Analysis of current-in-plane giant magnetoresistance using Co2FeAl0.5Si0.5 half-metallic Heusler alloy

Author(s):  
Kresna Bondan Fathoni ◽  
Yuya Sakuraba ◽  
Yoshio Miura ◽  
T. T. Sasaki ◽  
Tomoya Nakatani ◽  
...  

Abstract Current-in-plane giant magnetoresistance (CIP-GMR) devices receive revived interest for high-sensitivity magnetic sensors. However, further improvement in MR ratios is necessary to achieve sufficiently magnetic field sensitivity. The usage of half-metallic Co-based Heusler alloy ferromagnetic (FM) layer has been demonstrated to be effective in enhancing GMR in current-perpendicular-to-plane (CPP) configuration; however, only small MR ratios are obtained in the CIP configuration. To understand the origin of the disappointingly low MR in the CIP configuration using the Heusler alloy FM layers, we investigated magnetotransport properties of CIP-GMR devices using half-metallic Co2FeAl0.5Si0.5 (CFAS) Heusler alloy and conventional CoFe alloy as ferromagnetic (FM) layers in combination with Ag or Cu as nonmagnetic (NM) spacer layer. Regardless of high lattice and electronic band matching at the CFAS/Ag interface, CFAS/Ag CIP spin valves (SVs) shows the MR ratio of only 1.2% at RT, which is much smaller than those of reference CoFe/Cu and CoFe/Ag SVs, 21.6 and 8.4%, respectively. Current density distribution simulations suggest that large current shunting occurs in the Ag layer due to significant resistivity gap between CFAS and Ag, which limits the generation of highly spin-polarized current from the CFAS layer, resulting in the very small MR ratios. To enhance the MR ratio in CIP-GMR using half-metallic materials, resistivity matching between FM layers and NM layer is required in addition to the high electronic band match that has been considered as key factors to obtain high MR ratio in CIP-GMR.

SPIN ◽  
2014 ◽  
Vol 04 (02) ◽  
pp. 1440009 ◽  
Author(s):  
SAYANI MAJUMDAR ◽  
SUKUMAR DEY ◽  
HANNU HUHTINEN ◽  
JOHNNY DAHL ◽  
MARJUKKA TUOMINEN ◽  
...  

Recent experimental reports suggest the formation of a highly spin-polarized interface ("spinterface") between a ferromagnetic (FM) Cobalt ( Co ) electrode and a metal-phthalocyanine (Pc) molecule. Another report shows an almost 60% giant magnetoresistance (GMR) response measured on Co / H 2 Pc -based single molecule spin valves. In this paper, we compare the spin injection and transport properties of organic spin valves with two different organic spacers, namely Tris(8-hydroxyquinolinato) aluminum ( Alq 3) and CoPc sandwiched between half-metallic La 0.7 Sr 0.3 MnO 3 (LSMO) and Co electrodes. Alq 3-based spin valves exhibit clear and reproducible spin valve switching with almost 35% negative GMR at 10 K, in accordance with previous reports. In contrast, cobalt-pthalocyanine ( CoPc )-based spin valves fail to show clear GMR response above noise level despite high expectations based on recent reports. Investigations of electronic, magnetic and magnetotransport properties of electrode/spacer interfaces of LSMO/ CoPc / Co devices offer three plausible explanations for the absence of GMR: (1) CoPc films are strongly chemisorbed on the LSMO surface. This improves the LSMO magnetic properties but also induces local traps at the LSMO interface for spin-polarized charge carriers. (2) At the Co / CoPc interface, diffusion of Co atoms into the organic semiconductor (OS) layer and chemical reactivity between Co and the OS deteriorates the FM properties of Co . This renders the Co / CoPc interface as unsuitable for efficient spin injection. (3) The presence of heavy Co atoms in CoPc leads to large spin–orbit coupling in the spacer. The spin relaxation time in the CoPc layer is therefore considerably smaller compared to Alq 3. Based on these findings, we suggest that the absence of GMR in CoPc -based spin valves is caused by a combined effect of inefficient spin injection from FM contacts and poor spin transport in the CoPc spacer layer.


2010 ◽  
Vol 84 (6) ◽  
pp. 717-721 ◽  
Author(s):  
Dibya Prakash Rai ◽  
Javad Hashemifar ◽  
Morteeza Jamal ◽  
Lalmuanpuia ◽  
M. P. Ghimire ◽  
...  

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