Generation of few-cycle optical pulses in free-electron laser (FEL) oscillators has been experimentally demonstrated in FEL facilities based on normal-conducting and superconducting linear accelerators. Analytical and numerical studies have revealed that the few-cycle FEL lasing can be explained in the frame of superradiance, cooperative emission from self-bunched systems. In the present paper, we review historical remarks of superradiance FEL experiments in short-pulse FEL oscillators with emphasis on the few-cycle pulse generation and discuss the application of the few-cycle FEL pulses to the scheme of FEL-HHG, utilization of infrared FEL pulses to drive high-harmonic generation (HHG) from gas and solid targets. The FEL-HHG enables one to explore ultrafast science with attosecond ultraviolet and X-ray pulses with a MHz repetition rate, which is difficult with HHG driven by solid-state lasers. A research program has been launched to develop technologies for the FEL-HHG and to conduct a proof-of-concept experiment of FEL-HHG.
Detecting multiple chirality centers in chiral molecules with high harmonic generation
