Characterization of Supercritical Carbon Dioxide Transport within a Brine-Filled Porous Media Using a Two-Phase Pore Network Model

Author(s):  
J. S. Ellis ◽  
A. Ebrahimi ◽  
A. Bazylak

Sequestration of carbon dioxide in deep underground reservoirs has been discussed for the reduction of atmospheric greenhouse gas emissions in the short- to medium-term until more sustainable technologies are available. Cost and long-term stability are major factors in adoption, so techniques to improve the storage efficiency and trapping security are essential. Such improvements require modeling of the porous geological formations involved in the sequestration process, and comparison to both lab- and field-based experimental studies. To this end, we are developing a comprehensive, large-scale pore-network model to describe multi-phase flow in porous media, including the structural, dissolution, and mineral trapping regimes. To explore the optimal operating parameters for mineralization trapping, we describe a two-phase pore-network model of brine-saturated aquifers and model the invasion of supercritical carbon dioxide (CO2) into the pore structure. Regularly-aligned 2D and 3D pore networks are constructed, and rules-based transport models are used to characterize the saturation behavior over a range of viscosity and capillary parameters, and coordination numbers. Finally, saturation patterns are presented for model caprock and sandstone reservoir conditions, taking into account different contact angles for CO2 on mica and quartz at supercritical conditions. These saturation patterns demonstrate the importance of surface heterogeneities in pore-scale modeling of deep saline aquifers.


2008 ◽  
Vol 16 (5) ◽  
pp. 404-410 ◽  
Author(s):  
Zhen Xiu Zhang ◽  
Sung Hyo Lee ◽  
Jin Kuk Kim ◽  
Shu Ling Zhang ◽  
Zhen Xiang Xin

Author(s):  
Wenrui Bao ◽  
Ce Yang ◽  
Li Fu ◽  
Changmao Yang ◽  
Lucheng Ji

Abstract An asymmetric structure of volute in a supercritical carbon dioxide centrifugal compressor induces a non-uniform circumferential distribution of the upstream flow field, which inevitably affects the formation of a two-phase region of carbon dioxide in an impeller. In this work, unsteady simulations for centrifugal compressors were conducted. First, the influence of low static strip induced by low static pressure near volute tongue on the impeller flow field was presented. Then, the non-uniform flow field distribution in the impeller passages and flow characteristics of the passages at the impeller inlet were obtained. Finally, the two-phase regions in the impeller were presented. The results demonstrate that for a centrifugal compressor with volute, the two-phase region appears not only on the suction surface of the leading edge of the blade, but also in some impeller passages, on the pressure surface of the blade near the leading edge, and in the leading edge and mid-chord of tip clearance, under the design conditions. The low static pressure strip induced by the volute leads to a high-speed region in the impeller passages where the temperature and pressure of supercritical carbon dioxide fall below the critical point and carbon dioxide enters the two-phase region. Meanwhile, the static pressure on the blade surface is distorted under the influence of a high-speed region in the passages, resulting in the formation of a two-phase region at the tip clearance. The flow distortion of passages at the impeller inlet results in the appearance of two-phase regions on the both sides of leading edge of the blade. The dryness on the suction side of the blade leading edge and the leading edge of the tip clearance is lower, which indicated that the proportion of liquid-phase carbon dioxide is higher in these two-phase regions.


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