scholarly journals Radioactivity of soil in Croatia I: naturally occurring decay chains

2021 ◽  
Vol 72 (1) ◽  
pp. 6-14
Author(s):  
Marko Šoštarić ◽  
Branko Petrinec ◽  
Mak Avdić ◽  
Ljerka Petroci ◽  
Milica Kovačić ◽  
...  
Keyword(s):  
Gamma Ray ◽  
Internal Exposure ◽  
Gamma Ray Spectrometry ◽  
Systematic Research ◽  
Naturally Occurring ◽  
Activity Concentrations ◽  
Direct Emission ◽  
Uncultivated Soil ◽  
High Concentrations ◽  
Part Presentation

Abstract The assessment of environmental radioactivity much relies on radionuclide content in soil. This stems from the significant contribution of soil to both external and internal exposure to ionising radiation via direct emission of gamma radiation and soil-to-plant radionuclide transfer, respectively. This motivated us to carry out a systematic research on the radioactivity of soil in Croatia to obtain relevant data that can be used as a basis for understanding the related effects of geomorphological, biogeographical, and climatological properties of the environment. We collected samples of the surface layer of uncultivated soil (0–10 cm) at 138 sites from all over the country and measured them for radionuclide activity concentrations by means of high-resolution gamma-ray spectrometry. This resulted in radioactivity maps containing data on activity concentrations of representative radionuclides in the environment. In this paper, which is the first in our two-part presentation, we focus on the naturally occurring 232Th and 238U decay chains and their correlations with the diversity of Croatian regions. For both of the chains, activity concentrations were the highest in the Dinaric region, the lowest in the Pannonian region, and intermediate in the Adriatic region. Relatively high concentrations of 226Ra in the soil of the Dinaric region implied a possibility of an enhanced emanation of its progeny 222Rn into the air. Activity concentrations of 210Pb were additionally elevated in areas with dense vegetation, most probably due to an atmospheric deposition of airborne 210Pb onto the surface of plants and their eventual decomposition on the ground.

scholarly journals Radioactivity of soil in Croatia II: 137Cs, 40K, and absorbed dose rate

2021 ◽  
Vol 72 (1) ◽  
pp. 15-22
Author(s):  
Marko Šoštarić ◽  
Branko Petrinec ◽  
Mak Avdić ◽  
Ljerka Petroci ◽  
Milica Kovačić ◽  
...  
Keyword(s):  
Dose Rate ◽  
Gamma Ray ◽  
Absorbed Dose ◽  
Gamma Ray Spectrometry ◽  
External Exposure ◽  
Vegetation Density ◽  
Absorbed Dose Rate ◽  
Dose Rates ◽  
Activity Concentrations ◽  
Uncultivated Soil

Abstract We took samples of uncultivated soil from the surface layer (0–10 cm) at 138 sites from all over Croatia and measured their radionuclide activity concentrations with high-resolution gamma-ray spectrometry. This second part of our report brings the results on 40K and 137Cs to complement those on the 232Th and 238U decay chains addressed in the first part. Together they give the most complete picture of radioactivity of Croatian soil so far. Activity concentrations of 40K were the highest in the Pannonian region, and there was an opposite trend for 137Cs. We found that the concentrations of 137Cs tended to increase with altitude, annual precipitation, and vegetation density. The concentration ratio of 137Cs and K in soil, which indicates the potential for 137Cs entering food chains via uptake by plants, was the lowest in agriculturally important areas in the east of the Pannonian region. In addition, we used the obtained results on activity concentrations to calculate the related absorbed dose rate as a measure of external exposure to ionising radiation from soil. The sum of the absorbed dose rates for naturally occurring radionuclides and 137Cs showed that external exposure was generally the highest in the Dinaric region and Istrian Peninsula.

