scholarly journals The study of emission inventory on anthropogenic air pollutants and VOC species in the Yangtze River Delta region, China

2011 ◽  
Vol 11 (1) ◽  
pp. 951-983 ◽  
Author(s):  
C. Huang ◽  
C. H. Chen ◽  
L. Li ◽  
Z. Cheng ◽  
H. L. Wang ◽  
...  

Abstract. The purpose of this study is to develop an emission inventory for major anthropogenic air pollutants and VOC species in the Yangtze River Delta (YRD) region for the year 2007. A "bottom-up" methodology was adopted to compile the inventory based on major emission sources in the sixteen cities of this region. Results show that the emissions of SO2, NOx, CO, PM10, PM2.5, VOCs, and NH3 in the YRD region for the year 2007 are 2391.8 kt, 2292.9 kt, 6697.1 kt, 3115.7 kt, 1510.8 kt, 2767.4 kt, and 458.9 kt, respectively. Ethylene, mp-xylene, o-xylene, toluene, and 1,2,4-trimethylbenzene, 2,4-dimethylpentane, ethyl benzene, propylene, 1-pentene, and isoprene are the key species contributing 77% to the total OFPs. The spatial distribution of the emissions shows the emissions and OFPs are mainly concentrated in the urban and industrial areas along the Yangtze River and around the Hangzhou Bay. The industrial sources including power plant, other fuel combustion facilities, and non-combustion processes contribute about 97%, 86%, 89%, 91%, and 69% of the total SO2, NOx, PM10, PM2.5, and VOC emissions. Vehicles take up 12.3% and 12.4% of the NOx and VOC emissions, respectively. Regarding OFPs, chemical industry, domestic use of paint and printing, and gasoline vehicle contribute 38.2%, 23.9%, and 11.6% to the ozone formation in the YRD region.

2011 ◽  
Vol 11 (9) ◽  
pp. 4105-4120 ◽  
Author(s):  
C. Huang ◽  
C. H. Chen ◽  
L. Li ◽  
Z. Cheng ◽  
H. L. Wang ◽  
...  

Abstract. The purpose of this study is to develop an emission inventory for major anthropogenic air pollutants and VOC species in the Yangtze River Delta (YRD) region for the year 2007. A "bottom-up" methodology was adopted to compile the inventory based on major emission sources in the sixteen cities of this region. Results show that the emissions of SO2, NOx, CO, PM10, PM2.5, VOCs, and NH3 in the YRD region for the year 2007 are 2392 kt, 2293 kt, 6697 kt, 3116 kt, 1511 kt, 2767 kt, and 459 kt, respectively. Ethylene, mp-xylene, o-xylene, toluene, 1,2,4-trimethylbenzene, 2,4-dimethylpentane, ethyl benzene, propylene, 1-pentene, and isoprene are the key species contributing 77 % to the total ozone formation potential (OFP). The spatial distribution of the emissions shows the emissions and OFPs are mainly concentrated in the urban and industrial areas along the Yangtze River and around Hangzhou Bay. The industrial sources, including power plants other fuel combustion facilities, and non-combustion processes contribute about 97 %, 86 %, 89 %, 91 %, and 69 % of the total SO2, NOx, PM10, PM2.5, and VOC emissions. Vehicles take up 12.3 % and 12.4 % of the NOx and VOC emissions, respectively. Regarding OFPs, the chemical industry, domestic use of paint & printing, and gasoline vehicles contribute 38 %, 24 %, and 12 % to the ozone formation in the YRD region.


2019 ◽  
Vol 206 ◽  
pp. 170-182 ◽  
Author(s):  
Tong Sha ◽  
Xiaoyan Ma ◽  
Hailing Jia ◽  
Ronald J. van der A ◽  
Jieying Ding ◽  
...  

