scholarly journals Controlling Spontaneous Emission from Perovskite Nanocrystals with Metal-Emitter-Metal Nanostructures

Author(s):  
Liliana Tjahjana ◽  
Kwan Lee ◽  
Xin Yu Chin ◽  
Landobasa Y.M. Tobing ◽  
Gede W.P. Adhyaksa ◽  
...  

We show the enhancement in the intensity and emission rate of perovskite cesium lead bromide (CsPbBr3) and formamidinium lead bromide (FAPbBr3) nanocrystals in the presence of single and double gold layer cavities, which we refer to as Metal-Emitter (ME) and Metal-Emitter-Metal (MEM) nanostructures. Up to 1.9-fold photoluminescence intensity and up to 5.4-fold emission rate enhancements were obtained for FAPbBr3 nanocrystals confined by double gold layers, which are attributed to plasmonic confinement from the gold layers. The experimentally obtained values are validated by analytical calculations and electromagnetic simulations. Such an effective method of manipulation of the spontaneous emission rate by simple plasmonic nanostructures can be utilized in sensing and detection applications.

Author(s):  
Liliana Tjahjana ◽  
Kwan Lee ◽  
Xin Yu Chin ◽  
Landobasa Y.M. Tobing ◽  
Gede W.P. Adhyaksa ◽  
...  

We show the enhancement in the intensity and emission rate of perovskite cesium lead bromide (CsPbBr3) and formamidinium lead bromide (FAPbBr3) nanocrystals in the presence of single and double gold layer cavities, which we refer to as Metal-Emitter (ME) and Metal-Emitter-Metal (MEM) nanostructures. Up to 1.9-fold photoluminescence intensity and up to 5.4-fold emission rate enhancements were obtained for FAPbBr3 nanocrystals confined by double gold layers, which are attributed to plasmonic confinement from the gold layers. The experimentally obtained values are validated by analytical calculations and electromagnetic simulations. Such an effective method of manipulation of the spontaneous emission rate by simple plasmonic nanostructures can be utilized in sensing and detection applications.


Crystals ◽  
2020 ◽  
Vol 11 (1) ◽  
pp. 1
Author(s):  
Liliana Tjahjana ◽  
Kwan Lee ◽  
Xin Yu Chin ◽  
Landobasa Y.M. Tobing ◽  
Gede W.P. Adhyaksa ◽  
...  

We show the increase of the photoluminescence intensity ratio (PLR) and the emission rate enhancement of perovskite cesium lead bromide (CsPbBr3) and formamidinium lead bromide (FAPbBr3) nanocrystals (NCs) in the presence of single and double gold layer cavities, which we refer to as Metal-Emitter (ME) and Metal-Emitter-Metal (MEM) nanostructures. Up to 1.9-fold PLRs and up to 5.4-fold emission rate enhancements were obtained for FAPbBr3 NCs confined by double gold layers, which are attributed to plasmonic confinement from the gold layers. The experimentally obtained values are validated by analytical calculations and electromagnetic simulations. Such an effective method of manipulation of the spontaneous emission by simple plasmonic nanostructures can be utilized in sensing and detection applications.


1990 ◽  
Vol 26 (9) ◽  
pp. 1492-1499 ◽  
Author(s):  
S.D. Brorson ◽  
H. Yokoyama ◽  
E.P. Ippen

Nanoscale ◽  
2021 ◽  
Author(s):  
Anjun Huang ◽  
Konstantin K Pukhov ◽  
Ka Leung Wong ◽  
Peter A Tanner

The spontaneous emission rate (SER) of a chromophore in a nanoparticle (NP) is determined by the modification of the electric field by its environment. Previous studies of this local field...


2019 ◽  
Vol 9 (1) ◽  
Author(s):  
Ling Li ◽  
Cherian J. Mathai ◽  
Shubhra Gangopadhyay ◽  
Xiaodong Yang ◽  
Jie Gao

2012 ◽  
Vol 2 (5) ◽  
pp. 566 ◽  
Author(s):  
Renaud A. L. Vallée ◽  
Mélanie Ferrié ◽  
Hassan Saadaoui ◽  
Serge Ravaine

2019 ◽  
Vol 123 (14) ◽  
pp. 9343-9351 ◽  
Author(s):  
Belkıs Gökbulut ◽  
Arda Inanç ◽  
Gokhan Topcu ◽  
Tugrul Guner ◽  
Mustafa M. Demir ◽  
...  

2014 ◽  
Vol 116 (4) ◽  
pp. 1867-1875 ◽  
Author(s):  
Sabriye Acikgoz ◽  
Mustafa M. Demir ◽  
Ece Yapasan ◽  
Alper Kiraz ◽  
Ahmet A. Unal ◽  
...  

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