scholarly journals A Modified Sequential Deposition Route for High-Performance Carbon-Based Perovskite Solar Cells under Atmosphere Condition

Molecules ◽  
2022 ◽  
Vol 27 (2) ◽  
pp. 481
Author(s):  
Jinyu Wu ◽  
Lei Zhang ◽  
Qiao Kang ◽  
Hongxi Shi ◽  
Long Li ◽  
...  

Carbon-based hole transport material (HTM)-free perovskite solar cells have exhibited a promising commercialization prospect, attributed to their outstanding stability and low manufacturing cost. However, the serious charge recombination at the interface of the carbon counter electrode and titanium dioxide (TiO2) suppresses the improvement in the carbon-based perovskite solar cells’ performance. Here, we propose a modified sequential deposition process in air, which introduces a mixed solvent to improve the morphology of lead iodide (PbI2) film. Combined with ethanol treatment, the preferred crystallization orientation of the PbI2 film is generated. This new deposition strategy can prepare a thick and compact methylammonium lead halide (MAPbI3) film under high-humidity conditions, which acts as a natural active layer that separates the carbon counter electrode and TiO2. Meanwhile, the modified sequential deposition method provides a simple way to facilitate the conversion of the ultrathick PbI2 capping layer to MAPbI3, as the light absorption layer. By adjusting the thickness of the MAPbI3 capping layer, we achieved a power conversation efficiency (PCE) of 12.5% for the carbon-based perovskite solar cells.

RSC Advances ◽  
2020 ◽  
Vol 10 (59) ◽  
pp. 35831-35839 ◽  
Author(s):  
Mustafa K. A. Mohammed

Carbon-based perovskite solar cells (C-PSCs) are the most promising photovoltaic (PV) due to their low material and manufacturing cost and superior long-term stability.


2021 ◽  
Author(s):  
Hamed Moeini Alishah ◽  
Fatma Pinar Gokdemir Choi ◽  
Serap Gunes

Abstract Inverted-type perovskite solar cells have drawn remarkable attention due to solution-processable, straightforward configuration, low-cost processing, and manufacturing at very high throughput, even on top of flexible materials. The hole transport material (HTM) plays a vital role to achieve high performance in inverted type of perovskite solar cells. Herein, we report on the effect of different commercial PEDOT: PSS such as PH 1000, PH 500, P VP AI, and P T2, on the performance of CH3NH3PbI3 based planar perovskite solar cells.


Author(s):  
Yan Yang ◽  
Wangen Zhao ◽  
Tengteng Yang ◽  
Jiali Liu ◽  
Jingru Zhang ◽  
...  

Guanidinium thiocyanate was selected to modify the surface terminations of methylamine lead iodide (MAPbI3) perovskite films and a 21.26% PCE was acquired for a solar cell based on the MAPbI3 system, and the voltage deficit is reduced to 0.426 V.


2018 ◽  
Vol 246 ◽  
pp. 195-203 ◽  
Author(s):  
Dian Wang ◽  
Naveen Kumar Elumalai ◽  
Md Arafat Mahmud ◽  
Haimang Yi ◽  
Mushfika Baishakhi Upama ◽  
...  

2020 ◽  
Vol 8 (25) ◽  
pp. 12723-12734 ◽  
Author(s):  
Yang Yang ◽  
Minh Tam Hoang ◽  
Disheng Yao ◽  
Ngoc Duy Pham ◽  
Vincent Tiing Tiong ◽  
...  

Carbon electrode-based planar PSCs demonstrated higher device performance and reduced hysteresis using a CuSCN based HTL owing to its favourable energy level alignment with the perovskite compared to conventional spiro-OMeTAD based HTL.


2019 ◽  
Vol 12 (1) ◽  
pp. 230-237 ◽  
Author(s):  
E. Yalcin ◽  
M. Can ◽  
C. Rodriguez-Seco ◽  
E. Aktas ◽  
R. Pudi ◽  
...  

Herein, we studied the use of two different Self Assembled Monolayers (SAMs) made of semiconductor hole transport organic molecules to replace the most common p-type contact, PEDOT:PSS, in PiN methyl ammonium lead iodide perovskite solar cells (PSCs).


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