Experimental evidence for an optical interference model for vibrational sum frequency generation on multilayer organic thin film systems. II. Consideration for higher order terms

2015 ◽  
Vol 142 (2) ◽  
pp. 024704 ◽  
Author(s):  
Daniel B. O’Brien ◽  
Aaron M. Massari
2020 ◽  
Vol 2020 ◽  
pp. 1-9
Author(s):  
Dilip Kumar Giri ◽  
Binod Kumar Choudhary

Sum squeezing of the field amplitude is studied in the nondegenerate and degenerate frequency upconversion process under the short interaction time. It is shown that sum squeezing can be converted into normal squeezing via sum-frequency generation in the nondegenerate frequency upconversion process, while the amplitude-squared squeezing of the fundamental mode directly changed into the squeezing of the harmonic in the degenerate frequency upconversion process. All reachable conditions of uncorrelated modes for obtaining a sum squeezing in two modes and its dependence on the squeezing of individual field modes are investigated. It is found that the squeezed states are associated with large number of pump photons. It is also confirmed that the higher-order squeezing (sum squeezing) is directly associated with coupling of the field and interaction time.


2020 ◽  
Vol 12 (23) ◽  
pp. 26515-26524
Author(s):  
Dhritiman Bhattacharyya ◽  
Purnim Dhar ◽  
Yifei Liu ◽  
Peter I. Djurovich ◽  
Mark E. Thompson ◽  
...  

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