(Invited) Enable Efficient Solar Driven CO2 Reduction with Stable and Highly Active Oxygen Evolution Catalyst in Neutral pH

2021 ◽  
Vol MA2021-01 (39) ◽  
pp. 1281-1281
Author(s):  
Hongfei Jia ◽  
Li Zhou ◽  
Ling Chen
2019 ◽  
Vol 10 (1) ◽  
Author(s):  
Li Qin Zhou ◽  
Chen Ling ◽  
Hui Zhou ◽  
Xiang Wang ◽  
Joseph Liao ◽  
...  

Abstract The efficiency of sunlight-driven reduction of carbon dioxide (CO2), a process mimicking the photosynthesis in nature that integrates the light harvester and electrolysis cell to convert CO2 into valuable chemicals, is greatly limited by the sluggish kinetics of oxygen evolution in pH-neutral conditions. Current non-noble metal oxide catalysts developed to drive oxygen evolution in alkaline solution have poor performance in neutral solutions. Here we report a highly active and stable oxygen evolution catalyst in neutral pH, Brownmillerite Sr2GaCoO5, with the specific activity about one order of magnitude higher than that of widely used iridium oxide catalyst. Using Sr2GaCoO5 to catalyze oxygen evolution, the integrated CO2 reduction achieves the average solar-to-CO efficiency of 13.9% with no appreciable performance degradation in 19 h of operation. Our results not only set a record for the efficiency in sunlight-driven CO2 reduction, but open new opportunities towards the realization of practical CO2 reduction systems.


Joule ◽  
2018 ◽  
Vol 2 (8) ◽  
pp. 1511-1521 ◽  
Author(s):  
Nien-Chu Lai ◽  
Guangtao Cong ◽  
Zhuojian Liang ◽  
Yi-Chun Lu

2021 ◽  
pp. 139630
Author(s):  
Miaomiao Wu ◽  
Yi Zhang ◽  
Renyuan Zhang ◽  
Jiwei Ma ◽  
Nicolas Alonso-Vante

2019 ◽  
Vol 2 (12) ◽  
pp. 8930-8938 ◽  
Author(s):  
Alberto Bucci ◽  
Suvendu Sekhar Mondal ◽  
Vlad Martin-Diaconescu ◽  
Alexandr Shafir ◽  
Julio Lloret-Fillol

2018 ◽  
Vol 6 (11) ◽  
pp. 4636-4641 ◽  
Author(s):  
Liyong Chen ◽  
Yuting Guo ◽  
Huifang Wang ◽  
Zhizhi Gu ◽  
Yingyue Zhang ◽  
...  

To fully achieve an eco-friendly means of storing electricity in the form of chemical fuels, the development of a green synthetic route towards highly active oxygen evolution reaction (OER) electrocatalysts is required.


2019 ◽  
Vol 63 (3) ◽  
pp. 356-363 ◽  
Author(s):  
Pengsong Li ◽  
Xiuping Zhao ◽  
Xinxuan Duan ◽  
Yaping Li ◽  
Yun Kuang ◽  
...  

2019 ◽  
Vol 334 ◽  
pp. 59-67 ◽  
Author(s):  
Lisa Geerts ◽  
Salvatore Cosentino ◽  
Ting-Wei Liao ◽  
Anupam Yadav ◽  
Pin-Cheng Lin ◽  
...  

2018 ◽  
Vol 54 (43) ◽  
pp. 5462-5465 ◽  
Author(s):  
Jinxiu Zhao ◽  
Xianghong Li ◽  
Guanwei Cui ◽  
Xuping Sun

An Fe-doped NiCr2O4 nanoparticle film on Ni foam (Fe–NiCr2O4/NF) acts as a durable water oxidation electrocatalyst with superior activity, needing an overpotential of 318 mV to drive 500 mA cm−2 in 1.0 M KOH.


2019 ◽  
Vol 11 (11) ◽  
pp. 10608-10615 ◽  
Author(s):  
Hyung Jong Choi ◽  
Gwon Deok Han ◽  
Kiho Bae ◽  
Joon Hyung Shim

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