scholarly journals Supplementary material to "Comparison of different Aethalometer correction schemes and a reference multi-wavelength absorption technique for ambient aerosol data"

Author(s):  
Jorge Saturno ◽  
Christopher Pöhlker ◽  
Dario Massabò ◽  
Joel Brito ◽  
Samara Carbone ◽  
...  
2016 ◽  
Author(s):  
Jorge Saturno ◽  
Christopher Pöhlker ◽  
Dario Massabò ◽  
Joel Brito ◽  
Samara Carbone ◽  
...  

Abstract. Deriving absorption coefficients from Aethalometer attenuation data requires different corrections to compensate for artifacts related to filter-loading effects, scattering by filter fibers, and scattering by aerosol particles. In this study, two different correction schemes were applied to 7-wavelength Aethalometer data, using Multi-Angle Absorption Photometer (MAAP) data as a reference absorption measurement at 637 nm. The compensation algorithms were compared to 5-wavelength offline absorption measurements obtained with a Multi-Wavelength Absorbance Analyzer (MWAA), which serves as a multiple-wavelength reference measurement. The online measurements took place in the Amazon rainforest, from the wet-to-dry transition season to the dry season (June–September 2014). The mean absorption coefficient (at 637 nm) during this period was 1.8 ± 2.1 Mm−1, with a maximum of 15.9 Mm−1. Under these conditions, the filter-loading compensation was negligible. One of the correction schemes was found to artificially increase the short-wavelength absorption coefficients. It was found that accounting for the aerosol optical properties in the scattering compensation significantly affects the absorption Ångström exponent (AAE) retrievals. Proper Aethalometer data compensation schemes are crucial to retrieve the correct AAE, which is commonly implemented in brown carbon contribution calculations. We found that a "hybrid" algorithm was more appropriate to achieve optimal correlations with the MAAP absorption coefficients and with the AAE retrieved from offline MWAA measurements.


2021 ◽  
Vol 227 ◽  
pp. 147-161
Author(s):  
Jérôme Yon ◽  
Juan José Cruz ◽  
Felipe Escudero ◽  
José Morán ◽  
Fengshan Liu ◽  
...  

2017 ◽  
Vol 10 (8) ◽  
pp. 2837-2850 ◽  
Author(s):  
Jorge Saturno ◽  
Christopher Pöhlker ◽  
Dario Massabò ◽  
Joel Brito ◽  
Samara Carbone ◽  
...  

Abstract. Deriving absorption coefficients from Aethalometer attenuation data requires different corrections to compensate for artifacts related to filter-loading effects, scattering by filter fibers, and scattering by aerosol particles. In this study, two different correction schemes were applied to seven-wavelength Aethalometer data, using multi-angle absorption photometer (MAAP) data as a reference absorption measurement at 637 nm. The compensation algorithms were compared to five-wavelength offline absorption measurements obtained with a multi-wavelength absorbance analyzer (MWAA), which serves as a multiple-wavelength reference measurement. The online measurements took place in the Amazon rainforest, from the wet-to-dry transition season to the dry season (June–September 2014). The mean absorption coefficient (at 637 nm) during this period was 1.8 ± 2.1 Mm−1, with a maximum of 15.9 Mm−1. Under these conditions, the filter-loading compensation was negligible. One of the correction schemes was found to artificially increase the short-wavelength absorption coefficients. It was found that accounting for the aerosol optical properties in the scattering compensation significantly affects the absorption Ångström exponent (åABS) retrievals. Proper Aethalometer data compensation schemes are crucial to retrieve the correct åABS, which is commonly implemented in brown carbon contribution calculations. Additionally, we found that the wavelength dependence of uncompensated Aethalometer attenuation data significantly correlates with the åABS retrieved from offline MWAA measurements.


2018 ◽  
Author(s):  
Sara D. Forestieri ◽  
Taylor M. Helgestad ◽  
Andrew Lambe ◽  
Lindsay Renbaum-Wolff ◽  
Daniel A. Lack ◽  
...  

2019 ◽  
Vol 27 (16) ◽  
pp. 23576 ◽  
Author(s):  
Guangsheng Deng ◽  
Xianglian Song ◽  
Sina Abedini Dereshgi ◽  
Haiqing Xu ◽  
Koray Aydin

2000 ◽  
Vol 123 (6) ◽  
pp. 1093-1097 ◽  
Author(s):  
Yudaya Sivathanu ◽  
Anthony Hamins ◽  
George Mulholland ◽  
Takashi Kashiwagi ◽  
Robert Buch

The optical properties of particulate emitted from fires burning two distinct polydimethylsiloxane fluids (D4 and M2 or MM, where D=CH32SiO and M=CH33SiO2) were obtained using a transmission cell-reciprocal nephelometer in conjunction with gravimetric sampling. The specific absorption coefficient of particulate ash from fires burning D4 and MM is significantly lower than that of particulate soot from an acetylene (hydrocarbon) flame. Scattering is the dominant part of extinction in fires burning the silicone fluids. This is very different from extinction by soot particles in hydrocarbon fires, where absorption is approximately five times greater than scattering. Temperatures and particulate volume fractions along the axis of a silicone fire D4 were measured using multi-wavelength absorption/emission spectroscopy. The structure of the D4 flames is markedly different from hydrocarbon flames. The temperatures and particulate volume fractions very close to the burner surface are much higher than in comparably sized hydrocarbon flames.


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