The Study of the Third Order Nonlinear Susceptibility in GaSe

1982 ◽  
Vol 74 (1) ◽  
pp. 75-78 ◽  
Author(s):  
Yu. F. Solomonov ◽  
V. K. Subashiev
2001 ◽  
Vol 15 (28n30) ◽  
pp. 3809-3812 ◽  
Author(s):  
H. Ishihara ◽  
T. Amakata

An analytical expression of the third order nonlinear susceptibility χ(3) has been derived rigorously for a system of interacting Frenkel excitons in a one-dimensional chain of size N with the periodic boundary conditions. It has been clarified that the magnitude of interacting potential between excitons strongly influences the size dependence of χ(3) in the long wavelength approximation, which is well explained in terms of the cancellation effect between the contributions from [ground state] - [one-exciton] transitions and those from [one-exciton] - [two-exciton state] transitions.


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