A Ragged Porous Hollow Tubular Carbon Nitride Towards Boosting Visible-Light Photocatalytic Hydrogen Production in Water and Seawater

2021 ◽  
Author(s):  
Feng Guo ◽  
Zhihao Chen ◽  
Yuxing Shi ◽  
Longwen Cao ◽  
Xiaofang Cheng ◽  
...  
Catalysts ◽  
2018 ◽  
Vol 8 (9) ◽  
pp. 366 ◽  
Author(s):  
Hongwei Wang ◽  
Guiqing Huang ◽  
Zhiwei Chen ◽  
Weibing Li

In this study, we prepared carbon self-doped carbon nitride nanosheets through a glucose synergic co-condensation method. In the carbon self-doped structure, the N atoms in the triazine rings were substituted by C atoms, resulting in enhanced visible-light photocatalytic hydrogen production, which is three-times higher than that of bulk carbon nitride. The enhanced photocatalytic hydrogen production was attributed to the higher charge-carrier transfer rate and widened light absorption range of the carbon nitride nanosheets after carbon self-doping. Thus, this work highlights the importance of carbon self-doping for improving the photocatalytic performance. Meanwhile, it provides a feasible method for the preparation of carbon self-doped carbon nitride without destroying the 2D conjugated backbone structures.


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