Delayed neutron measurements with a natural uranium fission product source in Fast Breeder Test Reactor

2014 ◽  
Vol 65 ◽  
pp. 314-319 ◽  
Author(s):  
G. Srinivasan ◽  
R.S. Keshavamurthy ◽  
D.V. Subramanian ◽  
Adish Haridas ◽  
C.P. Reddy ◽  
...  
1996 ◽  
Vol 122 (3) ◽  
pp. 359-365 ◽  
Author(s):  
P. Mohanakrishnan ◽  
C. P. Reddy ◽  
V. Gopalakrishnan ◽  
John Arul

2021 ◽  
Vol 372 ◽  
pp. 110992
Author(s):  
Neethu Hanna Stephen ◽  
C.P. Reddy ◽  
G. Raghukumar ◽  
K. Dinesh ◽  
K.V. Suresh Kumar

Author(s):  
S. Varatharajan ◽  
K. V. Sureshkumar ◽  
K. V. Kasiviswanathan ◽  
G. Srinivasan

The second stage of Indian nuclear programme envisages the deployment of fast reactors on a large scale for the effective use of India’s limited uranium reserves. The Fast Breeder Test Reactor (FBTR) at Kalpakkam is a loop type, sodium cooled fast reactor, meant as a test bed for the fuels and structural materials for the Indian fast reactor programme. The reactor was made critical with a unique high plutonium MK-I carbide fuel (70% PuC+30%UC). Being a unique untested fuel of its kind, it was decided to test it as a driver fuel, with conservative limits on Linear Heat Rating and burn-up, based on out-of-pile studies. FBTR went critical in Oct 1985 with a small core of 23 MK-I fuel subassemblies. The Linear Heat Rating and burn-up limits for the fuel were conservatively set at 250 W/cm & 25 GWd/t respectively. Based on out-of-pile simulation in 1994, it was possible to raise the LHR to 320 W/cm. It was decided that when the fuel reaches the target burn-up of 25 GWd/t, the MK-I core would be progressively replaced with a larger core of MK-II carbide fuel (55% PuC+45%UC). Induction of MK-II subassemblies was started in 1996. However, based on the Post-Irradiation Examination (PIE) of the MK-I fuel at 25, 50 & 100 GWd/t, it became possible to enhance the burn-up of the MK-I fuel to 155 GWd/t. More than 900 fuel pins of MK-I composition have reached 155 GWd/t without even a single failure and have been discharged. One subassembly (61 pins) was taken to 165 GWd/t on trial basis, without any clad failure. The core has been progressively enlarged, adding MK-I subassemblies to compensate for the burn-up loss of reactivity and replacement of discharged subassemblies. The induction of MK-II fuel was stopped in 2003. One test subassembly simulating the composition of the MOX fuel (29% PuO2) to be used in the 500 MWe Prototype Fast Breeder Reactor was loaded in 2003. It is undergoing irradiation at 450 W/cm, and has successfully seen a burn-up of 92.5 GWd/t. In 2006, it was proposed to test high Pu MOX fuel (44% PuO2), in order to validate the fabrication and fuel cycle processes developed for the power reactor MOX fuel. Eight MOX subassemblies were loaded in FBTR core in 2007. The current core has 27 MK-I, 13 MK-II, eight high Pu MOX and one power reactor MOX fuel subassemblies. The reactor power has been progressively increased from 10.5 MWt to 18.6 MWt, due to the progressive enlargement of the core. This paper presents the evolution of the core based on the progressive enhancement of the burn-up limit of the unique high Pu carbide fuel.


2008 ◽  
Vol 35 (12) ◽  
pp. 2332-2337 ◽  
Author(s):  
M. Ramakrishnan ◽  
A. John Arul ◽  
S. Usha ◽  
C. Senthil Kumar

Author(s):  
Indra Saptiama ◽  
Herlina Herlina ◽  
Sriyono Sriyono ◽  
E. Sarmini ◽  
Abidin Abidin ◽  
...  

