Size Mismatch Induces Cation Segregation in CsPbI3: Forming Energy Level Gradient and 3D/2D Heterojunction Promotes the Efficiency of Carbon-based Perovskite Solar Cells to over 15%

Nano Energy ◽  
2021 ◽  
pp. 106411
Author(s):  
Hailiang Wang ◽  
Huicong Liu ◽  
Zijing Dong ◽  
Tinglu Song ◽  
Weiping Li ◽  
...  
2020 ◽  
Vol 8 (25) ◽  
pp. 12723-12734 ◽  
Author(s):  
Yang Yang ◽  
Minh Tam Hoang ◽  
Disheng Yao ◽  
Ngoc Duy Pham ◽  
Vincent Tiing Tiong ◽  
...  

Carbon electrode-based planar PSCs demonstrated higher device performance and reduced hysteresis using a CuSCN based HTL owing to its favourable energy level alignment with the perovskite compared to conventional spiro-OMeTAD based HTL.


Nano Energy ◽  
2021 ◽  
pp. 106285
Author(s):  
Yousheng Wang ◽  
Hui Ju ◽  
Tahmineh Mahmoudi ◽  
Chong Liu ◽  
Cuiling Zhang ◽  
...  

2021 ◽  
Vol 16 (1) ◽  
Author(s):  
Chi Zhang ◽  
Zhiyuan He ◽  
Xuanhui Luo ◽  
Rangwei Meng ◽  
Mengwei Chen ◽  
...  

AbstractIn this work, inorganic tin-doped perovskite quantum dots (PQDs) are incorporated into carbon-based perovskite solar cells (PSCs) to improve their photovoltaic performance. On the one hand, by controlling the content of Sn2+ doping, the energy level of the tin-doped PQDs can be adjusted, to realize optimized band alignment and enhanced separation of photogenerated electron–hole pairs. On the other hand, the incorporation of tin-doped PQDs provided with a relatively high acceptor concentration due to the self-p-type doping effect is able to reduce the width of the depletion region near the back surface of the perovskite, thereby enhancing the hole extraction. Particularly, after the addition of CsSn0.2Pb0.8I3 quantum dots (QDs), improvement of the power conversion efficiency (PCE) from 12.80 to 14.22% can be obtained, in comparison with the pristine device. Moreover, the experimental results are analyzed through the simulation of the one-dimensional perovskite/tin-doped PQDs heterojunction.


2021 ◽  
Vol 414 ◽  
pp. 128878
Author(s):  
Cong Geng ◽  
Peng Wei ◽  
Huamei Chen ◽  
Haichao Liu ◽  
Shenshen Zheng ◽  
...  

2018 ◽  
Vol 7 ◽  
pp. 221-231 ◽  
Author(s):  
Miao Duan ◽  
Yue Hu ◽  
Anyi Mei ◽  
Yaoguang Rong ◽  
Hongwei Han

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