scholarly journals Magic Numbers in Boson 4He Clusters: The Auger Evaporation Mechanism

Molecules ◽  
2021 ◽  
Vol 26 (20) ◽  
pp. 6244
Author(s):  
Elena Spreafico ◽  
Giorgio Benedek ◽  
Oleg Kornilov ◽  
Jan Peter Toennies

The absence of magic numbers in bosonic 4He clusters predicted by all theories since 1984 has been challenged by high-resolution matter-wave diffraction experiments. The observed magic numbers were explained in terms of enhanced growth rates of specific cluster sizes for which an additional excitation level calculated by diffusion Monte Carlo is stabilized. The present theoretical study provides an alternative explanation based on a simple independent particle model of the He clusters. Collisions between cluster atoms in excited states within the cluster lead to selective evaporation via an Auger process. The calculated magic numbers as well as the shape of the number distributions are in quite reasonable agreement with the experiments.

Investigation of the Rb I absorption spectrum between 40 and 120 Å has revealed a broad absorption maximum in the 3d photoionization continuum, as well as discrete features associated with the excitation of a 3d-subshell electron. The discrete structure is identified, Hartree-Fock calculations of the transition energies are given and the absorption maximum is discussed in relation to similar spectra and to recent random phase approximation with exchange (r.p.a.e.) and independent particle model calculations.


2007 ◽  
Vol 46 (1) ◽  
pp. 27-36 ◽  
Author(s):  
A. Surzhykov ◽  
U. D. Jentschura ◽  
T. Stöhlker ◽  
S. Fritzsche

1996 ◽  
Vol 74 (11-12) ◽  
pp. 703-712 ◽  
Author(s):  
Ian E. McCarthy

Electron momentum spectroscopy of atoms, molecules, and solids is based on (e,2e) reactions that observe the distribution of recoil momenta for energy-resolved states of the residual system. It is interpreted simply in terms of the momentum-space orbitals of the independent-particle model. The relevant ideas originated in nuclear physics. The earliest experiments observed that strongly excited final states belong to orbital manifolds that extend the independent-particle ideas to correlated systems. Some weakly excited final states do not belong to orbital manifolds. They give sensitive information about target ground-state correlations. The energy-momentum distribution of valence bands is observed for solids. Calculations for atoms, molecules, and crystals converge to the experimental result as the structure calculation is improved.


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