Catalytic Wet Air Oxidation of Acetic Acid on Carbon-Supported Ruthenium Catalysts

1997 ◽  
Vol 168 (1) ◽  
pp. 104-109 ◽  
Author(s):  
Pierre Gallezot ◽  
Stéphane Chaumet ◽  
Alain Perrard ◽  
Pascal Isnard
Keyword(s):  
Acetic Acid ◽  
Ruthenium Catalysts ◽  
Catalytic Wet Air Oxidation ◽  
Air Oxidation ◽  
Wet Air Oxidation

Catalytic wet air oxidation of acetic acid over different ruthenium catalysts

2008 ◽  
Vol 9 (13) ◽  
pp. 2163-2167 ◽  
Author(s):  
Jianbing Wang ◽  
Wanpeng Zhu ◽  
Xuwen He ◽  
Shaoxia Yang
Keyword(s):  
Acetic Acid ◽  
Ruthenium Catalysts ◽  
Catalytic Wet Air Oxidation ◽  
Air Oxidation ◽  
Wet Air Oxidation

Catalysts for Wet Air Oxidation Based on Ce-Zr-Pr-O Mixed Oxides Prepared by Soft Chemistry

2006 ◽  
Vol 45 ◽  
pp. 2089-2095
Author(s):  
Jana Mikulová ◽  
Sylvie Rossignol ◽  
Jacques Barbier Jr. ◽  
Charles Kappenstein ◽  
Daniel Duprez
Keyword(s):  
Aqueous Solution ◽  
Mixed Oxides ◽  
Platinum Catalyst ◽  
Sol Gel ◽  
Ruthenium Catalysts ◽  
Catalytic Wet Air Oxidation ◽  
Air Oxidation ◽  
Wet Air Oxidation ◽  
Soft Chemistry ◽  
Pure Ceria

Sol-gel Zr0.1Ce0.9O2 and Zr0.1(Ce0.75Pr0.25)O2 mixed oxides and coprecipitated pure ceria CeO2 displaying the fluorine type structure have been used as platinum or ruthenium catalysts’ supports for catalytic wet air oxidation (CWAO) of aqueous solution of acetic acid (78 mmol.L-1). These catalysts were prepared by conventional impregnation (5 wt-%) from platinum and ruthenium precursor salts or by exchange (~2 wt-%) in the case of ruthenium. A screening of catalysts in CWAO at 200°C under 2 MPa was performed and reveals that the best platinum catalyst is supported on pure ceria displaying large surface. For ruthenium catalysts, the highest conversion after 3 hours of reaction has been reached by the Ru/Zr-Ce-O system.

scholarly journals Single-atom nickel confined nanotube superstructure as support for catalytic wet air oxidation of acetic acid

2019 ◽  
Vol 2 (1) ◽  
Author(s):  
Chengyu Jin ◽  
Lei Ma ◽  
Wenjing Sun ◽  
Peiwei Han ◽  
Xiangdong Tan ◽  
...  
Keyword(s):  
Acetic Acid ◽  
Catalytic Activity ◽  
Noble Metal ◽  
Intrinsic Property ◽  
Single Atom ◽  
General Strategy ◽  
Catalytic Wet Air Oxidation ◽  
Air Oxidation ◽  
Wet Air Oxidation ◽  
Ru Nanoparticles

AbstractSingle-atom confined materials (SACMs) have been widely researched as catalysts in many fields within recent years. However, this class of materials may not only serve as a catalyst but also as a support material for certain reactions. Here we propose a general strategy to use SACMs as supports for tuning loaded noble metal (e.g., Ru) nanoparticles with enhanced catalytic activity. As a proof of concept, a nickel single-atom confined nitrogen-doped carbon nanotube (NCNT) superstructure is prepared as a support to load noble metal Ru for catalytic wet air oxidation of acetic acid. Improved catalytic activity with a mineralization rate of ~97.5% is achieved. Further, adsorption configurations based on DFT calculations also confirm our deduction that the introduction of single-atom Ni changes the intrinsic property of NCNTs and affects the loaded active Ru nanoparticles.

scholarly journals Recycling Strategy for Bioaqueous Phase via Catalytic Wet Air Oxidation to Biobased Acetic Acid Solution

2020 ◽  
Vol 8 (39) ◽  
pp. 14694-14699
Author(s):  
Songbo He ◽  
Anton Bijl ◽  
Patryk Kamil Barana ◽  
Leon Lefferts ◽  
Sascha R. A. Kersten ◽  
...  
Keyword(s):  
Acetic Acid ◽  
Acid Solution ◽  
Acetic Acid Solution ◽  
Catalytic Wet Air Oxidation ◽  
Air Oxidation ◽  
Wet Air Oxidation
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