A generalizable, data-driven online approach to forecast capacity degradation trajectory of lithium batteries

Author(s):  
Xinyan Liu ◽  
Xue-Qiang Zhang ◽  
Xiang Chen ◽  
Gao-Long Zhu ◽  
Chong Yan ◽  
...  
Polymers ◽  
2020 ◽  
Vol 12 (6) ◽  
pp. 1324 ◽  
Author(s):  
Jin Cui ◽  
Zehao Zhou ◽  
Mengyang Jia ◽  
Xin Chen ◽  
Chuan Shi ◽  
...  

Composite electrolytes consisting of polymers and three-dimensional (3D) fillers are considered to be promising electrolytes for solid lithium batteries owing to their virtues of continuous lithium-ion pathways and good mechanical properties. In the present study, an electrolyte with polyethylene oxide–lithium (bis trifluoromethyl) sulfate–succinonitrile (PLS) and frameworks of three-dimensional SiO2 nanofibers (3D SiO2 NFs) was prepared. Taking advantage of the highly conductive interfaces between 3D SiO2 NFs and PLS, the total conductivity of the electrolyte at 30 °C was approximately 9.32 × 10−5 S cm−1. With a thickness of 27 μm and a tensile strength of 7.4 MPa, the electrolyte achieved an area specific resistance of 29.0 Ω cm2. Moreover, such a 3D configuration could homogenize the electrical field, which was beneficial for suppressing dendrite growth. Consequently, Li/LiFePO4 cells assembled with PLS and 3D SiO2 NFs (PLS/3D SiO2 NFs), which delivered an original specific capacity of 167.9 mAh g−1, only suffered 3.28% capacity degradation after 100 cycles. In particular, these cells automatically shut down when PLS was decomposed above 400 °C, and the electrodes were separated by the solid framework of 3D SiO2 NFs. Therefore, the solid lithium batteries based on composite electrolytes reported here offer high safety at elevated temperatures.


Nature Energy ◽  
2019 ◽  
Vol 4 (5) ◽  
pp. 383-391 ◽  
Author(s):  
Kristen A. Severson ◽  
Peter M. Attia ◽  
Norman Jin ◽  
Nicholas Perkins ◽  
Benben Jiang ◽  
...  

Author(s):  
Zhimin Xi ◽  
Xiangxue Zhao

Data-driven prognostics typically requires sufficient offline training data sets for accurate remaining useful life (RUL) prediction of engineering products. This paper investigates performances of typical data-driven methodologies when the amount of training data sets is insufficient. The purpose is to better understand these methodologies especially when offline training datasets are insufficient. The neural network, similarity-based approach, and copula-based sampling approach were investigated when only three run-to-failure training units were available. The example of lithium-ion (Li-ion) battery capacity degradation was employed for the demonstration.


2020 ◽  
Vol 3 (6) ◽  
pp. 5472-5478
Author(s):  
Kentaro Kuratani ◽  
Atsushi Sakuda ◽  
Tomonari Takeuchi ◽  
Hironori Kobayashi

2018 ◽  
Vol 929 ◽  
pp. 93-102
Author(s):  
Didik Djoko Susilo ◽  
Achmad Widodo ◽  
Toni Prahasto ◽  
Muhammad Nizam

Lithium-ion batteries play a critical role in the reliability and safety of a system. Battery health monitoring and remaining useful life (RUL) prediction are needed to prevent catastrophic failure of the battery. The aim of this research is to develop a data-driven method to monitor the batteries state of health and predict their RUL by using the battery capacity degradation data. This paper also investigated the effect of prediction starting point to the RUL prediction error. One of the data-driven method drawbacks is the need of a large amount of data to obtain accurate prediction. This paper proposed a method to generate a series of degradation data that follow the Gaussian distribution based on limited battery capacity degradation data. The prognostic model was constructed from the new data using least square support vector machine (LSSVM) regression. The remaining useful life prediction was carried out by extrapolating the model until reach the end of life threshold. The method was applied to three differences lithium-ion batteries capacity data. The results showed that the proposed method has good performance. The method can predict the lithium-ion batteries RUL with a small error, and the optimal RUL starting point was found at the point where the battery has experienced the highest capacity recovery due to the self-recharge phenomenon.


2020 ◽  
Vol 13 (5) ◽  
pp. 1429-1461 ◽  
Author(s):  
Xiaona Li ◽  
Jianwen Liang ◽  
Xiaofei Yang ◽  
Keegan R. Adair ◽  
Changhong Wang ◽  
...  

This review focuses on fundamental understanding, various synthesis routes, chemical/electrochemical stability of halide-based lithium superionic conductors, and their potential applications in energy storage as well as related challenges.


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