scholarly journals Referee Comment on "Estimating Upper Silesian coal mine methane emissions from airborne in situ observations and dispersion modeling"

2020 ◽  
Author(s):  
Anonymous
2020 ◽  
Author(s):  
Julian Kostinek ◽  
Anke Roiger ◽  
Maximilian Eckl ◽  
Alina Fiehn ◽  
Andreas Luther ◽  
...  

Abstract. Abundant mining and industrial activities located in the Upper Silesian Coal Basin (USCB) lead to large emissions of the potent greenhouse gas (GHG) methane (CH4). The strong localization of CH4 emitters (mostly confined to known coal mine ventilation shafts) and the large emissions of 448/720 kt CH4 yr−1 reported in the European Pollutant Release and Transfer Register (E-PRTR 2017) and the Emissions Database for Global Atmospheric Research (EDGAR v4.3.2) make the USCB a prime research target for validating and improving CH4 flux estimation techniques. High-precision observations of this GHG were made downwind of local (e.g. single facilities) to regional-scale sources (e.g. agglomerations) in the context of the CoMet 1.0 campaign in early summer 2018. A Quantum Cascade/Interband Cascade Laser (QCL/ICL) based spectrometer adapted for airborne research was deployed aboard the German Aerospace Centers (DLR) Cessna 208B to sample the planetary boundary layer (PBL) in situ. Regional CH4 emission estimates for the USCB are derived using a model approach including assimilated wind soundings from three ground-based Doppler lidars. Although retrieving estimates for individual emitters is difficult using only single flights, due to sparse data availability, the combination of two flights allows for exploiting different meteorological conditions (analogous to a sparse tomography algorithm) to establish confidence on facility level estimates. Emission rates from individual sources are not only needed for unambiguous comparisons between bottom-up and top-down inventories but become indispensable if (independently verifiable) sanctions are to be imposed on individual companies emitting GHGs. An uncertainty analysis is presented for both the regional scale and facility level emission estimates. We find instantaneous emission estimates of 452/442 ± 78/75 kt CH4 yr−1 for the morning/afternoon flight of June 6th, 2018. The derived emission rates coincide (±2 %) with annual-average inventorial data from E-PRTR 2017 albeit they are distinctly lower (−37 %/−40 %) than values reported in EDGAR v4.3.2. Discrepancies in available emission inventories could potentially be narrowed down with sufficient observations using the method described herein to bridge the gap between instantaneous emission estimates and yearly averaged inventories.


2021 ◽  
Vol 21 (11) ◽  
pp. 8791-8807
Author(s):  
Julian Kostinek ◽  
Anke Roiger ◽  
Maximilian Eckl ◽  
Alina Fiehn ◽  
Andreas Luther ◽  
...  

Abstract. Abundant mining and industrial activities located in the Upper Silesian Coal Basin (USCB) lead to large emissions of the potent greenhouse gas (GHG) methane (CH4). The strong localization of CH4 emitters (mostly confined to known coal mine ventilation shafts) and the large emissions of 448 and 720 kt CH4 yr−1 reported in the European Pollutant Release and Transfer Register (E-PRTR 2017) and the Emissions Database for Global Atmospheric Research (EDGAR v4.3.2), respectively, make the USCB a prime research target for validating and improving CH4 flux estimation techniques. High-precision observations of this GHG were made downwind of local (e.g., single facilities) to regional-scale (e.g., agglomerations) sources in the context of the CoMet 1.0 campaign in early summer 2018. A quantum cascade–interband cascade laser (QCL–ICL)-based spectrometer adapted for airborne research was deployed aboard the German Aerospace Center (DLR) Cessna 208B to sample the planetary boundary layer (PBL) in situ. Regional CH4 emission estimates for the USCB are derived using a model approach including assimilated wind soundings from three ground-based Doppler lidars. Although retrieving estimates for individual emitters is difficult using only single flights due to sparse data availability, the combination of two flights allows for exploiting different meteorological conditions (analogous to a sparse tomography algorithm) to establish confidence on facility-level estimates. Emission rates from individual sources not only are needed for unambiguous comparisons between bottom-up and top-down inventories but also become indispensable if (independently verifiable) sanctions are to be imposed on individual companies emitting GHGs. An uncertainty analysis is presented for both the regional-scale and facility-level emission estimates. We find instantaneous coal mine emission estimates of 451/423 ± 77/79 kt CH4 yr−1 for the morning/afternoon flight of 6 June 2018. The derived fuel-exploitation emission rates coincide (±6 %) with annual-average inventorial data from E-PRTR 2017 although they are distinctly lower (−28 %/−32 %) than values reported in EDGAR v4.3.2. Discrepancies in available emission inventories could potentially be narrowed down with sufficient observations using the method described herein to bridge the gap between instantaneous emission estimates and yearly averaged inventories.