PEMBUATAN RADIONUKLIDA MOLIBDENUM-99 (99Mo) HASIL AKTIVASI NEUTRON DARI MOLIBDENUM ALAM UNTUK MEMPEROLEH TEKNESIUM-99m (99mTc). Pembatasan penggunaan uranium sebagai target untuk produksi 99mTc menyebabkan rumah sakit di Indonesia  kesulitan mendapatkan pasokan 99mTc. Saat ini 99mTc diperoleh dari 99Mo hasil fisi (pembelahan uranium).  Pembuatan radionuklida 99Mo dari aktivasi neutron  molibdenum alam (MoO3) di teras reaktor G.A Siwabessy digunakan sebagai metode alternatif untuk memperoleh 99mTc. Tujuan penelitian ini adalah untuk melakukan pembuatan radionuklida 99Mo dari aktivasi neutron molibdenum alam untuk memperoleh 99mTc. Serbuk MoO3 alam sebanyak 5 gram dikemas dalam ampul kuarsa dan dimasukkan ke dalam inner capsul selanjutnya dikemas menggunakan outer capsul sebagai bahan target. Bahan target diiradiasi di reaktor G.A Siwabessy selama 100 jam. Hasil perhitungan diperoleh aktivitas  99Mo sebesar 65 % dari nilai maksimum yang dapat diperoleh. MoO3 paska iradiasi dilarutkan dengan NaOH 4 M sehingga diperoleh larutan natrium molibdat (Na2MoO4). Radionuklida 99Mo dan 99mTc diukur menggunakan spektrometer gamma. Radionuklida 99Mo terdeteksi dalam produk larutan  Na2MoO4 dengan  aktivitas jenis 99Mo yang diperoleh sebesar 0,81 Ci 99Mo/g Mo.  Radionuklida anak luruh 99mTc dipisahkan dari radionuklida induk 99Mo menggunakan kolom pemisah yang berisi material berbasis zirkonium (MBZ) sebagai penyerap 99Mo. Radionuklida 99mTc hasil pemisahan diperoleh dalam bentuk natrium pertehnetat (Na99mTcO4).dengan recovery yang masih rendah yaitu sekitar 52 hingga 71 %.Kata kunci: Molibdenum, teknesium, radionuklida, pemisahan, iradiasi. PRODUCTION OF ACTIVATED  NEUTRON MOLYBDENUM-99 (99Mo) RADIONUCLIDE FROM NATURAL MOLYBDENUM TO OBTAIN TECHNETIUM-99m (99mTc).  Uranium usage restriction causes the hospitals in indonesia difficult to obtain the suply of  99mTc. At Present, 99mTc is obtanied from molybdenum as a uranium fission product. Production of 99Mo radionuclide resulted from neutron activated natural molybdenum (MoO3) in G.A Siwabessy reactor could be used  as a alternatif method for producing 99mTc. The aim of this research is synthesize of   99Mo radionuclide from neutron activated natural molybdenum  (MoO3) to obtain 99mTc. The five grams of  MoO3 powder was packed in a quartz ampule and inserted into inner capsule then also inserted into outer capsule as a target material. It was iradiated in G.A Siwabessy reactor for 100hours. Based on theoritical calculation, about 65 % of maximum 99Mo activity could be recovered. After Irradiation,  MoO3 was dissolved by NaOH 4 M solution so it was natrium molybdate (Na2MoO4) solution. 99Mo and 99mTc radionuclide were analyzed using gamma spectrometer. 99Mo radionuclide was detected on Na2MoO4 solution as product that had specific activity of 0.81 Ci 99Mo/ g Mo. 99mTc as daughter radionuclide was separated from 99Mo as parent radionuclide using separated column containing zirconium based material (ZBM) as 99Mo adsobent. 99mTc radionuclide has been succesfully separated using ZBM column although recovery of 99mTc  was quite low in which approximately 52 to 71 %. The 99mTc radionuclide was recovered in the form of sodium pertechnetate (NaTcO4) solution.Keywords: Molybdenum, technetium, radionuclide, separation, irradiation.


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