Temperature Dependence of the Zero-Field Splitting of Cr3+ Ions in CsAl(SO4)2∙12H2O
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A Value
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The zero-field splitting of Cr3+ ions in CsAl(SO4)2∙12H2O was studied in the temperature range 4.2 to 300 K. The experimental spectrum is described with a spin Hamiltonian with S = 3/2 and g = 1.975 ± 0.005; the zero-field splitting parameter D changes with temperature having a value of −0.074 ± 0.0003 cm−1 at room temperature and a value of −0.070 ± 0.0003 cm−1 at liquid helium temperature.
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