In this paper, we present the results of the study of the statistics of pulse energy fluctuations in a Raman laser under optical pump by the multimode nanosecond pulses. A system of coupled differential equations for slowly varying envelopes of the pump field and first three Stokes lines was integrated numerically with taking into account spatial inhomogeneity of the pump beam, spontaneous noise, and optical feedback. Data of the numerical simulation revealed a sharp increase in the fluctuation amplitude in the nonlinear regime of Raman frequency conversion when the optical length of the Raman cavity was matched with the cavity length of the multimode pump laser. At a mean 1st Stokes conversion efficiency of 3.5–3.8 %, the calculations showed an increase in the coefficient of variation (CV) of a random value from 9 % to 118 %. In the linear regime of Raman frequency conversion, when the conversion efficiency was 0.2–0.03 %, a further increase in the CV value up to 270–500 % was predicted. It is also numerically shown that the fluctuation statistics under the conditions of the cavity length matching is essentially non-Gaussian and described by the L-type probability density distributions (PDDs) with long tails and maxima located near zero. The numerical data were quantitatively confirmed by an experiment for a Raman laser on a barium nitrate crystal operated near the Raman threshold, when the 1st Stokes conversion efficiency did not exceed 0.3 %. A Raman cavity was formed by two flat mirrors providing a double-pass pump configuration. The Raman laser was excited by the linearly polarized frequency-doubled radiation of a Q-switched Nd:YAG laser generating multimode pulses with a duration of 7–8 ns. A Raman laser operating regime characterized by the hyperexponential PDDs with CVs reaching 480 %, which is 2–2.5 times higher than those observed earlier for the single-pass conditions of stimulated Raman scattering, was realized.
Polarization-Tailored Raman Frequency Conversion in Chiral Gas-Filled Hollow-Core Photonic Crystal Fibers