2020 ◽  
Vol 12 (19) ◽  
pp. 7872
Author(s):  
Yijia Huang ◽  
Jiaqi Zhang ◽  
Jinqun Wu

Rapid urbanization has led to a growing number of environmental challenges in large parts of China, where the Yangtze River Delta (YRD) urban agglomerations serve as a typical example. To evaluate the relationship between environmental sustainability gaps and urbanization in 26 cities of the YRD, this study revisited the environmental sustainability assessment (ESA) by combining the metrics of environmental footprints and planetary boundaries at the city level, and then integrated the footprint-boundary ESA framework into decoupling analysis. The results demonstrated considerable spatiotemporal heterogeneity in the environmental sustainability of water use, land use, carbon emissions, nitrogen emissions, phosphorus emissions and PM2.5 emissions across the YRD cities during the study period 2007–2017. Decoupling analysis revealed a positive sign that more than half of the 26 cities had achieved the decoupling of each category of environmental sustainability gaps from urbanization since 2014, especially for nitrogen and phosphorus emissions. On the basis of ESA and decoupling analysis, all the cities were categorized into six patterns, for which the optimal pathways towards sustainable development were discussed in depth. Our study will assist policy makers in formulating more tangible and differentiated policies to achieve decoupling between environmental sustainability gaps and urbanization.


2016 ◽  
Author(s):  
Lei Shu ◽  
Min Xie ◽  
Tijian Wang ◽  
Pulong Chen ◽  
Yong Han ◽  
...  

Abstract. Severe high ozone (O3) episodes usually have close relations to synoptic systems. A regional continuous O3 pollution episode is detected over the Yangtze River Delta (YRD) region in China during August 7–12, 2013, in which the O3 concentrations in more than half of the cities exceeding the national air quality standard. The maximum hourly concentration of O3 reaches 167.1 ppb. By means of the observational analysis and the WRF/CMAQ numerical simulation, the characteristics and the essential impact factors of the typical regional O3 pollution is integratedly investigated. The observational analysis shows that the atmospheric subsidence dominated by Western Pacific subtropical high plays a crucial role in the formation of high-level O3. The favorable weather conditions, such as extremely high temperature, low relative humidity and weak wind speed, caused by the abnormal strong subtropical high are responsible for the trapping and the chemical production of O3 in the boundary layer. In addition, when the YRD cities at the front of Typhoon Utor, the periphery circulation of typhoon system can enhance the downward airflows and cause worse air pollution. But when the typhoon system weakens the subtropical high, the prevailing southeasterly surface wind leads to the mitigation of the O3 pollution. The Integrated Process Rate (IPR) analysis incorporated in CMAQ is applied to further illustrate the combined influence of subtropical high and typhoon system in this O3 episode. The results show that the vertical diffusion (VDIF) and the gas-phase chemistry (CHEM) are two major contributors to O3 formation. During the episode, the contributions of VDIF and CHEM to O3 maintain the high values over 10 ppb/h in Shanghai, Hangzhou, and Nanjing. On August 10–11, the cities close to the sea are apparently affected by the typhoon system, with the contribution of VDIF increasing to 28.45 ppb/h in Shanghai and 19.76 ppb/h in Hangzhou. When the YRD region is under the control of the typhoon system, the contribution values of all individual processes decrease to a low level in all cities. These results provide an insight for the O3 pollution synthetically impacted by the Western Pacific subtropical high and the tropical cyclone system.


2013 ◽  
Vol 13 (8) ◽  
pp. 21507-21540
Author(s):  
X. Fu ◽  
S. X. Wang ◽  
Z. Cheng ◽  
J. Xing ◽  
B. Zhao ◽  
...  

Abstract. During 1 to 6 May 2011, a dust event was observed in the Yangtze River Delta region (YRD). The highest PM10 concentration reached over 1000 μg m−3 and the visibility was below 3 km. In this study, the Community Multi-scale Air Quality modeling system (CMAQ5.0) coupled with an in-line windblown dust model was used to simulate the formation, spatial and temporal characteristics of this dust event, and analyze its impacts on deposition and photochemistry. The threshold friction velocity for loose smooth surface in the dust model was revised based on Chinese data to improve the model performance. The comparison between predictions and observations indicates the revised model can reproduce the transport and pollution of the event. The simulation results show that the dust event was affected by formation and transport of Mongolian cyclone and cold air. Totally about 695 kt dust particles (PM10) were emitted in Xinjiang Province and Mongolia during 28 to 30 April, the dust band swept northern, eastern China and then arrived in the YRD region on 1 May 2011. The transported dust particles increased the mean surface layer concentrations of PM10 in the YRD region by 372% during 1 to 6 May and the impacts weakened from north to south due to the removal of dust particles along the path. Accompanied by high PM concentration, the dry deposition, wet deposition and total deposition of PM10 in the YRD reached 184.7 kt, 172.6 kt and 357.32 kt, respectively. These deposited particles are very harmful because of their impacts on urban environment as well as air quality and human health when resuspending in the atmosphere. Due to the impacts of mineral dust on atmospheric photolysis, the concentrations of O3 and OH were reduced by 1.5% and 3.1% in the whole China, and by 9.4% and 12.1% in the YRD region, respectively. The work of this manuscript is meaningful for understanding the dust emissions in China as well as for the application of CMAQ in Asia. It is also helpful to understand the formation mechanism and impacts of dust pollution in the YRD.