BASELINE EVALUATION STUDY OF NATURALLY OCCURRING RADIONUCLIDES IN SOIL SAMPLES FROM VICINITY OF INDIA’S FIRST FAST REACTOR FUEL CYCLE FACILITY (FRFCF), DAE COMPLEX, KALPAKKAM, INDIA

2018 ◽  
Vol 185 (1) ◽  
pp. 87-95 ◽  
Author(s):  
S N Bramha ◽  
H Krishnan ◽  
V Subramanian ◽  
R Baskaran ◽  
B Venkatraman
Keyword(s):  
Fast Reactor ◽  
Gamma Ray ◽  
Fuel Cycle ◽  
Soil Samples ◽  
Reactor Fuel ◽  
Gamma Ray Spectrometry ◽  
Naturally Occurring ◽  
Activity Concentrations ◽  
Naturally Occurring Radionuclides ◽  
Fast Reactor Fuel

Abstract The activity concentration of 238U, 232Th and 40K were measured in the soil samples collected from Fast Reactor Fuel Cycle Facility (FRFCF) site, using high-resolution gamma-ray spectrometry. This study is aimed to establish the baseline data of naturally occurring radionuclides within the site. The average activity concentrations were found to be 416.5, 61.7 and 622.3 Bq kg−1 for 40K, 238U and 232Th, respectively. The activity concentrations and its radiological indices were evaluated and were compared with the international values reported by the United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR). The ratio of 40K/232Th and 40K /238U were calculated, which indicates the presence of 5.79 and 2.69 times more K-bearing minerals as compared with Th and U-bearing minerals in the soil samples, respectively. The study provides baseline information on concentration of radionuclides and background radiological assessment of the FRFCF site.

scholarly journals Inter-comparison exercise utilizing x- and γ-ray spectrometry

2020 ◽  
Vol 27 ◽  
pp. 121
Author(s):  
Filothei K. Pappa ◽  
Christos Tsabaris ◽  
Dionisis Patiris ◽  
Georgios Eleftheriou ◽  
Effrossini G. Androulakaki ◽  
...  
Keyword(s):  
Gamma Ray ◽  
Natural Radionuclides ◽  
Atomic Spectrometry ◽  
Gamma Ray Spectrometry ◽  
Metal Concentrations ◽  
Activity Concentrations ◽  
Great Divergence ◽  
Set Up ◽  
Comparison Exercise ◽  
Good Agreement

Radionuclides are characterized by their nuclear and chemical behavior. Additionally, the geochemical characteristics of radionuclides result in their accumulation in the sediments via sorption processes. In this work the radionuclide activity concentrations obtained by gamma-ray spectrometry (HPGe detector) were converted to metal concentrations as described in [1]. The results were compared with the measured metal concentrations obtained by atomic spectrometry (X-ray fluorescence system-XRF). The samples originate from the coastal environment of two Greek areas, characterized by elevated values of natural radionuclides (e.g. 226Ra) and metals. The preliminary study revealed a good agreement among the concentrations of potassium calculated via activity concentrations of 40K and those of XRF measurement, while a great divergence was observed for the thorium case. These differences can be attributed to the low statistics, as well as to the calibration set-up of Th XRF measurement.

ASSESSMENT OF NATURAL RADIOACTIVITY IN MAIZE AND ESTIMATION OF CONCOMITANT DOSE TO NIGERIAN VIA INGESTION PATHWAY

2019 ◽  
Vol 184 (3-4) ◽  
pp. 359-362
Author(s):  
Mudassir H Yarima ◽  
M U Khandaker ◽  
A Nadhiya ◽  
M A Olatunji
Keyword(s):  
Cancer Risk ◽  
Natural Radioactivity ◽  
Gamma Ray ◽  
Gamma Ray Spectrometry ◽  
Detailed Knowledge ◽  
Dose Limit ◽  
Annual Dose ◽  
Lifetime Cancer Risk ◽  
Environmental Media ◽  
Naturally Occurring

Abstract Uranium, thorium and potassium are the most abundant naturally occurring radioactive materials (NORMs) found in soils and other environmental media including foodstuffs. Since the human exposures to NORMs is an unavoidable phenomenon, in such a way that they can easily find their way to human being via food chain, detailed knowledge on their presence in foodstuffs is necessary to assess the radiation dose to the population. Thus, the present study concerns the assessment of natural radioactivity in maize, a staple foodstuff for Nigerian, via HPGe gamma-ray spectrometry. Activity concentrations (Bq/kg) in the maize samples were found to be in the range of 6.1 ± 0.6–8.2 ± 1.3, 2.2 ± 0.4–5.1 ± 0.7 and 288 ± 16–401 ± 24 for 226Ra, 232Th and 40K, respectively. Measured data for 226Ra and 232Th show below the world average values of 67 Bq/kg and 82 Bq/kg, respectively, while the activity of 40K exceeds the global average of 310 Bq/kg. The annual effective dose via the maize consumption was found to be far below the UNSCEAR recommended ingestion dose limit of 290 μSv/y, and the estimated lifetime cancer risk show lower than the ICRP (1991) cancer risk factor of 2.5 × 10−3 based on the additional annual dose limit of 1 mSv for general public, thus pose no adverse health risk to the Nigerian populace.

