Probing the Purcell effect without radiative decay: Lessons in the frequency and time domains

The effect of cavities or plates upon the electromagnetic quantum vacuum are considered in the context of electro-optic sampling, revealing how they can be directly studied. These modifications are at the heart of e.g. the Casimir force or the Purcell effect such that a link between electro-optic sampling of the quantum vacuum and environment-induced vacuum effects is forged. Furthermore, we discuss the microscopic processes underlying electro-optic sampling of quantum-vacuum fluctuations, leading to an interpretation of these experiments in terms of exchange of virtual photons. With this in mind it is shown how one can reveal the dynamics of vacuum fluctuations by resolving them in the frequency and time domains using electro-optic sampling experiments.

Photonic Cavity Effects for Enhanced Efficiency in Layered Perovskite-Based Light-Emitting Diodes

Layered architectures for light-emitting diodes (LEDs) are the standard approach for solution-processable materials such as metal-halide perovskites. Upon designing the composition and thicknesses of the layers forming the LED, the primary focus is typically on the optimization of charge injection and balance. However, this approach only considers the process until electrons and holes recombine to generate photons, while for achieving optimized LED performance, the generated light must also be efficiently outcoupled. Our work focuses on the latter aspect. We assume efficient photon generation and analyze the effects of the geometrical configuration together with the dipole orientation, mimicking the light emission, on the main characteristics defining the LED, such as the Purcell effect and the outcoupling efficiency. We find that in-plane dipoles result in significantly increased outcoupling efficiency. Furthermore, the mismatch in refractive index among the layers and their different thicknesses can be tuned to maximize the Purcell effect and minimize internal losses. The combined optimization of dipole orientation and layer thicknesses can improve the efficiency of the LED up to a factor 10, hence highlighting the importance of considering also the photonic properties of the LED structures if the objective is to maximize the LED performance.

Free-electron Driven Terahertz Wave Sources Based on Simth-Purcell Effect

Terahertz electromagnetic wave is one of the hottest research topics in nowadays scientific world thanks to its broad applications in material characterization, medical imaging, wireless communication, and security checking etc. Using free-electron beams to interact with periodic structures via the famous Smith-Purcell effect is an efficient way of generating high-power terahertz radiation. In this chapter, we introduce the basic theory and latest developments of the terahertz radiation schemes using a free-electron beam (including continuous electron beam, a single electron bunch, and a train of electron bunches, etc.) to interact with periodic electromagnetic structures, including grating, surface plasmonics, and subwavelength hole arrays, via a special Smith-Purcell effect or Cherenkov-like effect. A kind of free-electron lasers based on the special Smith-Purcell radiation in the terahertz region is proposed and investigated, which can be developed as high-power terahertz wave sources for practical applications.

A numerical study of plasmon-induced enhancement of dipole emission by arrays of silver nanospheres and nanoprisms

Plasmon-induced enhancement of the photoluminescence (PL) intensity of quantum emitters by plasmon nanoparticles (PNPs) is a promising approach for the design and fabrication of PL hybrid materials with improved properties for biosensing and optoelectronics applications. This enhancement can be achieved through careful selection of such parameters as the PNP’s shape, material, size, the type of the medium around them, as well as the excitation and emission wavelengths of the emitter. Here, we simulated the nano-hybrid materials based on arrays of silver nanospheres, nanoprisms, and their combinations, located on polymer films with embedded dipole emitters. For these systems, the Purcell effect, as well as the excitation enhancement, transmittance, and absorption were evaluated. The results show the way to improve the PL properties of thin hybrid films by careful design of their composition using developed models.