Toward ab-initio simulations of multiple ionization processes in intense laser field

2009 ◽  
Vol 366 (1-3) ◽  
pp. 71-84 ◽  
Author(s):  
Thanh-Tung Nguyen-Dang ◽  
Michel Peters ◽  
Sen-Ming Wang ◽  
François Dion
2019 ◽  
Vol 5 (5) ◽  
pp. eaaw1885 ◽  
Author(s):  
Hiroshi Akagi ◽  
Tomohito Otobe ◽  
Ryuji Itakura

Valence molecular orbitals play a crucial role in chemical reactions. Here, we reveal that an intense laser field deforms an inner valence orbital (10a′) in the ethanol molecule. We measure the recoil-frame photoelectron angular distribution (RFPAD), which corresponds to the orientation dependence of the ionization probability of the orbital, using photoelectron-photoion coincidence momentum imaging with a circularly polarized laser pulse. Ab initio simulations show that the orbital deformation depends strongly on the laser field direction and that the measured RFPAD cannot be reproduced without taking the orbital deformation into account. Our findings suggest that the laser-induced orbital deformation occurs before electron emission on a suboptical cycle time scale.


2004 ◽  
Vol 22 (1) ◽  
pp. 45-50 ◽  
Author(s):  
B. SHOKRI ◽  
A.R. NIKNAM ◽  
M. SMIRNOV

Multiple ionization of large clusters when they are irradiated by an intense ultrashort laser pulse is investigated. Different mechanisms, responsible for cluster ionization, are investigated. It is found that the ionization of large clusters, irradiated by a strong intense ultrashort laser pulse, is realized by means of the surface thermoemission.


2005 ◽  
Vol 404 (4-6) ◽  
pp. 365-369 ◽  
Author(s):  
Kazuya Shiratori ◽  
Katsuyuki Nobusada ◽  
Kazuhiro Yabana

1990 ◽  
Vol 39 (6) ◽  
pp. 40
Author(s):  
CHEN RONG-QING ◽  
YAO GUAN-HUA ◽  
XU ZHI-ZHAN

2011 ◽  
Vol 83 (4) ◽  
Author(s):  
S. Bhattacharyya ◽  
Mina Mazumder ◽  
J. Chakrabarti ◽  
F. H. M. Faisal

2011 ◽  
Vol 80 (1) ◽  
pp. 89-93 ◽  
Author(s):  
F. Ungan ◽  
E. Kasapoglu ◽  
C. A. Duque ◽  
U. Yesilgul ◽  
S. Şakiroglu ◽  
...  

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