scholarly journals Determination of the activity concentration levels of the artificial radionuclide137Cs in soil samples collected from Qatar using high-resolution gamma-ray spectrometry

2016 ◽  
Vol 44 ◽  
pp. 1660237
Author(s):  
Huda Al-Sulaiti ◽  
Tabassum Nasir ◽  
K. S. Al Mugren ◽  
N. Alkhomashi ◽  
N. Al-Dahan ◽  
...  
Keyword(s):  
High Resolution ◽  
Nuclear Power ◽  
Activity Concentration ◽  
Gamma Ray ◽  
Germanium Detector ◽  
Soil Samples ◽  
Gamma Ray Spectrometry ◽  
Activity Concentrations ◽  
High Resolution Gamma

The goal of this study was to establish the first baseline measurements for radioactivity concentration of the artificial radionuclide [Formula: see text]Cs in soil samples collected from the Qatarian peninsula. The work focused on the determination of the activity concentrations levels of man-made radiation in 129 soil samples collected across the landscape of the State of Qatar. All the samples were collected before the most recent accident in Japan, “the 2011 Fukushima Dai-ichi nuclear power plant accident”. The activity concentrations have been measured via high-resolution gamma-ray spectrometry using a hyper-pure germanium detector situated in a low-background environment with a copper inner-plated passive lead shield. A radiological map showing the activity concentrations of [Formula: see text]Cs is presented in this work. The concentration was[Formula: see text]found to range from 0.21 to 15.41 Bq/kg. The highest activity concentration of [Formula: see text]Cs was observed in sample no. 26 in North of Qatar. The mean value was found to be around 2.15 ± 0.27 Bq/kg. These values lie within the expected range relative to the countries in the region. It is expected that this contamination is mainly due to the Chernobyl accident on 26 April 1986, but this conclusion cannot be confirmed because of the lack of data before this accident.

scholarly journals ESTIMATION ON THE RADIOLOGICAL LEVEL OF NATURAL OCCURRING RADIONUCLIDES PRESENT IN FLOODED SOIL SAMPLES IN KADUNA NORTH, NIGERIA

2017 ◽  
Vol 5 (10) ◽  
pp. 81-91
Author(s):  
P.M. Gyuk ◽  
J.O. Anaegbu ◽  
H.O. Aboh ◽  
R. Daniel ◽  
A. Aruwa ◽  
...  
Keyword(s):  
Gamma Ray ◽  
Background Radiation ◽  
Absorbed Dose ◽  
Soil Samples ◽  
Gamma Ray Spectrometry ◽  
Published Data ◽  
Absorbed Dose Rate ◽  
Radium Equivalent Activity ◽  
Activity Concentrations ◽  
Radium Equivalent

The background radiation of the areas was collected at random for each point using a rados survey meter. The detectors (two rados survey meter were used) were placed 1 meter above the ground with the operator positioned a few meters away. Three (3) readings were taking from each detector in other to reduce error or reach accuracy in obtaining the background readings from each randomly selected point where soil samples were later collected. In the current study, the concentration levels of naturally occurring radioactive materials (NORMs) of 40K, 232Th, and 238U in the surface soil samples of selected areas in kigo road new extension Kaduna north, Kaduna in Nigeria were studied. The collected soil samples were analyzed by means of gamma-ray spectrometry. The mean activity concentrations of the natural occurring radionuclides of  226Ra, 232Th and 40K in the soil samples were estimated to be 62, 78.35, 227.17 Bq/kg respectively for kigo road new extension respectively. Radium equivalent activity, absorbed dose rate, annual effective dose equivalent were also calculated for assessment of radiological risk. External hazard value (Hex) is between 0.3163 and 0.9557 and Internal hazard value is between 0.4462 and 1.1618. The worldwide average activity concentrations of 226Ra, 232Th and 40K in soil samples from various studies around the world have values of 37, 30 and 400 Bq/kg respectively [UNSCEAR, 2000]. The values compared well with published data from UNSCEAR shows Ra-226, Th-232 from the location are well above the standards while K-40 below the risk value.

scholarly journals Naturally Occurring Radioactive Materials in Bracelets and Necklaces: Radiological Risk Evaluation

