scholarly journals Observation of counterion effects and dimensionality reduction in single-crystal (EDO-TTF)2SbF6 with ultrafast electron diffraction

2019 ◽  
Vol 205 ◽  
pp. 04007
Author(s):  
Lai Chung Liu ◽  
Yifeng Jiang ◽  
Henrike M. Mueller-Werkmeister ◽  
Cheng Lu ◽  
Gustavo Moriena ◽  
...  

Femtosecond electron diffraction is used to resolve structural dynamics in single-crystal (EDO-TTF)2XF6 (X = P, Sb). The retarded and lower-dimensional dynamics of the latter illustrate the dominant role of counterion motion in stabilizing electron transfer.

2017 ◽  
Vol 683 ◽  
pp. 160-165 ◽  
Author(s):  
Lai Chung Liu ◽  
Yifeng Jiang ◽  
Henrike M. Mueller-Werkmeister ◽  
Cheng Lu ◽  
Gustavo Moriena ◽  
...  

2019 ◽  
Vol 205 ◽  
pp. 07005
Author(s):  
Yifeng Jiang ◽  
Lai Chung Liu ◽  
Henrike M. Müller-Werkmeister ◽  
Cheng Lu ◽  
Dongfang Zhang ◽  
...  

Photoinduced spin transitions are studied by femtosecond electron diffraction to understand ultrafast structural dynamics associated with intersystem crossing. The results indicate the structural reorganization occurs within 2.3 ps, as the metal-ligand bond distribution narrows during intramolecular vibrational energy redistribution.


2019 ◽  
Vol 127 (1) ◽  
pp. 19-25
Author(s):  
B. N. Mironov ◽  
S. A. Aseev ◽  
S. V. Chekalin ◽  
A. A. Ishchenko ◽  
V. O. Kompanets ◽  
...  

Nanoscale ◽  
2017 ◽  
Vol 9 (35) ◽  
pp. 13313-13319 ◽  
Author(s):  
Zhongwen Li ◽  
Shuaishuai Sun ◽  
Zi-An Li ◽  
Ming Zhang ◽  
Gaolong Cao ◽  
...  

Ultrafast electron diffraction studies of structural dynamics of boron nitride nanotubes using a transmission electron microscope with a femtosecond laser system.


Author(s):  
Ahmed H. Zewail

In this article we highlight recent developments of ultrafast electron diffraction and crystallography at Caltech. These developments have made it possible to resolve transient structures, both spatially (0.01 Å) and temporally (picosecond and now femtosecond), in the gas phase and condensed media—surfaces, interfaces, and crystals—with wide-ranging applications. With the extension to ultrafast electron microscopy, discussed here and elsewhere, we present an overview of one major research area at our centre, the Laboratory for Molecular Sciences.


2017 ◽  
Vol 129 (25) ◽  
pp. 7236-7240 ◽  
Author(s):  
Yifeng Jiang ◽  
Lai Chung Liu ◽  
Henrike M. Müller-Werkmeister ◽  
Cheng Lu ◽  
Dongfang Zhang ◽  
...  

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