scholarly journals Low-symmetry nonlocal transport in microstructured squares of delafossite metals

2021 ◽  
Vol 118 (47) ◽  
pp. e2113185118
Author(s):  
Philippa H. McGuinness ◽  
Elina Zhakina ◽  
Markus König ◽  
Maja D. Bachmann ◽  
Carsten Putzke ◽  
...  

Intense work studying the ballistic regime of electron transport in two-dimensional systems based on semiconductors and graphene had been thought to have established most of the key experimental facts of the field. In recent years, however, additional forms of ballistic transport have become accessible in the quasi–two-dimensional delafossite metals, whose Fermi wavelength is a factor of 100 shorter than those typically studied in the previous work and whose Fermi surfaces are nearly hexagonal in shape and therefore strongly faceted. This has some profound consequences for results obtained from the classic ballistic transport experiment of studying bend and Hall resistances in mesoscopic squares fabricated from delafossite single crystals. We observe pronounced anisotropies in bend resistances and even a Hall voltage that is strongly asymmetric in magnetic field. Although some of our observations are nonintuitive at first sight, we show that they can be understood within a nonlocal Landauer-Büttiker analysis tailored to the symmetries of the square/hexagonal geometries of our combined device/Fermi surface system. Signatures of nonlocal transport can be resolved for squares of linear dimension of nearly 100 µm, approximately a factor of 15 larger than the bulk mean free path of the crystal from which the device was fabricated.

2019 ◽  
Vol 10 (1) ◽  
Author(s):  
Maja D. Bachmann ◽  
Aaron L. Sharpe ◽  
Arthur W. Barnard ◽  
Carsten Putzke ◽  
Markus König ◽  
...  

Abstract Geometric electron optics may be implemented in solids when electron transport is ballistic on the length scale of a device. Currently, this is realized mainly in 2D materials characterized by circular Fermi surfaces. Here we demonstrate that the nearly perfectly hexagonal Fermi surface of PdCoO2 gives rise to highly directional ballistic transport. We probe this directional ballistic regime in a single crystal of PdCoO2 by use of focused ion beam (FIB) micro-machining, defining crystalline ballistic circuits with features as small as 250 nm. The peculiar hexagonal Fermi surface naturally leads to enhanced electron self-focusing effects in a magnetic field compared to circular Fermi surfaces. This super-geometric focusing can be quantitatively predicted for arbitrary device geometry, based on the hexagonal cyclotron orbits appearing in this material. These results suggest a novel class of ballistic electronic devices exploiting the unique transport characteristics of strongly faceted Fermi surfaces.


Nanomaterials ◽  
2021 ◽  
Vol 11 (9) ◽  
pp. 2361
Author(s):  
John Stearns ◽  
Garret Moddel

Geometric diodes are planar conductors patterned asymmetrically to provide electrical asymmetry, and they have exhibited high-frequency rectification in infrared rectennas. These devices function by ballistic or quasi-ballistic transport in which the transport characteristics are sensitive to the device geometry. Common methods for predicting device performance rely on the assumption of totally ballistic transport and neglect the effects of electron momentum relaxation. We present a particle-in-cell Monte Carlo simulation method that allows the prediction of the current–voltage characteristics of geometric diodes operating quasi-ballistically, with the mean-free-path length shorter than the critical device dimensions. With this simulation method, we analyze a new diode geometry made from graphene that shows an improvement in rectification capability over previous geometries. We find that the current rectification capability of a given geometry is optimized for a specific mean-free-path length, such that arbitrarily large mean-free-path lengths are not desirable. These results present a new avenue for understanding geometric effects in the quasi-ballistic regime and show that the relationship between device dimensions and the carrier mean-free-path length can be adjusted to optimize device performance.


Author(s):  
L. Reimer ◽  
R. Oelgeklaus

Quantitative electron energy-loss spectroscopy (EELS) needs a correction for the limited collection aperture α and a deconvolution of recorded spectra for eliminating the influence of multiple inelastic scattering. Reversely, it is of interest to calculate the influence of multiple scattering on EELS. The distribution f(w,θ,z) of scattered electrons as a function of energy loss w, scattering angle θ and reduced specimen thickness z=t/Λ (Λ=total mean-free-path) can either be recorded by angular-resolved EELS or calculated by a convolution of a normalized single-scattering function ϕ(w,θ). For rotational symmetry in angle (amorphous or polycrystalline specimens) this can be realised by the following sequence of operations :(1)where the two-dimensional distribution in angle is reduced to a one-dimensional function by a projection P, T is a two-dimensional Fourier transform in angle θ and energy loss w and the exponent -1 indicates a deprojection and inverse Fourier transform, respectively.


Nano Letters ◽  
2021 ◽  
Author(s):  
Fei Zhou ◽  
Yang Li ◽  
Xingqi Liao ◽  
Shuren Lin ◽  
Haizeng Song ◽  
...  

2009 ◽  
Vol 78 (5) ◽  
pp. 053705 ◽  
Author(s):  
Hiroshi Muranaka ◽  
Yusuke Doi ◽  
Keisuke Katayama ◽  
Hitoshi Sugawara ◽  
Rikio Settai ◽  
...  

1993 ◽  
Vol 07 (23n24) ◽  
pp. 3973-4003 ◽  
Author(s):  
P. FOURY ◽  
J.P. POUGET

The structural instabilities towards the formation of a charge density wave (CDW) ground state exhibited by several layered Mo and W bronzes and oxides are reviewed. It is shown that in these two-dimensional (2D) metals, including the purple bronzes A x Mo 6 O 17 (A=K, Na, Tl; x≈1), the γ and η phases of MO 4 O 11 and the monophosphate tungsten bronzes with pentagonal tunnels ( PO 2)4 ( WO 3)2m(m=4, 6, 7), the CDW instability can be associated with particular chains of MoO 6 or WO 6 octahedra of the ReO 3 type slabs along which there is a strong overlap of the t 2g orbitals. The CDW critical wave vectors of the purple bronzes, Mo 4 O 11 and the tungsten bronzes with m=4 and 6 lead to a common nesting between differently oriented 1D Fermi surfaces. It is suggested that the anharmonic CDW modulation, which occurs in the tungsten bronzes with m≥7, could be the structural fingerprint of electron localization effects.


Author(s):  
А.Н. Афанасьев ◽  
П.С. Алексеев ◽  
А.А. Грешнов ◽  
М.А. Семина

In conductors with a very small density of defects, electrons at low temperatures collide predominantly with a sample edges. Therefore, the ballistic regime of charge and heat transport is realized. The application of a perpendicular magnetic field substantially modifies the character of ballistic transport. For the case of two-dimensional (2D) electrons in the magnetic fields corresponding to the diameter of the cyclotron trajectories smaller than the sample width a hydrodynamic transport regime is formed. In the latter regime, the flow is mainly controlled by rare electron–electron collisions, which determine the viscosity effect. In this work, we study the ballistic flow of 2D electrons in long samples in magnetic fields up to the critical field of the transition to the hydrodynamic regime. From solution of the kinetic equation, we obtain analytical formulas for the profiles of the current density and the Hall electric field far and near the ballistic-hydrodynamic transition as well as for the longitudinal and Hall resistances in these ranges. Our theoretical results, apparently, describe the observed longitudinal resistance of pure graphene samples in the diapason of magnetic fields below the ballistic-hydrodynamic transition.


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