2021 ◽  
Vol 18 (21) ◽  
pp. 11170
Author(s):  
Halmat Jalal Hassan ◽  
Suhairul Hashim ◽  
Noor Zati Hani Abu Hanifah ◽  
Sib Krishna Ghoshal ◽  
Mohamad Syazwan Mohd Sanusi ◽  
...  
Keyword(s):  
Effective Dose ◽  
Gamma Ray ◽  
Annual Effective Dose ◽  
Threshold Model ◽  
Negative Ions ◽  
Radioactive Material ◽  
Gamma Ray Spectrometry ◽  
Radiological Risk ◽  
Naturally Occurring ◽  
Dose Conversion Coefficient

A particular category of jewelry is one involving bracelets and necklaces that are deliberately made to contain naturally occurring radioactive material (NORM)—purveyors making unsubstantiated claims for health benefits from the release of negative ions. Conversely, within the bounds of the linear no-threshold model, long-term use presents a radiological risk to wearers. Evaluation is conducted herein of the radiological risk arising from wearing these products and gamma-ray spectrometry is used to determine the radioactivity levels and annual effective dose of 15 commercially available bracelets (samples B1 to B15) and five necklaces (samples N16 to N20). Various use scenarios are considered; a Geant4 Monte Carlo (Geant4 MC) simulation is also performed to validate the experimental results. The dose conversion coefficient for external radiation and skin equivalent doses were also evaluated. Among the necklaces, sample N16 showed the greatest levels of radioactivity, at 246 ± 35, 1682 ± 118, and 221 ± 40 Bq, for 238U, 232Th, and 40K, respectively. For the bracelets, for 238U and 232Th, sample B15 displayed the greatest level of radioactivity, at 146 ± 21 and 980 ± 71 Bq, respectively. N16 offered the greatest percentage concentrations of U and Th, with means of 0.073 ± 0.0002% and 1.51 ± 0.0015%, respectively, giving rise to an estimated annual effective dose exposure of 1.22 mSv, substantially in excess of the ICRP recommended limit of 1 mSv/year.

scholarly journals A radiological study of some ornamental stones: the bluish granites from Extremadura (Spain)

2012 ◽  
Vol 12 (2) ◽  
pp. 395-401 ◽  
Author(s):  
D. Pereira ◽  
L. Neves ◽  
A. Pereira ◽  
M. Peinado ◽  
J. A. Blanco ◽  
...  
Keyword(s):  
Gamma Ray ◽  
Physical And Mechanical Properties ◽  
Internal Exposure ◽  
Gamma Ray Spectrometry ◽  
Radon Emanation ◽  
Crushed Material ◽  
Ornamental Stone ◽  
Ornamental Stones ◽  
Representative Samples

Abstract. In the area of Trujillo (Extremadura, Spain) we have found a variety of striking bluish and secondary yellow granites outcropping within the Plasenzuela pluton. They are all quarried under different names and are characterized by leucocratic minerals in which a bluish phosphate is dispersed throughout the rock. Their physical and mechanical properties make these granites a perfect option for most applications as ornamental rocks. Within the pluton the radiological background is fairly homogeneous, with no significant differences between the gamma ray fluxes of the different facies. U (6.4 ± 0.51 ppm), Th (2.9 ± 0.47 ppm) and K2O (4.32 ± 0.26%) contents determined in the laboratory by gamma-ray spectrometry from representative samples are in good accordance with fast in situ measurements carried out with the same technique and also with conventional chemical analysis. Estimated activities for K-40, Ra-226 and Th-232 were, on average, 1022 ± 36 Bq kg−1, 84 ± 9 Bq kg−1 and 6.8 ± 1.6 Bq kg−1. On the basis of these results, the I index of EU technical document 112 was determined, with an average result of 0.66 ± 0.03. This suggests that the rock can be used with no restrictions for all types of construction purposes. Striking differences were observed between the blue facies and the yellow facies in radon exhalation tests from crushed material (0.03 Bq kg−1 vs. 0.20 Bq kg−1). Since both granites have similar uranium contents (6.3 ppm and 6.5 ppm, respectively), these results can probably be explained in terms of important differences in the mineralogical distribution of this chemical element, radon emanation being enhanced in the yellow facies. However, due to the ordinary use as ornamental stone, the yellow facies does not present a radiological risk in terms of excess effective dose due to internal exposure to radon.

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