Gas diffusion layer/flow-field unified membrane-electrode assembly in fuel cell using graphene foam

2019 ◽  
Vol 323 ◽  
pp. 134808 ◽  
Author(s):  
Ji Eun Park ◽  
Jongkoo Lim ◽  
Myung Su Lim ◽  
Sungjun Kim ◽  
Ok-Hee Kim ◽  
...  
2021 ◽  
Vol 12 (3) ◽  
pp. 148
Author(s):  
Qinwen Yang ◽  
Shujun Chen ◽  
Gang Xiao ◽  
Lexi Li

A collaborative design for the uneven distributions of a flow channel, gas diffusion layer porosity and catalyst layer porosity are newly proposed to improve the utilization ratio of the membrane electrode assembly of the proton exchange membrane fuel cell. The effects of the uneven design of the rib width and of the uneven porosity parameters of the cathode and anode gas diffusion layer and catalyst layer on the fuel cell performance were studied in detail. Numerical simulations were designed and implemented for validation. The results show that the fuel cell performance could be improved through the collaborative design of uneven distributions for different layers. The rib width gradually decreasing and the porosity of the cathode gas diffusion layer and the cathode catalyst layer gradually increasing along the fluid flow direction would contribute to a better design compared to the regular even design. The new uneven design can make the fuel penetrate into the catalyst layer in time to participate in the reaction, improve the utilization rate of the membrane electrode assembly, and greatly improve the performance of the fuel cell.


Author(s):  
P. Quan ◽  
M.-C. Lai ◽  
D. S. Hussey ◽  
D. L. Jacobson ◽  
A. Kumar ◽  
...  

The dynamic process of water transport along the through-plane direction in the membrane electrode assembly of a proton exchange membrane fuel cell was investigated using the high-resolution neutron imaging. Four different membrane/gas diffusion layer or membrane/gas diffusion electrode assemblies were tested by measuring the through-plane water thickness profiles. The results indicate that proper design and assembly of the test fixture are critical for accurate water measurement; the accumulation speed of liquid water inside an assembly varies with time; the ionomer in catalyst layers could facilitate water management in the membrane; the time constants for wetting and drying processes are functions of gas diffusion layer thickness, inlet flow rate, and gas dew point; and the time constant for the wetting process is about 1.4 times longer than the corresponding drying process.


2018 ◽  
Vol 32 (12) ◽  
pp. 1850145 ◽  
Author(s):  
Yingli Zhu ◽  
Xiaojian Zhang ◽  
Jianyu Li ◽  
Gary Qi

The gas diffusion layer (GDL), as an important structure of the membrane electrode assembly (MEA) of the direct methanol fuel cell (DMFC), provides a support layer for the catalyst and the fuel and the product channel. Traditionally, the material of GDL is generally carbon paper (CP). In this paper, a new material, namely three-dimensional graphene (3DG) is used as GDL for micro DMFC. The experimental results reveal that the performance of the DMFC has been improved significantly by application of 3DG. The peak powers increase from 25 mW to 31.2 mW and 32 mW by using 3DG as the anode and cathode GDL instead of CP, respectively. The reason may be the decrease of charge and mass transfer resistance of the cell. This means that the unique 3D porous architecture of the 3DG can provide lower contact resistance and sufficient fuel diffusion paths. The output performance of the cell will be further improved when porous metal current collectors is used.


Author(s):  
Jiankui Chen ◽  
Xi Jiang ◽  
Wei Tang ◽  
Liang Ma ◽  
Yiqun Li ◽  
...  

A membrane electrode assembly is the core component of a proton-exchange membrane fuel cell stack. It consists of multilayer structured membranes which are flexible, heterogeneous and have variable cross section. To improve the efficiency of membrane electrode assembly processing and manufacturing, a roll-to-roll system with gas diffusion layer is designed. By peeling the protective membrane and the upper and lower gas diffusion layers’ hot-pressing, proton-exchange membrane is manufactured into a five-layer catalyst-coated membrane. Then, the catalyst-coated membrane is manufactured into membrane electrode assembly by multilayer membrane breakpoint die-cutting and laying-off. The system integrates multiple key technologies, including roll-to-roll precise feeding, gas diffusion layer multi-degree accurate operation and multichannel temperature control, to realize the precise positioning of flexible multilayer membrane and brittle gas diffusion layer. The tension inhomogeneity and critical wrinkling tension are modeled for web traveling in the continuous roll-to-roll manufacturing equipment. The proposed roll-to-roll stack and lamination system effectively combines discontinuous hot-pressing, die-cutting, laying-off technics to realize the high-efficiency manufacturing of membrane electrode assembly.


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