2019 ◽  
Vol 6 (8) ◽  
pp. 473-478 ◽  
Author(s):  
Jianxiong Sheng ◽  
Shaojie Song ◽  
Yuzhong Zhang ◽  
Ronald G. Prinn ◽  
Greet Janssens-Maenhout

2015 ◽  
Vol 12 (2) ◽  
pp. 1907-1973 ◽  
Author(s):  
T. J. Bohn ◽  
J. R. Melton ◽  
A. Ito ◽  
T. Kleinen ◽  
R. Spahni ◽  
...  

Abstract. Wetlands are the world's largest natural source of methane, a powerful greenhouse gas. The strong sensitivity of methane emissions to environmental factors such as soil temperature and moisture has led to concerns about potential positive feedbacks to climate change. This risk is particularly relevant at high latitudes, which have experienced pronounced warming and where thawing permafrost could potentially liberate large amounts of labile carbon over the next 100 years. However, global models disagree as to the magnitude and spatial distribution of emissions, due to uncertainties in wetland area and emissions per unit area and a scarcity of in situ observations. Recent intensive field campaigns across the West Siberian Lowland (WSL) make this an ideal region over which to assess the performance of large-scale process-based wetland models in a high-latitude environment. Here we present the results of a follow-up to the Wetland and Wetland CH4 Intercomparison of Models Project (WETCHIMP), focused on the West Siberian Lowland (WETCHIMP-WSL). We assessed 21 models and 5 inversions over this domain in terms of total CH4 emissions, simulated wetland areas, and CH4 fluxes per unit wetland area and compared these results to an intensive in situ CH4 flux dataset, several wetland maps, and two satellite inundation products. We found that: (a) despite the large scatter of individual estimates, 12 year mean estimates of annual total emissions over the WSL from forward models (5.34 ± 0.54 Tg CH4 y-1), inversions (6.06 ± 1.22 Tg CH4 y-1), and in situ observations (3.91 ± 1.29 Tg CH4 y-1) largely agreed, (b) forward models using inundation products alone to estimate wetland areas suffered from severe biases in CH4 emissions, (c) the interannual timeseries of models that lacked either soil thermal physics appropriate to the high latitudes or realistic emissions from unsaturated peatlands tended to be dominated by a single environmental driver (inundation or air temperature), unlike those of inversions and more sophisticated forward models, (d) differences in biogeochemical schemes across models had relatively smaller influence over performance; and (e) multi-year or multi-decade observational records are crucial for evaluating models' responses to long-term climate change.


2011 ◽  
Vol 45 (13) ◽  
pp. 2220-2232 ◽  
Author(s):  
Shi Su ◽  
Jiaye Han ◽  
Jinyan Wu ◽  
Hongjun Li ◽  
Rhys Worrall ◽  
...  

2021 ◽  
Author(s):  
Alina Fiehn ◽  
Julian Kostinek ◽  
Maximilian Eckl ◽  
Michal Galkowski ◽  
Christoph Gerbig ◽  
...  

<p>Emissions from fossil fuels are one of the primary sources of atmospheric methane (CH<sub>4</sub>) growth. However, estimates of anthropogenic CH<sub>4</sub> emissions still show large uncertainties on global and regional scales. Differences in CH<sub>4</sub> isotopic source signatures δ<sup>13</sup>C and δD can help to constrain different source contributions (e.g. fossil, thermogenic, or biogenic).</p><p>The Upper Silesian Coal Basin (USCB) represents one of the largest European CH<sub>4</sub> emission source regions, with more than 500 Gg CH<sub>4</sub> yr<sup>-1</sup> released by more than 50 coal mine ventilation shafts. During the CoMet (Carbon Dioxide and Methane Mission) campaign in June 2018 methane observations were conducted from a variety of platforms including aircraft and cars. Beside the continuous sampling of atmospheric methane concentration, numerous air samples were taken from inside the ventilation shafts, around the ventilation shafts (1‑2 km distance) and aboard the DLR Cessna Caravan aircraft and analyzed in the laboratory for the isotopic composition of CH<sub>4</sub>.</p><p>The ground-based samples allowed determining the source signatures of individual ventilation shafts. These signatures displayed a considerable range between different shafts and also varied from day to day. The airborne samples contained a mixture of methane emissions from several mines and thus enabled accurately determining the signature of the entire region. The mean isotopic signature of methane emissions over the USCB derived from the aircraft samples was -51.9 ± 0.5 ‰ for δ<sup>13</sup>C and -233 ± 6 ‰ for δD. This is in between the range of other microbial and thermogenic coal reservoirs, but more depleted in δD than previous USCB studies reported based on samples taken within the mines. Signatures of methane enhancements sampled upwind of the mines and in the free troposphere clearly showed the presence of methane of biogenic origin (e.g. wetlands, waste, ruminants).</p><p>Furthermore, we simulated the methane isotopologues using the on-line three-times nested global regional chemistry climate model MECO(n). We implemented a submodel extension, which includes the kinetic fractionation and uses the isotopic source signatures determined by the ground-based observations. We compare the regional simulations to flask samples taken during CoMet.</p>


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