scholarly journals Observation of plaquette fluctuations in the spin-1/2 honeycomb lattice

2020 ◽  
Vol 5 (1) ◽  
Author(s):  
Christian Wessler ◽  
Bertrand Roessli ◽  
Karl W. Krämer ◽  
Bernard Delley ◽  
Oliver Waldmann ◽  
...  

AbstractQuantum spin liquids are materials that feature quantum entangled spin correlations and avoid magnetic long-range order at T = 0 K. Particularly interesting are two-dimensional honeycomb spin lattices where a plethora of exotic quantum spin liquids have been predicted. Here, we experimentally study an effective S = 1/2 Heisenberg honeycomb lattice with competing nearest and next-nearest-neighbour interactions. We demonstrate that YbBr3 avoids order down to at least T = 100 mK and features a dynamic spin–spin correlation function with broad continuum scattering typical of quantum spin liquids near a quantum critical point. The continuum in the spin spectrum is consistent with plaquette type fluctuations predicted by theory. Our study is the experimental demonstration that strong quantum fluctuations can exist on the honeycomb lattice even in the absence of Kitaev-type interactions, and opens a new perspective on quantum spin liquids.

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Lucile Savary

AbstractThe search for truly quantum phases of matter is a center piece of modern research in condensed matter physics. Quantum spin liquids, which host large amounts of entanglement—an entirely quantum feature where one part of a system cannot be measured without modifying the rest—are exemplars of such phases. Here, we devise a realistic model which relies upon the well-known Haldane chain phase, i.e. the phase of spin-1 chains which host fractional excitations at their ends, akin to the hallmark excitations of quantum spin liquids. We tune our model to exactly soluble points, and find that the ground state realizes Haldane chains whose physical supports fluctuate, realizing both quantum spin liquid like and symmetry-protected topological phases. Crucially, this model is expected to describe actual materials, and we provide a detailed set of material-specific constraints which may be readily used for an experimental realization.


2020 ◽  
Vol 102 (14) ◽  
Author(s):  
Jiucai Wang ◽  
Qirong Zhao ◽  
Xiaoqun Wang ◽  
Zheng-Xin Liu

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Oliver Hart ◽  
Yuan Wan ◽  
Claudio Castelnovo

AbstractRealistic model Hamiltonians for quantum spin liquids frequently exhibit a large separation of energy scales between their elementary excitations. At intermediate, experimentally relevant temperatures, some excitations are sparse and hop coherently, whereas others are thermally incoherent and dense. Here, we study the interplay of two such species of quasiparticle, dubbed spinons and visons, which are subject to nontrivial mutual statistics – one of the hallmarks of quantum spin liquid behaviour. Our results for $${{\mathbb{Z}}}_{2}$$ Z 2 quantum spin liquids show an intriguing feedback mechanism, akin to the Nagaoka effect, whereby spinons become localised on temperature-dependent patches of expelled visons. This phenomenon has important consequences for the thermodynamic and transport properties of the system, as well as for its response to quenches in temperature. We argue that these effects can be measured in experiments and may provide viable avenues for obtaining signatures of quantum spin liquid behaviour.


2021 ◽  
pp. 2000126
Author(s):  
Cheng Peng ◽  
Yi‐Fan Jiang ◽  
Dong‐Ning Sheng ◽  
Hong‐Chen Jiang

2021 ◽  
Vol 103 (1) ◽  
Author(s):  
Yan-Cheng Wang ◽  
Zheng Yan ◽  
Chenjie Wang ◽  
Yang Qi ◽  
Zi Yang Meng

2021 ◽  
Vol 3 (1) ◽  
Author(s):  
Ilia Khait ◽  
P. Peter Stavropoulos ◽  
Hae-Young Kee ◽  
Yong Baek Kim

2012 ◽  
Vol 44 (5) ◽  
pp. 845-859 ◽  
Author(s):  
Gregory A. Fiete ◽  
Victor Chua ◽  
Mehdi Kargarian ◽  
Rex Lundgren ◽  
Andreas Rüegg ◽  
...  

2021 ◽  
Vol 6 (1) ◽  
Author(s):  
S. Lee ◽  
S.-H. Do ◽  
W. Lee ◽  
Y. S. Choi ◽  
J. van Tol ◽  
...  

AbstractA breathing pyrochlore system is predicted to host a variety of quantum spin liquids. Despite tremendous experimental and theoretical efforts, such sought-after states remain elusive as perturbation terms and lattice distortions lead to magnetic order. Here, we utilize bond alternation and disorder to tune a magnetic ground state in the Cr-based breathing pyrochlore LiGa1−xInxCr4O8. By combining thermodynamic and magnetic resonance techniques, we provide experimental signatures of a spin-liquid-like state in x = 0.8, namely, a nearly T2-dependent magnetic specific heat and persistent spin dynamics by muon spin relaxation (μSR). Moreover, 7Li NMR, ZF-μSR, and ESR unveil the temporal and thermal dichotomy of spin correlations: a tetramer singlet on a slow time scale vs. a spin-liquid-like state on a fast time scale. Our results showcase that a bond disorder in the breathing pyrochlore offers a promising route to disclose exotic magnetic phases.


2018 ◽  
Vol 4 (11) ◽  
pp. eaat5535 ◽  
Author(s):  
Wei Zhu ◽  
Xiao Chen ◽  
Yin-Chen He ◽  
William Witczak-Krempa

Quantum spin liquids (QSLs) are exotic phases of matter that host fractionalized excitations. It is difficult for local probes to characterize QSL, whereas quantum entanglement can serve as a powerful diagnostic tool due to its nonlocality. The kagome antiferromagnetic Heisenberg model is one of the most studied and experimentally relevant models for QSL, but its solution remains under debate. Here, we perform a numerical Aharonov-Bohm experiment on this model and uncover universal features of the entanglement entropy. By means of the density matrix renormalization group, we reveal the entanglement signatures of emergent Dirac spinons, which are the fractionalized excitations of the QSL. This scheme provides qualitative insights into the nature of kagome QSL and can be used to study other quantum states of matter. As a concrete example, we also benchmark our methods on an interacting quantum critical point between a Dirac semimetal and a charge-ordered phase.


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