Two-photon resonance degenerate four-wave mixing in a three-level polar molecule (model calculations)

1996 ◽  
Vol 28 (8) ◽  
Author(s):  
P.P. Kircheva ◽  
G.B. Hadjichristov ◽  
M.D. Stamova
2019 ◽  
Vol 52 (23) ◽  
pp. 235402
Author(s):  
Hideaki Hara ◽  
Yuki Miyamoto ◽  
Takahiro Hiraki ◽  
Kei Imamura ◽  
Takahiko Masuda ◽  
...  

We present a study of optical phase conjugation through degenerate four-wave mixing in CuCl, as a function of light frequency, intensity, polarization and sample temperature. The phase-conjugate signal exhibits two maxima at the frequencies of the T 5 exciton (one-photon resonance) and of the biexciton (two-photon resonance). By appropriate combinations of the input beam polarizations, it is possible to single out the various terms contributing to the signal (small-spaced, large-spaced population grating and two-photon coherent excitation). The absolute value of X (3) responsible for the two-photon resonance has been determined ( x (3) (-w,w,w, -w) = 3.10 -7 e.s.u.). It leads to ‘mirror’ efficiencies of the order of 10% for input pump intensities I 0 » 10 5 W cm -2 and sample thickness d» 10 -4 cm. At higher I 0 , a saturation of the reflection takes place. The variation of the conjugate beam with temperature has been studied in the range 15 K < T <70 K. Finally, the phase-conjugate nature of the signal has been verified by inserting an aberrator in the path of the input probe beam, and by checking the reconstruction of the reflected beam.


1992 ◽  
Vol 17 (10) ◽  
pp. 716 ◽  
Author(s):  
P. A. Fleitz ◽  
R. L. Sutherland ◽  
T. Pottenger ◽  
N. C. Fernelius ◽  
L. V. Natarajan

1979 ◽  
Vol 4 (10) ◽  
pp. 334 ◽  
Author(s):  
Horace P. Yuen ◽  
Jeffrey H. Shapiro

1995 ◽  
Vol 28 (15) ◽  
pp. 3441-3451 ◽  
Author(s):  
G B Hadjichristov ◽  
M D Stamova ◽  
P P Kircheva

2008 ◽  
Vol 8 (3) ◽  
pp. 1364-1370 ◽  
Author(s):  
Wenling Jia ◽  
Fengqi Guo ◽  
Elliot P. Douglas ◽  
Wenfang Sun

The two-photon absorption coefficients (β) and the third-order nonlinear susceptibilities (χ(3)) of several semiconductor nanoparticles (CdS, CdxAg1–xS, and core–shell CdS/Ag2S) that are confined and stabilized by random and block ionomers have been measured by nonlinear transmission and degenerate four-wave mixing techniques using 21 picosecond laser pulses at near-infrared spectral region. The imaginary part of the third-order nonlinear susceptibility that is related to the two-photon absorption coefficient was then calculated. The absorptive nonlinearity of the nanoparticles (2∼9 nm) was found to be dependent on the particle size, composition and wavelength, i.e., larger CdS particles exhibit higher two-photon absorption coefficients and the presence of Ag improves two-photon absorption of CdS nanoparticles. The obtained two-photon absorption coefficients of nanoparticles corrected for their volume fraction in solution are significantly greater that those of corresponding bulk semiconductors.


ChemInform ◽  
2010 ◽  
Vol 24 (28) ◽  
pp. no-no
Author(s):  
R. L. SUTHERLAND ◽  
E. REA ◽  
L. V. NATARAJAN ◽  
T. POTTENGER ◽  
P. A. FLEITZ

1992 ◽  
Vol 94 (1-3) ◽  
pp. 99-102 ◽  
Author(s):  
Nikola Georgiev ◽  
Ulf Westblom ◽  
Marcus Aldén

Sign in / Sign up

Export Citation Format

Share Document