Role of conductive binder to direct solid–electrolyte interphase formation over silicon anodes

With the use of in situ neutron reflectometry (NR) we show how the addition of an electronically conductive polymeric binder, PEFM, mediates the solid–electrolyte interphase (SEI) formation and composition on an amorphous Si (a-Si) electrode as a function of the state-of-charge.

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In Situ Neutron Reflectometry for the Direct Measurement of Cyclic and Evolving Structures in the Lithium Battery Solid Electrolyte Interphase

ECS Meeting Abstracts ◽

10.1149/ma2012-01/9/505 ◽

2012 ◽

Keyword(s):

Solid Electrolyte ◽

Direct Measurement ◽

Lithium Battery ◽

Solid Electrolyte Interphase ◽

Neutron Reflectometry

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In Situ Measurement of Solid Electrolyte Interphase Evolution on Silicon Anodes Using Atomic Force Microscopy

Advanced Energy Materials ◽

10.1002/aenm.201600099 ◽

2016 ◽

Vol 6 (12) ◽

pp. 1600099 ◽

Cited By ~ 47

Author(s):

Insun Yoon ◽

Daniel P. Abraham ◽

Brett L. Lucht ◽

Allan F. Bower ◽

Pradeep R. Guduru

Keyword(s):

Atomic Force Microscopy ◽

Solid Electrolyte ◽

Solid Electrolyte Interphase ◽

In Situ Measurement ◽

Force Microscopy ◽

Silicon Anodes ◽

Atomic Force

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Advanced Characterization of a Stabilized Solid Electrolyte Interphase on Silicon Anodes for Lithium-Ion Batteries By in-Situ Electrochemical Surfaces Forces Apparatus

ECS Meeting Abstracts ◽

10.1149/ma2016-02/4/568 ◽

2016 ◽

Keyword(s):

Solid Electrolyte ◽

Lithium Ion Batteries ◽

Solid Electrolyte Interphase ◽

Lithium Ion ◽

Advanced Characterization ◽

Silicon Anodes

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Role of Polyacrylic Acid (PAA) Binder on the Solid Electrolyte Interphase in Silicon Anodes

Chemistry of Materials ◽

10.1021/acs.chemmater.8b05020 ◽

2019 ◽

Vol 31 (7) ◽

pp. 2535-2544 ◽

Cited By ~ 21

Author(s):

Pritesh Parikh ◽

Mahsa Sina ◽

Abhik Banerjee ◽

Xuefeng Wang ◽

Macwin Savio D’Souza ◽

...

Keyword(s):

Solid Electrolyte ◽

Polyacrylic Acid ◽

Solid Electrolyte Interphase ◽

Silicon Anodes

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Understanding Failure Mechanisms of Solid Electrolyte Interphase on Silicon Anodes: An in-Situ AFM Approach

ECS Meeting Abstracts ◽

10.1149/ma2016-03/2/165 ◽

2016 ◽

Keyword(s):

Solid Electrolyte ◽

Failure Mechanisms ◽

Solid Electrolyte Interphase ◽

Silicon Anodes

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In Situ Studies of Solid Electrolyte Interphase (SEI) Formation on Crystalline Carbon Surfaces by Neutron Reflectometry and Atomic Force Microscopy

ACS Applied Materials & Interfaces ◽

10.1021/acsami.7b09181 ◽

2017 ◽

Vol 9 (41) ◽

pp. 35794-35801 ◽

Cited By ~ 27

Author(s):

Miriam Steinhauer ◽

Michael Stich ◽

Mario Kurniawan ◽

Beatrix-Kamelia Seidlhofer ◽

Marcus Trapp ◽

...

Keyword(s):

Atomic Force Microscopy ◽

Solid Electrolyte ◽

Solid Electrolyte Interphase ◽

Neutron Reflectometry ◽

Force Microscopy ◽

In Situ Studies ◽

Atomic Force ◽

Carbon Surfaces

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Lithium metal protection through in-situ formed solid electrolyte interphase in lithium-sulfur batteries: The role of polysulfides on lithium anode

Journal of Power Sources ◽

10.1016/j.jpowsour.2016.07.056 ◽

2016 ◽

Vol 327 ◽

pp. 212-220 ◽

Cited By ~ 162

Author(s):

Chong Yan ◽

Xin-Bing Cheng ◽

Chen-Zi Zhao ◽

Jia-Qi Huang ◽

Shu-Ting Yang ◽

...

Keyword(s):

Solid Electrolyte ◽

Solid Electrolyte Interphase ◽

Lithium Metal ◽

Lithium Anode ◽

Lithium Sulfur Batteries ◽

Metal Protection ◽

Lithium Sulfur

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Evaluating the solid electrolyte interphase formed on silicon electrodes: a comparison of ex situ X-ray photoelectron spectroscopy and in situ neutron reflectometry

Physical Chemistry Chemical Physics ◽

10.1039/c6cp00978f ◽

2016 ◽

Vol 18 (20) ◽

pp. 13927-13940 ◽

Cited By ~ 44

Author(s):

T. M. Fears ◽

M. Doucet ◽

J. F. Browning ◽

J. K. S. Baldwin ◽

J. G. Winiarz ◽

...

Keyword(s):

Solid Electrolyte ◽

Photoelectron Spectroscopy ◽

Solid Electrolyte Interphase ◽

Solvent Molecule ◽

Neutron Reflectometry ◽

Ex Situ ◽

X Ray

This work details the in situ characterization of the interface between a silicon electrode and an electrolyte using a linear fluorinated solvent molecule.

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