scholarly journals CLOUD DROPLET FORMATION UTILIZING ATMOSPHERIC POLLUTANT (NH4) 2SO4 AS CONDENSATION NUCLEUS

1998 ◽  
Vol 6 ◽  
pp. 91-96
Author(s):  
Sadataka SHIBA ◽  
Taku KATO ◽  
Yushi HIRATA ◽  
Shunsaku YAGI
2009 ◽  
Vol 9 (2) ◽  
pp. 8635-8665 ◽  
Author(s):  
P. Reutter ◽  
J. Trentmann ◽  
H. Su ◽  
M. Simmel ◽  
D. Rose ◽  
...  

Abstract. We have investigated the formation of cloud droplets under (pyro-)convective conditions using a cloud parcel model with detailed spectral microphysics and with the κ-Köhler model approach for efficient and realistic description of the cloud condensation nucleus (CCN) activity of aerosol particles. Assuming a typical biomass burning aerosol size distribution (accumulation mode centred at 120 nm), we have calculated initial cloud droplet number concentrations (NCD) for a wide range of updraft velocities (w=0.5–20 m s−1) and aerosol particle number concentrations (NCN=103–105 cm−3) at the cloud base. Depending on the ratio between updraft velocity and particle number concentration (w/NCN), we found three distinctly different regimes of CCN activation and cloud droplet formation: 1. An aerosol-limited regime that is characterized by high w/NCN ratios (>≈10−3 m s−1 cm3), high maximum values of water vapour supersaturation (Smax>≈0.5%), and high activated fractions of aerosol particles (NCD/NCN>≈90%). In this regime NCD is directly proportional to NCN and practically independent of w. 2. An updraft-limited regime that is characterized by low w/NCN ratios (


2009 ◽  
Vol 9 (18) ◽  
pp. 7067-7080 ◽  
Author(s):  
P. Reutter ◽  
H. Su ◽  
J. Trentmann ◽  
M. Simmel ◽  
D. Rose ◽  
...  

Abstract. We have investigated the formation of cloud droplets under pyro-convective conditions using a cloud parcel model with detailed spectral microphysics and with the κ-Köhler model approach for efficient and realistic description of the cloud condensation nucleus (CCN) activity of aerosol particles. Assuming a typical biomass burning aerosol size distribution (accumulation mode centred at 120 nm), we have calculated initial cloud droplet number concentrations (NCD) for a wide range of updraft velocities (w=0.25–20 m s−1) and aerosol particle number concentrations (NCN=200–105 cm−3) at the cloud base. Depending on the ratio between updraft velocity and particle number concentration (w/NCN), we found three distinctly different regimes of CCN activation and cloud droplet formation: (1) An aerosol-limited regime that is characterized by high w/NCN ratios (>≈10−3 m s−1 cm3), high maximum values of water vapour supersaturation (Smax>≈0.5%), and high activated fractions of aerosol particles (NCN/NCN>≈90%). In this regime NCD is directly proportional to NCN and practically independent of w. (2) An updraft-limited regime that is characterized by low w/NCN ratios (


2004 ◽  
Vol 31 (5) ◽  
pp. n/a-n/a ◽  
Author(s):  
Ulrike Lohmann ◽  
Keith Broekhuizen ◽  
Richard Leaitch ◽  
Nicole Shantz ◽  
Jonathan Abbatt

2016 ◽  
Author(s):  
Sami Romakkaniemi ◽  
Zubair Maalick ◽  
Antti Hellsten ◽  
Antti Ruuskanen ◽  
Olli Väisänen ◽  
...  

Abstract. Long-term in situ measurements of aerosol-cloud interactions are usually performed in measurement stations residing on hills, mountains, or high towers. In such conditions, the surface topography of the surrounding area can affect the measured cloud droplet distributions by increasing turbulence or causing orographic flows and thus the observations might not be representative for a larger scale. The objective of this work is to analyse, how the local topography affects the observations at Puijo measurement station, which is located in the 75 m high Puijo tower, which itself stands on a 150 m high hill. The analysis of the measurement data shows that the observed cloud droplet number concentration mainly depends on the CCN concentration. However, when the wind direction aligns with the direction of the steepest slope of the hill, a clear topography effect is observed. This finding was further analysed by simulating 3D flow fields around the station and by performing trajectory ensemble modelling of aerosol- and wind-dependent cloud droplet formation. The results showed that in typical conditions, with geostrophic winds of about 10 m s−1, the hill can cause updrafts of up to 1 m s−1 in the air parcels arriving at the station. This is enough to produce in-cloud supersaturations higher than typically found at the cloud base (SS of ~ 0.2 %), and thus additional cloud droplets may form inside the cloud. In the observations, this is seen in the form of a bi-modal cloud droplet size distribution. The effect is strongest with high winds across the steepest slope of the hill and with low liquid water contents, and its relative importance quickly decreases as these conditions are relaxed. We therefore conclude that, after careful screening for wind speed and liquid water content, the observations at Puijo measurement station can be considered representative for clouds in a boreal environment.


Tellus B ◽  
1996 ◽  
Vol 48 (3) ◽  
pp. 347-360 ◽  
Author(s):  
Markku Kulmala ◽  
Pekka Korhonen ◽  
Timo Vesala ◽  
Hans-Christen Hansson ◽  
Kevin Noone ◽  
...  

1995 ◽  
Vol 26 ◽  
pp. S891-S892
Author(s):  
Markku Kulmala ◽  
Pekka Korhonen ◽  
Timo Vesala ◽  
Hans-Christen Hansson ◽  
Kevin Noone ◽  
...  

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