Light-emitting diodes with optoelectronic feedback loop display complex sequences of periodic mixed mode oscillations and chaotic spiking. In this paper, we propose an adaptive neural control scheme for chaos synchronization of two unidirectional coupled LED systems. Based on Lyapunov stability theory, the controller can stabilize the synchronization error dynamics at the origin point, thus chaos synchronization can be obtained. The simulation results demonstrate the effectiveness of the proposed control scheme.