Transition metal oxides supported on active carbons as low temperature catalysts for the selective catalytic reduction (SCR) of NO with NH3

1998 ◽  
Vol 18 (3-4) ◽  
pp. 199-213 ◽  
Author(s):  
J. Pasel ◽  
P. Käßner ◽  
B. Montanari ◽  
M. Gazzano ◽  
A. Vaccari ◽  
...  
Keyword(s):  
Low Temperature ◽  
Transition Metal ◽  
Metal Oxides ◽  
Selective Catalytic Reduction ◽  
Transition Metal Oxides ◽  
Catalytic Reduction ◽  
Active Carbons ◽  
Scr Of No

Theoretical Design of Transition Metal-Doped TiO2 for the Selective Catalytic Reduction of NO with NH3 by DFT Calculations

2022 ◽  
Author(s):  
Huiling Zheng ◽  
Renjie Li ◽  
Chengming Zhong ◽  
Zhi Li ◽  
Yikun Kang ◽  
...  
Keyword(s):  
Low Temperature ◽  
Transition Metal ◽  
Selective Catalytic Reduction ◽  
Transition Metal Oxides ◽  
Catalytic Reduction ◽  
Trade Off ◽  
Reduction Of No ◽  
Theoretical Design ◽  
Scr Of No ◽  
Metal Doped

Many transition metal oxides supported on TiO2 have been studied for selective catalytic reduction (SCR) of NO with NH3. However, the trade-off exists between the low-temperature activity and N2 selectivity....

Facile fabrication of hollow tubular mixed oxides for selective catalytic reduction of NOx at low temperature: a combined experimental and theoretical study

2017 ◽  
Vol 53 (5) ◽  
pp. 967-970 ◽  
Author(s):  
Xiuyun Wang ◽  
Zhixin Lan ◽  
Yi Liu ◽  
Yongjin Luo ◽  
Jianjun Chen ◽  
...  
Keyword(s):  
Low Temperature ◽  
Transition Metal ◽  
Metal Oxides ◽  
Transition Metal Oxides ◽  
Theoretical Study ◽  
Mixed Oxides ◽  
Catalytic Reduction ◽  
Heating Rates ◽  
Facile Fabrication ◽  
Reduction Of Nox

The 1D nanowire or hollow tubular structure of various transition metal oxides can be tuned by controlling heating rates.

Titania Supported Bimetallic Transition Metal Oxides for Low-Temperature SCR of NO with NH3

2006 ◽  
Vol 45 (19) ◽  
pp. 6444-6449 ◽  
Author(s):  
Pavani M. Sreekanth ◽  
Donovan A. Peña ◽  
Panagiotis G. Smirniotis
Keyword(s):  
Low Temperature ◽  
Transition Metal ◽  
Metal Oxides ◽  
Transition Metal Oxides ◽  
Scr Of No ◽  
Low Temperature Scr

Low-Temperature Selective Catalytic Reduction of NO with NH3 Over Mn-Fe Mixed Metal Oxides on the Nitric Vapor Functionalized Carbon Nanotubes Prepared by a Polyol Process

NANO ◽  
2017 ◽  
Vol 12 (04) ◽  
pp. 1750048
Author(s):  
Xin Lv ◽  
Liheng Zhang ◽  
Sheng Zhan ◽  
Zhen Li ◽  
Yi Zeng
Keyword(s):  
Carbon Nanotubes ◽  
Low Temperature ◽  
Metal Oxides ◽  
Selective Catalytic Reduction ◽  
Catalytic Reduction ◽  
Polyol Process ◽  
Mixed Metal Oxides ◽  
Functionalized Carbon Nanotubes ◽  
X Ray ◽  
Scr Of No

Highly dispersed Mn-Fe mixed metal oxides were supported on the nitric vapor functionalized carbon nanotubes (CNTs) by the polyol process for the low-temperature selective catalytic reduction (SCR) of NO with NH3. X-ray diffraction (XRD), transmission electron microscopy (TEM), X-ray photoelectron spectroscopy (XPS), H2 temperature-programmed reduction (H2-TPR) and Fourier transform infrared (FT-IR) spectroscopy have been used to elucidate the structure and surface properties of the obtained catalysts. It was found that the Mn-Fe/VF-CNTs catalysts synthesized by the polyol process exhibited higher activity and more extensive operating-temperature window, compared to the catalysts prepared by the impregnation method. On the basis of the catalyst characterization, the better dispersion of metal oxides on the CNTs surface, the more chemisorbed oxygen species, the higher Mn[Formula: see text]/Mn and O[Formula: see text]/O[Formula: see text]O[Formula: see text] ratios played key roles in the excellent catalytic performance of the catalyst in the low-temperature SCR of NO to N2 with NH3.

Influence of transition metal (Fe, Co, and Ag) doping on the MnOx–CeO2/Ti-bearing blast furnace slag catalyst for selective catalytic reduction of NOx with NH3 at low temperature

2017 ◽  
Vol 41 (19) ◽  
pp. 11299-11307 ◽  
Author(s):  
Rong Liu ◽  
Yifan Xu ◽  
Fei Ye ◽  
Feng Jia ◽  
Rui Xu
Keyword(s):  
Blast Furnace ◽  
Low Temperature ◽  
Transition Metal ◽  
Solid Waste ◽  
Selective Catalytic Reduction ◽  
Blast Furnace Slag ◽  
Catalytic Reduction ◽  
Industrial Solid Waste ◽  
Reduction Of Nox ◽  
Furnace Slag

Mn–Ce based catalysts supported on Ti-bearing blast furnace slag (industrial solid waste) and the doping of transition metals were studied.

scholarly journals Nanosized V-Ce Oxides Supported on TiO2 as a Superior Catalyst for the Selective Catalytic Reduction of NO

Catalysts ◽  
2020 ◽  
Vol 10 (2) ◽  
pp. 202
Author(s):  
Long Lu ◽  
Xueman Wang ◽  
Chunhua Hu ◽  
Ying Liu ◽  
Xiongbo Chen ◽  
...  
Keyword(s):  
Low Temperature ◽  
Selective Catalytic Reduction ◽  
Photoelectron Spectroscopy ◽  
Catalytic Reduction ◽  
X Ray Diffraction ◽  
X Ray ◽  
Transmission Electron ◽  
Redox Capacity ◽  
Scr Of No ◽  
Temperature Programmed

Nanosized V-Ce oxides supported on TiO2 (VCT) were prepared and utilized in the low-temperature selective catalytic reduction (SCR) of NO with NH3. Compared with the other V-Ce oxides-based catalysts supported on Al2O3, ZrO2, and ZSM-5, VCT showed the best SCR activity in a low-temperature range. The NOx conversion of 90% could be achieved at 220 °C. Characterizations including X-ray diffraction (XRD), scanning election micrograph (SEM), transmission electron microscopy (TEM), X-ray photoelectron spectroscopy (XPS), temperature-programmed desorption with NH3 (NH3-TPD), and temperature-programmed reduction with H2 (H2-TPR) showed that V1.05Ce1/TiO2 exhibited a good dispersion of V2O5, enrichment of surface Ce3+ and chemical-absorbed oxygen, and excellent redox capacity and acidity, which resulted in the best SCR performance at low temperature.

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