In quantum information processing, spin-3/2 electron or nuclear spin states are known as two-qubit states. For SI (S = 3/2, I = 1/2) spin system, there are eight three-qubit states. In this study, first, three-qubit CNOT logic gates are obtained. Then three-qubit entangled states are obtained by using the matrix representation of Hadamard and three-qubit CNOT logic gates. By considering single 31P@C60 molecule as SI (S = 3/2, I = 1/2) spin system, three-qubit entangled states are also obtained using the magnetic resonance pulse sequences of Hadamard and CNOT logic gates.