scholarly journals Electronic Energy Transfer and Quantum Coherence in Photosynthetic Light Harvesting

2013 ◽  
Vol 41 (6) ◽  
pp. 391
Author(s):  
Akihito ISHIZAKI
2014 ◽  
Vol 93 ◽  
pp. 225-234
Author(s):  
Elisabetta Collini

One of the most surprising and significant advances in the study of the photosynthetic light-harvesting process is the discovery that the electronic energy transfer (ET) might involve long-lived electronic coherences, also at physiologically relevant conditions. This means that the transfer of energy among different chromophores does not follow the expected classical incoherent hopping mechanism, but that quantum-mechanical laws can steer the migration of energy. The implications of such quantum transport regime, although currently under debate, might have a tremendous impact in our way to think about natural and artificial light-harvesting and suggest new directions for the development of artificial devices for the efficient capture and re-use of solar energy. Central to these discoveries has been the development of new ultrafast spectroscopic techniques, in particular two-dimensional electronic spectroscopy, which is now the primary tool to obtain clear and definitive experimental proof of such effects.


2014 ◽  
Vol 53 (49) ◽  
pp. 13609-13613 ◽  
Author(s):  
Christian B. Winiger ◽  
Shaoguang Li ◽  
Ganesh R. Kumar ◽  
Simon M. Langenegger ◽  
Robert Häner

2007 ◽  
Vol 111 (25) ◽  
pp. 6978-6982 ◽  
Author(s):  
Gregory D. Scholes ◽  
Carles Curutchet ◽  
Benedetta Mennucci ◽  
Roberto Cammi ◽  
Jacopo Tomasi

2010 ◽  
Vol 12 (27) ◽  
pp. 7319 ◽  
Author(s):  
Akihito Ishizaki ◽  
Tessa R. Calhoun ◽  
Gabriela S. Schlau-Cohen ◽  
Graham R. Fleming

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