Analysis of Controlled Rabi Flopping in a Double Rephasing Photon Echo Scheme for Quantum Memories

A double rephasing scheme of a photon echo is analyzed for inversion-free photon echo-based quantum memories using controlled Rabi flopping, where the Rabi flopping is used for phase control of collective atom coherence. Unlike the rephasing-caused π-phase shift in a single rephasing scheme, the control Rabi flopping between the excited state and an auxiliary third state induces coherence inversion. Thus, the absorptive photon echo in a double rephasing scheme can be manipulated to be emissive. Here, we present a quantum coherence control of atom phases in a double rephasing photon echo scheme for emissive photon echoes for quantum memory applications.

Understanding of Collective Atom Phase Control in Modified Photon Echoes for a Near-Perfect Storage Time-Extended Quantum Memory

A near-perfect storage time-extended photon echo-based quantum memory protocol has been analyzed by solving the Maxwell–Bloch equations for a backward scheme in a three-level system. The backward photon echo scheme is combined with a controlled coherence conversion process via controlled Rabi flopping to a third state, where the control Rabi flopping collectively shifts the phase of the ensemble coherence. The propagation direction of photon echoes is coherently determined by the phase-matching condition between the data (quantum) and the control (classical) pulses. Herein, we discuss the classical controllability of a quantum state for both phase and propagation direction by manipulating the control pulses in both single and double rephasing photon echo schemes of a three-level system. Compared with the well-understood uses of two-level photon echoes, the Maxwell–Bloch equations for a three-level system have a critical limitation regarding the phase change when interacting with an arbitrary control pulse area.

Photon echoes and two dimensional spectra of the amide I band of proteins measured by femtosecond IR – Raman spectroscopy

New ultrafast 2D-IR-Raman photon echo spectroscopy techniques are introduced and applied to the structural analysis of proteins.