A Co3O4–CeO2 functionalized SBA-15 monolith with a three-dimensional framework improves NOx-assisted soot combustion

RSC Advances ◽  
2015 ◽  
Vol 5 (34) ◽  
pp. 26815-26822 ◽  
Author(s):  
Qiongqiong Yang ◽  
Fangna Gu ◽  
Yufang Tang ◽  
Hui Zhang ◽  
Qing Liu ◽  
...  

Co3O4–CeO2/SBA-15 monolith can efficiently filter and catalyze the soot particles. The optimized one exhibited a low T10 (293 °C) and T90 (378 °C).

2015 ◽  
Vol 5 (9) ◽  
pp. 4594-4601 ◽  
Author(s):  
Jinguo Wang ◽  
Gaoyang Yang ◽  
Li Cheng ◽  
Eun Woo Shin ◽  
Yong Men

MCr2O4 catalysts with three-dimensional ordered macroporous structures displayed superior catalytic activity for soot combustion to their bulk counterparts.


RSC Advances ◽  
2014 ◽  
Vol 4 (29) ◽  
pp. 14879 ◽  
Author(s):  
Hui Zhang ◽  
Fangna Gu ◽  
Qing Liu ◽  
Jiajian Gao ◽  
Lihua Jia ◽  
...  

2018 ◽  
Vol 8 (21) ◽  
pp. 5462-5472 ◽  
Author(s):  
Peng Zhao ◽  
Nengjie Feng ◽  
Fan Fang ◽  
Geng Liu ◽  
Li Chen ◽  
...  

The appropriate incorporation of potassium into 3DOM SrTiO3 perovskites effectively improved the catalytic performance for soot combustion.


2020 ◽  
Vol 54 (4) ◽  
pp. 2439-2447 ◽  
Author(s):  
Begoña Sellers-Antón ◽  
Esther Bailón-García ◽  
Andrea Cardenas-Arenas ◽  
Arantxa Davó-Quiñonero ◽  
Dolores Lozano-Castelló ◽  
...  

2005 ◽  
Vol 5 (7) ◽  
pp. 1905-1913 ◽  
Author(s):  
K. Wittmaack

Abstract. Combustion of elemental carbon (EC) and organic carbon (OC) contained in ambient aerosol matter was explored using scanning electron microscopy (SEM) in combination with energy dispersive X-ray analysis (EDX). To ease identification of the particles of interest and to avoid or at least reduce interaction with simultaneously sampled inorganic oxides and salts, the approach used in this work differed in two ways from commonly applied procedures. First, rather than using a mixture of particles of vastly different sizes, as in PM10 or PM2.5, aerosol matter was collected in a 5-stage impactor. Second, the water soluble fraction of the collected matter was removed prior to analysis. Diesel soot particles, which appeared in the well-known form of chain-type aggregates, constituted the major fraction of EC. In contrast, OC containing particles were observed in a variety of shapes, including a sizable amount of bioaerosol matter appearing mostly in the size range above about 1 µm. During heating in ambient air for 1h, diesel soot particles were found to be stable up to 470°C, but complete combustion occurred in a narrow temperature interval between about 480 and 510°C. After diesel soot combustion, minute quantities of "ash" were observed in the form of aggregated tiny particles with sizes less than 10 nm. These particles could be due to elemental or oxidic contaminants of diesel soot. Combustion of OC was observed over a wide range of temperatures, from well below 200°C to at least 500°C. Incompletely burnt bioaerosol matter was still found after heating to 600°C. The results imply that the EC fraction in aerosol matter can be overestimated significantly if the contribution of OC to a thermogram is not well separated.


Author(s):  
Yin Ma ◽  
Tong Li ◽  
Jun Yan ◽  
Xiaorong Wang ◽  
Ji Gao ◽  
...  

Electric field assisted combustion is an important means to improve fuel combustion efficiency. This paper conducts extensive research on flame characteristics under different forms and different application methods of electric fields, emission of soot particles and simulation status. Different flame parameter measurement methods will lead to different degrees of error, and perfect numerical simulation can make simple predictions on experimental data. Most of the current numerical simulations are in two dimensions, and it is necessary to develop a complete and accurate three-dimensional model to simulate and predict the characteristics of the flame under an electric field. The emission of soot particles is also affected by the electric field, and reasonable electric field parameters can greatly reduce the emission of soot particles. It is recommended to conduct centralized measurement of different fuels under the electric field under high pressure and temperature conditions, so as to be able to develop a wider and more accurate flame dynamics and chemical model under the electric field.


2005 ◽  
Vol 5 (2) ◽  
pp. 2247-2268 ◽  
Author(s):  
K. Wittmaack

Abstract. Combustion of elemental carbon (EC) and organic carbon (OC) contained in ambient aerosol matter was explored using scanning electron microscopy (SEM) in combination with energy dispersive X-ray analysis (EDX). To ease identification of the particles of interest and to avoid or at least reduce interaction with simultaneously sampled inorganic oxides and salts, the approach used in this work differed in two ways from commonly applied procedures. First, rather than using a mixture of particles of vastly different sizes, as in PM10 or PM2.5, aerosol matter was collected in a 5-stage impactor. Second, the water soluble fraction of the collected matter was removed prior to analysis. Diesel soot particles, which appeared in the well-known form of chain-type aggregates, constituted the major fraction of EC. In contrast, OC containing particles were observed in a variety of shapes, including a sizable amount of bioaerosol matter appearing mostly in the size range above about 1 µm. During heating in ambient air for 1 h, diesel soot particles were found to be stable up to 480°C, but complete combustion occurred in a narrow temperature interval between about 490 and 510°C. After diesel soot combustion, minute quantities of ''ash'' were observed in the form of aggregated tiny particles with sizes less than 10 nm. These particles could be due to elemental or oxidic contaminants of diesel soot. Combustion of OC was observed over a wide range of temperatures, from well below 200°C to at least 500°C. Incompletely burnt bioaerosol matter was still found after heating to 600°C. The results imply that the EC fraction in aerosol matter can be overestimated significantly if the contribution of OC to a thermogram is not well separated.


2017 ◽  
Vol 37 (7) ◽  
pp. 2649-2655 ◽  
Author(s):  
Lina Yang ◽  
Xiaoxia Hu ◽  
Qingzhao Liu ◽  
Jianchen Liu ◽  
Lingyu Li ◽  
...  

1966 ◽  
Vol 25 ◽  
pp. 227-229 ◽  
Author(s):  
D. Brouwer

The paper presents a summary of the results obtained by C. J. Cohen and E. C. Hubbard, who established by numerical integration that a resonance relation exists between the orbits of Neptune and Pluto. The problem may be explored further by approximating the motion of Pluto by that of a particle with negligible mass in the three-dimensional (circular) restricted problem. The mass of Pluto and the eccentricity of Neptune's orbit are ignored in this approximation. Significant features of the problem appear to be the presence of two critical arguments and the possibility that the orbit may be related to a periodic orbit of the third kind.


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