Isolation and purification of the xenon fraction of 252Cf spontaneous fission products for the production of radioactive xenon calibration standards

2015 ◽  
Vol 307 (3) ◽  
pp. 2557-2562
Author(s):  
T. P. Houghton ◽  
C. A. Mcgrath ◽  
R. K. Hague ◽  
J. G. Eisenmenger ◽  
T. A. Robinson
1985 ◽  
Vol 91 (2) ◽  
pp. 291-296
Author(s):  
B. S. Tomar ◽  
H. Naik ◽  
A. Ramaswamy ◽  
Satya Prakash

2020 ◽  
Vol 239 ◽  
pp. 05003
Author(s):  
R. Vogt ◽  
J. Randrup ◽  
P. Talou ◽  
J. T. Van Dyke ◽  
L. A. Bernstein

For many years, the state of the art for simulating fission in transport codes amounted to sampling from average distributions. However, such "average" fission models have limited capabilities. Energy is not explicitly conserved and no correlations are available because all particles are emitted independently. However, in a true fission event, the emitted particles are correlated. Recently, Monte Carlo codes generating complete fission events have been developed, thus allowing the use of event-by-event analysis techniques. Such techniques are particularly useful because the complete kinematic information is available for the fission products and the emitted neutrons and photons. It is therefore possible to extract any desired observables, including correlations. The fast event-by-event fission code FREYA (Fission Reaction Event Yield Algorithm) generates large samples of complete fission events, employing only a few physics-based parameters. A recent optimization of these parameters for the isotopes in FREYA that undergo spontaneous fission is described and results are presented. The sensitivity of neutron observables in FREYA to the input yield functions is also discussed and the correlation between the average neutron multiplicity and fragment total kinetic energy is quantified.


Atomic Energy ◽  
2010 ◽  
Vol 108 (1) ◽  
pp. 46-52
Author(s):  
A. V. Bushuev ◽  
A. F. Kozhin ◽  
T. B. Aleeva ◽  
V. N. Zubarev ◽  
A. F. Myrzin ◽  
...  

2014 ◽  
Author(s):  
Ted W. Bowyer ◽  
Christopher J. Gesh ◽  
Derek A. Haas ◽  
James C. Hayes ◽  
Lenna A. Mahoney ◽  
...  

1960 ◽  
Vol 38 (1) ◽  
pp. 1-9 ◽  
Author(s):  
B. G. Young ◽  
H. G. Thode

The absolute abundances of the isotopes of fission-product xenon and krypton in six uranium minerals have been determined mass spectrometrically using the isotope dilution technique. The fission products were resolved into a U238 spontaneous fission component, a U235 neutron-induced fission component, and a U238 neutron-induced fission component. Internal consistency in the analysis was achieved only when the Xe129 yield used for the U235 thermal neutron fission component was 20% lower than that reported by Purkayastha and Martin at I129. This discrepancy in the mass 129 chain yield measured at I129 and at Xe129 has not been resolved.Only one of the six minerals, Cinch Lake pitchblende, retained essentially all of its fission product inert gases throughout geological time. Inert gas losses from the remaining five minerals ranged from 20% to 75%. The absolute yields of the stable xenon and krypton fission products in U238 spontaneous fission were determined from an analysis of the inert gases from the Cinch Lake mineral. This analysis showed that 95.9% of the fission gas in this case resulted from the spontaneous fission and only 4.1% from neutron-induced fission.


2019 ◽  
Vol 107 (7) ◽  
pp. 555-560 ◽  
Author(s):  
Heinz W. Gäggeler ◽  
Ilya Usoltsev ◽  
Robert Eichler

Abstract Fission products recoiling from a 252Cf spontaneous fission source were stopped in various mixtures of inert gases containing CO and NO. For the elements of the transisition metal series Mo, Tc, Ru, and Rh previous observations of pure carbonyl complexes were reproduced. However, no formation of volatile mixed nitrosyl-carbonyl complexes or pure nitrosyl complexes for these elements have been observed. Instead, efficient production of volatile nitrosyl compounds for single iodine atoms, presumably nitrosyl iodide, NOI, was detected. This observation is of interest as potential transport path for iodine in nuclear accident scenarios and as a model for radiochemistry with the recently discovered heaviest halogen tennessine (Z=117).


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