Continuous-flow synthesis of ultrahigh luminescent perovskite nanocrystals using forced thin film reactor and application for light-emitting diodes

Author(s):  
Kazuki Umemoto ◽  
Masaaki Yokoyama ◽  
Keisuke Kikuchi ◽  
Taisei Kimura ◽  
Naoaki Oshita ◽  
...  

Abstract Owing to their excellent optical properties, organolead halide perovskite nanocrystals (PeNCs) have gained significant attention. Considering their industrial contribution, exploring practical production of high-quality PeNCs is of major importance. In this work, we demonstrate continuous-flow synthesis of ultrahigh luminescent PeNCs with high color purity using a forced thin film reactor. We successfully demonstrate the effectiveness of this reactor as a crystal growth environment. The photoluminescence quantum yields were improved to 94% as a result of the unique mixing process. After film formation, this reactor enabled the application for perovskite light-emitting diodes.

1999 ◽  
Author(s):  
Eli Yablonovitch ◽  
Misha Boroditsky ◽  
Rutger Vrijen ◽  
Thomas F. Krauss ◽  
Roberto Coccioli

2021 ◽  
Vol 10 (1) ◽  
Author(s):  
Li Zhang ◽  
Changjiu Sun ◽  
Tingwei He ◽  
Yuanzhi Jiang ◽  
Junli Wei ◽  
...  

AbstractQuasi-two-dimensional (quasi-2D) perovskites have attracted extraordinary attention due to their superior semiconducting properties and have emerged as one of the most promising materials for next-generation light-emitting diodes (LEDs). The outstanding optical properties originate from their structural characteristics. In particular, the inherent quantum-well structure endows them with a large exciton binding energy due to the strong dielectric- and quantum-confinement effects; the corresponding energy transfer among different n-value species thus results in high photoluminescence quantum yields (PLQYs), particularly at low excitation intensities. The review herein presents an overview of the inherent properties of quasi-2D perovskite materials, the corresponding energy transfer and spectral tunability methodologies for thin films, as well as their application in high-performance LEDs. We then summarize the challenges and potential research directions towards developing high-performance and stable quasi-2D PeLEDs. The review thus provides a systematic and timely summary for the community to deepen the understanding of quasi-2D perovskite materials and resulting LED devices.


2011 ◽  
Vol 14 (11) ◽  
pp. H460 ◽  
Author(s):  
Surani Bin Dolmanan ◽  
Siew Lang Teo ◽  
Vivian Kaixin Lin ◽  
Hui Kim Hui ◽  
Armin Dadgar ◽  
...  

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