2020 ◽  
Author(s):  
Jingyu An ◽  
Yiwei Huang ◽  
Cheng Huang ◽  
Xin Wang ◽  
Rusha Yan ◽  
...  

Abstract. A high-resolution air pollutant emission inventory in the Yangtze River Delta (YRD) region was updated for the year 2017 using emission factors and chemical speciation mainly from local measurements in this study. The inventory includes 424 NMVOC species and 43 PM2.5 species, which can be subdivided into 259 specific source categories. The total emissions of SO2, NOx, CO, NMVOCs, PM10, PM2.5, and NH3 in the YRD region in 2017 are 1,552, 3,235, 38,507, 4,875, 3,770, 1,597, and 2,467 Gg, respectively. SO2 and CO emissions are mainly from boilers, accounting for 49 % and 73 %, respectively. Mobile sources dominate the NOx emissions and contribute 57 % of the total. VOC emissions mainly come from industrial sources, occupying 61 %. Dust sources take up to 55 % and 28 % of PM10 and PM2.5 emissions, respectively. Agricultural sources account for 91 % of NH3 emissions. Major PM2.5 species are OC, Ca, Si, PSO4 and EC, accounting for 9.0 %, 7.0 %, 6.4 %, 4.6 % and 4.3 % of total PM2.5 emissions. The main species of VOCs are aromatics, accounting for 25.3 %. OVOCs contribute 21.9 % of total VOC emissions. Toluene has the highest comprehensive contribution to ozone and SOA formation potentials, and the others are 1,2,4-trimethylbenzene, m,p-xylene, propylene, ethene, o-xylene, ethylbenzene and so on. Industrial process and solvent use sources are the main sources of ozone and SOA formation potential, followed by motor vehicles. Among industrial sources, chemical manufacturing, rubber & plastic manufacturing, appliance manufacturing and textile have made relatively outstanding contributions. The inventory can provide scientific guidance for future joint control of air pollutants in the YRD region, China.


2020 ◽  
Vol 15 (1) ◽  
Author(s):  
Lei Ye ◽  
Lingqian Hu

An outbreak of atypical pneumonia, now called COVID-19 and known to be caused by the novel coronavirus SARS-CoV-2, first detected in Wuhan, Hubei Province of the People’s Republic of China in December 2019 and afterwards rapidly spread worldwide. Wuhan and the Yangtze River Delta (YRD) region implemented first-level public health emergency responses to stop the spread of the virus on January 23rd, 2020. We tracked the geographical gravity centre of the disease and calculated spatial autocorrelation to explore the spatiotemporal patterns of distribution of imported and locally disseminated COVID-19 cases under the emergency-response control measure. We also applied polynomial regression analysis to estimate the trend of the COVID-19 in the YRD region before and after the control activities against the spread of the infection were instituted. The results show that the control measures applied have been effective. And, in the YRD region, areas with a large influx of population flow from Wuhan and Hubei Province had high risks of COVID-19. Therefore, identification of the spatiotemporal trends should be the first step when developing effective policies to manage and control any new epidemic. The results are not only informative locally but also useful for the rest of the world.


2016 ◽  
Vol 16 (9) ◽  
pp. 2159-2171 ◽  
Author(s):  
Honglei Wang ◽  
Bin Zhu ◽  
Lijuan Shen ◽  
Honghui Xu ◽  
Junlin An ◽  
...  

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