-latitude clouds have the wrong phase (ice instead of liquid water) in the absence of overlying clouds. In all other simulations, changes in cloud feedbacks associated with cloud amount and cloud top pressure, dominate.

scholarly journals Satellite‐Based Detection of Daytime Supercooled Liquid‐Topped Mixed‐Phase Clouds Over the Southern Ocean Using the Advanced Himawari Imager

2019 ◽  
Vol 124 (5) ◽  
pp. 2677-2701 ◽  
Author(s):  
Yoo‐Jeong Noh ◽  
Steven D. Miller ◽  
Andrew K. Heidinger ◽  
Gerald G. Mace ◽  
Alain Protat ◽  
...  
Keyword(s):  
Southern Ocean ◽  
Supercooled Liquid ◽  
Mixed Phase ◽  
Mixed Phase Clouds

scholarly journals The contribution of black carbon to global ice nucleating particle concentrations relevant to mixed-phase clouds

2020 ◽  
Vol 117 (37) ◽  
pp. 22705-22711
Author(s):  
Gregory P. Schill ◽  
Paul J. DeMott ◽  
Ethan W. Emerson ◽  
Anne Marie C. Rauker ◽  
John K. Kodros ◽  
...  
Keyword(s):  
Black Carbon ◽  
Biomass Burning ◽  
Fossil Fuel ◽  
Supercooled Liquid ◽  
Mixed Phase ◽  
Radiative Properties ◽  
Prescribed Burns ◽  
Earth’S Climate ◽  
Mixed Phase Clouds ◽  
Fossil Fuel Emissions

Black carbon (BC) aerosol plays an important role in the Earth’s climate system because it absorbs solar radiation and therefore potentially warms the climate; however, BC can also act as a seed for cloud particles, which may offset much of its warming potential. If BC acts as an ice nucleating particle (INP), BC could affect the lifetime, albedo, and radiative properties of clouds containing both supercooled liquid water droplets and ice particles (mixed-phase clouds). Over 40% of global BC emissions are from biomass burning; however, the ability of biomass burning BC to act as an INP in mixed-phase cloud conditions is almost entirely unconstrained. To provide these observational constraints, we measured the contribution of BC to INP concentrations ([INP]) in real-world prescribed burns and wildfires. We found that BC contributes, at most, 10% to [INP] during these burns. From this, we developed a parameterization for biomass burning BC and combined it with a BC parameterization previously used for fossil fuel emissions. Applying these parameterizations to global model output, we find that the contribution of BC to potential [INP] relevant to mixed-phase clouds is ∼5% on a global average.

scholarly journals Photomineralization mechanism changes the ability of dissolved organic matter to activate cloud droplets and to nucleate ice crystals

2019 ◽  
Author(s):  
Nadine Borduas-Dedekind ◽  
Rachele Ossola ◽  
Robert O. David ◽  
Lin S. Boynton ◽  
Vera Weichlinger ◽  
...  
Keyword(s):  
Organic Matter ◽  
Dissolved Organic Matter ◽  
Hydrological Cycle ◽  
Supercooled Liquid ◽  
Mixed Phase ◽  
Ice Crystals ◽  
Radiative Properties ◽  
Cloud Droplets ◽  
Photochemical Processing ◽  
Mixed Phase Clouds

Abstract. An organic aerosol particle has a lifetime of approximately one week in the atmosphere during which it will be exposed to sunlight. Yet, the effect of photochemistry on the propensity of organic matter to participate in the initial cloud-forming steps is difficult to predict. In this study, we quantify on a molecular scale the effect of photochemical exposure of naturally occurring dissolved organic matter (DOM) and of a fulvic acid standard on its ability to form mixed-phase clouds, by acting as cloud condensation nuclei (CCN) and by acting as ice nucleating particles (INPs). We find that photochemical processing, equivalent to 4.6 days in the atmosphere, of DOM increases its ability to form cloud droplets by up to a factor of 2.5 but decreases its ability to form ice crystals at a loss rate of −0.04°CT50 h−1 of sunlight at ground level. In other words, the ice nucleation activity of photooxidized DOM can require up to 4 degrees colder temperatures for 50 % of the droplets to activate as ice crystals under immersion freezing conditions. This temperature change could impact the ratio of ice to water droplets within a mixed phase cloud by delaying the onset of glaciation and by increasing the supercooled liquid fraction of the cloud, thereby modifying the radiative properties and the lifetime of the cloud. Concurrently, a photomineralization mechanism was quantified by monitoring the loss of organic carbon and the simultaneous production of organic acids, such as formic, acetic, oxalic and pyruvic acids, CO and CO2. This mechanism explains and predicts the observed increase in CCN and decrease in INP efficiencies. Indeed, we show that photochemical processing can be a dominant atmospheric aging process, impacting CCN and INP efficiencies and concentrations. Photomineralization can thus alter the aerosol-cloud radiative effects of organic matter by modifying the supercooled liquid water-to-ice crystal ratio in mixed-phase clouds with implications for cloud lifetime, precipitation patterns and the hydrological cycle.

scholarly journals On the Representation of High-Latitude Boundary Layer Mixed-Phase Cloud in the ECMWF Global Model

2014 ◽  
Vol 142 (9) ◽  
pp. 3425-3445 ◽  
Author(s):  
Richard M. Forbes ◽  
Maike Ahlgrimm
Keyword(s):  
Boundary Layer ◽  
Liquid Water ◽  
Large Scale ◽  
Weather Prediction ◽  
Supercooled Liquid ◽  
Mixed Phase ◽  
Radiative Properties ◽  
Small Scale ◽  
Physical Processes ◽  
Boundary Layer Clouds

Supercooled liquid water (SLW) layers in boundary layer clouds are abundantly observed in the atmosphere at high latitudes, but remain a challenge to represent in numerical weather prediction (NWP) and climate models. Unresolved processes such as small-scale turbulence and mixed-phase microphysics act to maintain the liquid layer at cloud top, directly affecting cloud radiative properties and prolonging cloud lifetimes. This paper describes the representation of supercooled liquid water in boundary layer clouds in the European Centre for Medium-Range Weather Forecasts (ECMWF) global NWP model and in particular the change from a diagnostic temperature-dependent mixed phase to a prognostic representation with separate cloud liquid and ice variables. Data from the Atmospheric Radiation Measurement site in Alaska and from the CloudSat/Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite missions are used to evaluate the model parameterizations. The prognostic scheme shows a more realistic cloud structure, with an SLW layer at cloud top and ice falling out below. However, because of the limited vertical and horizontal resolution and uncertainties in the parameterization of physical processes near cloud top, the change leads to an overall reduction in SLW water with a detrimental impact on shortwave and longwave radiative fluxes, and increased 2-m temperature errors over land. A reduction in the ice deposition rate at cloud top significantly improves the SLW occurrence and radiative impacts, and highlights the need for improved understanding and parameterization of physical processes for mixed-phase cloud in large-scale models.

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