<p>A stationary, computationally efficient &#160;scheme, ChAP-1.0 (Chemistry and Aerosol Processes, version 1.0) for the sulphur cycle in the troposphereis developed. This scheme is envisaged to be implemented into Earth system models of intermediate complexity (EMICs). The scheme accounts for sulphur dioxide emissions into the atmosphere, its deposition to the surface, oxidation to sulphates, and dry and wet deposition of sulphates on the surface.<br>The calculations with the scheme were performed with the anthropogenic emissions of sulphur compounds into the atmosphere for 1850-2000 according to the CMIP5 (Coupled Models Intercomparison Project, phase 5) 'historical' protocol, with the ERA-Interim meteorology, and assuming that natural sources of sulphur into the atmosphere remain unchanged during this period. The model reasonably reproduces characteristics of the tropospheric sulphur cycle known from observations and other simulations (e.g., in the Atmospheric Chemistry and Climate Model Intercomparison Project phase II (ACCMIP) simulations, Copernicus Atmosphere Monitoring Service (CAMS) reanalysis, and the Meteorological Synthesizing Centre&#8211;West of the European Monitoring and Evaluation Programme (EMEP MSC-W) data). In particular, in 1980's and 1990's, , when the global anthropogenic emission of sulphur, global atmospheric burdens of SO<sub>2</sub> and SO<sub>4</sub> account, correspondingly, 0.2 TgS and 0.4 TgS. In our scheme, about half of the emitted sulphur dioxide is deposited to the surface and the rest in oxidised into sulphates. The latter mostly removed from the atmosphere by wet deposition. The lifetime of the SO<sub>2</sub> and SO<sub>4</sub> in the atmosphere is, respectively, 1.0&#177;0.1 days and 4.1&#177;0.3 days.<br>Despite its simplicity, our scheme may be successfully used to simulate sulphur/sulphates pollution in the atmosphere at coarse spatial and time scales and an impact of this pollution to direct radiative effect of sulphates on climate, their respective indirect (cloud- and precipitation-related) effects, as well as an impact of sulphur compounds on the terrestrial carbon cycle.</p>
Studies of the soluble part of oxidised coals