Third-Order Optical Nonlinearity Due to Excitons and Biexcitons in a Self-Organized Quantum-Well Material (C6H13NH3)2PbI4
1998 ◽
Vol 07
(01)
◽
pp. 153-159
◽
Keyword(s):
Third-order optical nonlinearity around the exciton resonance in (C6H13NH3)2PbI4 was measured using time-integrated and spectrally-resolved four-wave-mixing (FWM) techniques. For excitation below the exciton resonance, biexciton contribution to the FWM signals was observed. The dephasing energy of the biexcitons was estimated to be larger than 10 meV.