Effects of the sea-land breeze on coastal ozone pollution in the Yangtze River Delta, China

2022 ◽  
Vol 807 ◽  
pp. 150306
Author(s):  
Dandan Zhao ◽  
Jinyuan Xin ◽  
Weifeng Wang ◽  
Danjie Jia ◽  
Zifa Wang ◽  
...  
2020 ◽  
Author(s):  
Wuke Wang

<p><span>Ozone pollution is currently a serious environmental issue in China. Most of studies have attributed the surface ozone pollution over China to the strong photochemical production from anthropogenic sources. As another important source of tropospheric ozone, the stratospheric intrusion (SI), however, has been less concerned. This study investigates the SI events over the Yangtze River Delta in eastern China using the newest ERA5 (the fifth generation of ECMWF atmospheric reanalysis) meteorological and ozone data, the In-service Aircraft for a Global Observing System (IAGOS) ozone profiles and the station-based ground-level ozone measurements. Results indicate that SI plays important roles in spring and summer ozone pollution episodes over the Yangtze River Delta, eastern China. Based on CAM-Chem (the Community Atmosphere Model with Chemistry) and LPDM (Lagrangian Particle Dispersion Modeling) model simulations, we found that deep SIs contribute ~15 ppbv in spring and ~10 ppbv in summer to surface ozone variations in eastern China. A deep SI event occurred in 2018 spring associated with a strong horizontal-trough, which brought ozone-rich air from the stratosphere to the troposphere and resulted in severe surface ozone pollution over the Yangtze River Delta. From 7-year statistics, we found that strong SI events during summer are associated with a cyclonic valley between the South Asian High and the Subtropical High, accompanied by downward fast transport of ozone from the stratosphere to the troposphere. Our results provide important information for surface ozone prediction and control in eastern China.</span></p>


2021 ◽  
Vol 21 (8) ◽  
pp. 5905-5917
Author(s):  
Kun Zhang ◽  
Ling Huang ◽  
Qing Li ◽  
Juntao Huo ◽  
Yusen Duan ◽  
...  

Abstract. In recent years, ozone pollution has become one of the most severe environmental problems in China. Evidence from observations have showed increased frequency of high O3 levels in suburban areas of the Yangtze River Delta (YRD) region. To better understand the formation mechanism of local O3 pollution and investigate the potential role of isoprene chemistry in the budgets of ROx (OH+HO2+RO2) radicals, synchronous observations of volatile organic compounds (VOCs), formaldehyde (HCHO), and meteorological parameters were conducted at a suburban site of the YRD region in 2018. Five episodes with elevated O3 concentrations under stagnant meteorological conditions were identified; an observation-based model (OBM) with the Master Chemical Mechanism was applied to analyze the photochemical processes during these high O3 episodes. The high levels of O3, nitrogen oxides (NOx), and VOCs facilitated strong production and recycling of ROx radicals with the photolysis of oxygenated VOCs (OVOCs) being the primary source. Our results suggest that local biogenic isoprene is important in suburban photochemical processes. Removing isoprene could drastically slow down the efficiency of ROx recycling and reduce the concentrations of ROx. In addition, the absence of isoprene chemistry could further lead to a decrease in the daily average concentrations of O3 and HCHO by 34 % and 36 %, respectively. Therefore, this study emphasizes the importance of isoprene chemistry in the suburban atmosphere, particularly with the participation of anthropogenic NOx. Moreover, our results provide insights into the radical chemistry that essentially drives the formation of secondary pollutants (e.g., O3 and HCHO) in suburban areas of the YRD region.


Author(s):  
Shufeng She ◽  
Bifeng Hu ◽  
Xianglin Zhang ◽  
Shuai Shao ◽  
Yefeng Jiang ◽  
...  

Potentially toxic elements (PTEs) pollution in the agricultural soil of China, especially in developed regions such as the Yangtze River Delta (YRD) in eastern China, has received increasing attention. However, there are few studies on the long-term assessment of soil pollution by PTEs over large regions. Therefore, in this study, a meta-analysis was conducted to evaluate the current state and temporal trend of PTEs pollution in the agricultural land of the Yangtze River Delta. Based on a review of 118 studies published between 1993 and 2020, the average concentrations of Cd, Hg, As, Pb, Cr, Cu, Zn, and Ni were found to be 0.25 mg kg−1, 0.14 mg kg−1, 8.14 mg kg−1, 32.32 mg kg−1, 68.84 mg kg−1, 32.58 mg kg−1, 92.35 mg kg−1, and 29.30 mg kg−1, respectively. Among these elements, only Cd and Hg showed significant accumulation compared with their background values. The eastern Yangtze River Delta showed a relatively high ecological risk due to intensive industrial activities. The contents of Cd, Pb, and Zn in soil showed an increasing trend from 1993 to 2000 and then showed a decreasing trend. The results obtained from this study will provide guidance for the prevention and control of soil pollution in the Yangtze River Delta.


Land ◽  
2021 ◽  
Vol 10 (8) ◽  
pp. 804
Author(s):  
Bo Niu ◽  
Dazhuan Ge ◽  
Rui Yan ◽  
Yingyi Ma ◽  
Dongqi Sun ◽  
...  

In recent years, the impact of land-use systems on global climate change has become increasingly significant, and land-use change has become a hot issue of concern to academics, both within China and abroad. Urbanization, as an important socioeconomic factor, plays a vital role in promoting land-use transition, which also shows a significant spatial dependence on urbanization. This paper constructs a theoretical framework for the interaction relationship between urbanization and land-use transition, taking the Yangtze River Delta as an example, and measures the level of urbanization from the perspective of population urbanization, economic urbanization and social urbanization, while also evaluating the level of land-use morphologies from the perspective of dominant and recessive morphologies of land-use. We construct a PVAR model and coupled coordination model based on the calculated indexes for empirical analysis. The results show that the relationship between urbanization and land-use transition is not a simple linear relationship, but tends to be complex with the process of urbanization, and reasonable urbanization and land-use morphologies will promote further benign coupling in the system. By analyzing the interaction relationship between urbanization and land-use transition, this study enriches the study of land-use change and provides new pathways for thinking about how to promote high-quality urbanization.


Sign in / Sign up

Export Citation Format

Share Document