Novel manganese oxide confined interweaved titania nanotubes for the low-temperature Selective Catalytic Reduction (SCR) of NO x by NH 3

2016 ◽  
Vol 334 ◽  
pp. 1-13 ◽  
Author(s):  
Dimitrios K. Pappas ◽  
Thirupathi Boningari ◽  
Punit Boolchand ◽  
Panagiotis G. Smirniotis
2015 ◽  
Vol 69 (12) ◽  
Author(s):  
Xian-Long Zhang ◽  
Shuang-Shuang Lv ◽  
Cui-Ping Zhang ◽  
Xue-Ping Wu ◽  
Lian-Feng Zhang ◽  
...  

AbstractPalygorskite (PG)-supported manganese oxide catalysts (MnOx/PG) were prepared for the selective catalytic reduction (SCR) of NO with ammonia in the presence of SO


RSC Advances ◽  
2015 ◽  
Vol 5 (37) ◽  
pp. 29353-29361 ◽  
Author(s):  
Sihui Zhan ◽  
Dandan Zhu ◽  
Mingying Qiu ◽  
Hongbing Yu ◽  
Yi Li

Highly ordered mesoporous MnO2 was prepared using KIT-6 as a hard template, for selective catalytic reduction (SCR) of NO with NH3 at low temperature, which was characterized using TEM, XRD, BET, XPS, H2-TPR, NH3-TPD and in situ DRIFT.


Author(s):  
Huiling Zheng ◽  
Renjie Li ◽  
Chengming Zhong ◽  
Zhi Li ◽  
Yikun Kang ◽  
...  

Many transition metal oxides supported on TiO2 have been studied for selective catalytic reduction (SCR) of NO with NH3. However, the trade-off exists between the low-temperature activity and N2 selectivity....


Catalysts ◽  
2020 ◽  
Vol 10 (2) ◽  
pp. 202
Author(s):  
Long Lu ◽  
Xueman Wang ◽  
Chunhua Hu ◽  
Ying Liu ◽  
Xiongbo Chen ◽  
...  

Nanosized V-Ce oxides supported on TiO2 (VCT) were prepared and utilized in the low-temperature selective catalytic reduction (SCR) of NO with NH3. Compared with the other V-Ce oxides-based catalysts supported on Al2O3, ZrO2, and ZSM-5, VCT showed the best SCR activity in a low-temperature range. The NOx conversion of 90% could be achieved at 220 °C. Characterizations including X-ray diffraction (XRD), scanning election micrograph (SEM), transmission electron microscopy (TEM), X-ray photoelectron spectroscopy (XPS), temperature-programmed desorption with NH3 (NH3-TPD), and temperature-programmed reduction with H2 (H2-TPR) showed that V1.05Ce1/TiO2 exhibited a good dispersion of V2O5, enrichment of surface Ce3+ and chemical-absorbed oxygen, and excellent redox capacity and acidity, which resulted in the best SCR performance at low temperature.


2011 ◽  
Vol 356-360 ◽  
pp. 974-979 ◽  
Author(s):  
Xian Long Zhang ◽  
Bo Wen Shi ◽  
Xue Ping Wu ◽  
Wei Ping Jiang ◽  
Bao Jun Yang ◽  
...  

Palygorskite supported manganese oxide catalysts (MnOx/PG) were prepared for lower temperature selective catalytic reduction (SCR) of NOx by NH3. Catalyst’s SCR activity was estimated at varied temperatures. Catalyst’s properties were characterized by XRD, NH3adsorption and TPD. Results showed that MnOx/PG catalyst was highly active for SCR at low-temperature. It was also found that NH3 was mainly adsorbed on palygorskite in two forms. Weakly adsorbed NH3, which was seldom inhibited by loading of MnOx, but was more favorable to SCR. Whereas strongly adsorbed NH3was more likely to be inhibited by MnOx loading but was inessential for SCR.


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