Third-Order Optical Nonlinearity Due to Excitons and Biexcitons in a Self-Organized Quantum-Well Material (C6H13NH3)2PbI4

1998 ◽  
Vol 07 (01) ◽  
pp. 153-159 ◽  
Author(s):  
J. Ishi ◽  
M. Mizuno ◽  
H. Kunugita ◽  
K. Ema ◽  
S. Iwamoto ◽  
...  

Third-order optical nonlinearity around the exciton resonance in (C6H13NH3)2PbI4 was measured using time-integrated and spectrally-resolved four-wave-mixing (FWM) techniques. For excitation below the exciton resonance, biexciton contribution to the FWM signals was observed. The dephasing energy of the biexcitons was estimated to be larger than 10 meV.

1992 ◽  
Vol 247 ◽  
Author(s):  
James S. Shirk ◽  
J. R. Undle ◽  
Steven R. Flom ◽  
F. J. Bartoli ◽  
Arthur W. Snow

ABSTRACTThis paper discusses the third-order nonlinear optical (NLO) properties of substituted phthalocyanines measured by time-resolved degenerate four-wave mixing at 1064 nm. The study explores optical pumping as a mechanism contributing to a large third-order optical nonlinearity in one member of this interesting class of NLO materials, PbPc(CP)4.


1997 ◽  
Vol 144 (4-6) ◽  
pp. 245-251 ◽  
Author(s):  
G. Ravindra Kumar ◽  
M. Ravikanth ◽  
Sudeep Banerjee ◽  
Armen Sevian

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