Polarisation-dependent single-pulse ultrafast optical switching of an elementary ferromagnet

The ultimate control of magnetic states of matter at femtosecond (or even faster) timescales defines one of the most pursued paradigm shifts for future information technology. In this context, ultrafast laser pulses developed into extremely valuable stimuli for the all-optical magnetization reversal in ferrimagnetic and ferromagnetic alloys and multilayers, while this remains elusive in elementary ferromagnets. Here we demonstrate that a single laser pulse with sub-picosecond duration can lead to the reversal of the magnetization of bulk nickel, in tandem with the expected demagnetization. As revealed by realistic time-dependent electronic structure simulations, the central mechanism involves ultrafast light-induced torques that act on the magnetization. They are only effective if the laser pulse is circularly polarized on a plane that contains the initial orientation of the magnetization. We map the laser pulse parameter space enabling the magnetization switching and unveil rich intra-atomic orbital-dependent magnetization dynamics featuring transient inter-orbital non-collinear states. Our findings open further perspectives for the efficient implementation of optically-based spintronic devices.

Self-supported ultrathin plasmonic film for ultrafast optical switching

Self-supporting gold nanowire (AuNW) gratings with a thickness of about 200 nm are produced by solution-processing and flexible-transfer techniques. Such an ultrathin structure is applied as an ultrafast optical switch...

Maintaining Constant Pulse-Duration in Highly Dispersive Media Using Nonlinear Potentials

A method is shown for preventing temporal broadening of ultrafast optical pulses in highly dispersive and fluctuating media for arbitrary signal-pulse profiles. Pulse pairs, consisting of a strong-field control-pulse and a weak-field signal-pulse, co-propagate, whereby the specific profile of the strong-field pulse precisely compensates for the dispersive phase in the weak pulse. A numerical example is presented in an optical system consisting of both resonant and gain dispersive effects. Here, we show signal-pulses that do not temporally broaden across a vast propagation distance, even in the presence of dispersion that fluctuates several orders of magnitude and in sign (for example, within a material resonance) across the pulse’s bandwidth. Another numerical example is presented in normal dispersion telecom fiber, where the length at which an ultrafast pulse does not have significant temporal broadening is extended by at least a factor of 10. Our approach can be used in the design of dispersion-less fiber links and navigating pulses in turbulent dispersive media. Furthermore, we illustrate the potential of using cross-phase modulation to compensate for dispersive effects on a signal-pulse and fill the gap in the current understanding of this nonlinear phenomenon.

Real-time ultrafast oscilloscope with a relativistic electron bunch train

The deflection of charged particles is an intuitive way to visualize an electromagnetic oscillation of coherent light. Here, we present a real-time ultrafast oscilloscope for time-frozen visualization of a terahertz (THz) optical wave by probing light-driven motion of relativistic electrons. We found the unique condition of subwavelength metal slit waveguide for preserving the distortion-free optical waveform during its propagation. Momentary stamping of the wave, transversely travelling inside a metal slit, on an ultrashort wide electron bunch enables the single-shot recording of an ultrafast optical waveform. As a proof-of-concept experiment, we successfully demonstrated to capture the entire field oscillation of a THz pulse with a sampling rate of 75.7 TS/s. Owing to the use of transversely-wide and longitudinally-short electron bunch and transversely travelling wave, the proposed “single-shot oscilloscope” will open up new avenue for developing the real-time petahertz (PHz) metrology.

Multi-mJ Scaling of 5-Optical Cycle, 3 µm OPCPA

We present the design of an ultrafast optical parametric chirped pulse amplifier (OPCPA) operating at 3 µm yielding few-cycle pulses and multi-mJ output energy. This design demonstrates that with a configuration of a single crystal or combination of crystals (KTA and MgO:LN) it is possible to achieve output energies above the mJ with sufficient bandwidth to allow compression to just 5-optical cycles. Here, we consider a 1 µm mJ-level picosecond chirped pulse amplifier (CPA), a typical pumping source for this type of non-linear amplifiers. Compression with a simple bulk material enables reaching close to the pulse Fourier-transform limited duration, paving the way to high energy, ultrafast mid-infrared pulses.

Spatiotemporal observation of light propagation in a three-dimensional scattering medium

Spatiotemporal information about light pulse propagation obtained with femtosecond temporal resolution plays an important role in understanding transient phenomena and light–matter interactions. Although ultrafast optical imaging techniques have been developed, it is still difficult to capture light pulse propagation spatiotemporally. Furthermore, imaging through a three-dimensional (3-D) scattering medium is a longstanding challenge due to the optical scattering caused by the interaction between light pulse and a 3-D scattering medium. Here, we propose a technique for ultrafast optical imaging of light pulses propagating inside a 3D scattering medium. We record an image of the light pulse propagation using the ultrashort light pulse even when the interaction between light pulse and a 3-D scattering medium causes the optical scattering. We demonstrated our proposed technique by recording converging, refracted, and diffracted propagating light for 59 ps with femtosecond temporal resolution.