The electrically-pumped terahertz quantum cascade laser (QCL) is characterized by high power emission, compact, broad frequency coverage, and so on, which shows abilities for frequency comb operations. Although free-running QCLs can work as frequency combs by designing the laser structure with small group velocity dispersions and/or inserting mirrors to compensate laser intrinsic dispersions, the ideal comb operation can only be obtained by firmly locking the repetition frequency and carrier frequency of a laser. In this work, we have reported a repetition frequency locking of a terahertz QCL emitting around 4.2 THz. When the 6-mm-long laser is operated in continuous wave mode without any locking techniques, the repetition frequency is measured to be ~6.15 GHz with a linewidth of hundred kilohertz. Once a phase lock loop (PLL) is applied to dynamically control the drive current of the QCL, we have demonstrated a successful repetition frequency locking of the laser with a signal to noise ratio of 80 dB. This technique can be employed for the frequency comb and dual-comb operations of terahertz QCLs for high-resolution applications.
Mass fluxes and isofluxes of methane (CH4) at a New Hampshire fen measured by a continuous wave quantum cascade laser spectrometer
