scholarly journals Low-temperature MIR to submillimeter mass absorption coefficient of interstellar dust analogues

2017 ◽  
Vol 606 ◽  
pp. A50 ◽  
Author(s):  
K. Demyk ◽  
C. Meny ◽  
H. Leroux ◽  
C. Depecker ◽  
J.-B. Brubach ◽  
...  

Context. To model the cold dust emission observed in the diffuse interstellar medium, in dense molecular clouds or in cold clumps that could eventually form new stars, it is mandatory to know the physical and spectroscopic properties of this dust and to understand its emission. Aims. This work is a continuation of previous studies aiming at providing astronomers with spectroscopic data of realistic cosmic dust analogues for the interpretation of observations. The aim of the present work is to extend the range of studied analogues to iron-rich silicate dust analogues. Methods. Ferromagnesium amorphous silicate dust analogues were produced by a sol-gel method with a mean composition close to Mg1−xFexSiO3 with x = 0.1, 0.2, 0.3, 0.4. Part of each sample was annealed at 500 °C for two hours in a reducing atmosphere to modify the oxidation state of iron. We have measured the mass absorption coefficient (MAC) of these eight ferromagnesium amorphous silicate dust analogues in the spectral domain 30−1000 μm for grain temperature in the range 10−300 K and at room temperature in the 5−40 μm range. Results. The MAC of ferromagnesium samples behaves in the same way as the MAC of pure Mg-rich amorphous silicate samples. In the 30−300 K range, the MAC increases with increasing grain temperature whereas in the range 10−30 K, we do not see any change of the MAC. The MAC cannot be described by a single power law in λ− β. The MAC of the samples does not show any clear trend with the iron content. However the annealing process has, on average, an effect on the MAC that we explain by the evolution of the structure of the samples induced by the processing. The MAC of all the samples is much higher than the MAC calculated by dust models. Conclusions. The complex behavior of the MAC of amorphous silicates with wavelength and temperature is observed whatever the exact silicate composition (Mg vs. Fe amount). It is a universal characteristic of amorphous materials, and therefore of amorphous cosmic silicates, that should be taken into account in astronomical modeling. The enhanced MAC of the measured samples compared to the MAC calculated for cosmic dust model implies that dust masses are overestimated by the models.

2017 ◽  
Vol 600 ◽  
pp. A123 ◽  
Author(s):  
K. Demyk ◽  
C. Meny ◽  
X.-H. Lu ◽  
G. Papatheodorou ◽  
M. J. Toplis ◽  
...  

1992 ◽  
Vol 7 (4) ◽  
pp. 194-196 ◽  
Author(s):  
Stefano Battaglia ◽  
Marco Franzini ◽  
Leonardo Leoni

AbstractThis paper describes a new method for the simultaneous determination of mineral composition, mass thickness and mass absorption coefficient of a thin layer of a crystalline substance deposited on a crystalline substrate.The samples were deposited on membrane disc filters, consisting of mixtures of cellulose acetate and cellulose nitrate. Quantitative results are achieved by measuring the diffraction intensity of the analyte and the attenuation of a reflection of the crystalline material supporting the deposited sample. The mean accuracy of the analysis was found to be: ≈ 3% for mass thickness, ≈ 1% for mass absorption coefficient and ≈ 4% for quantitative mineralogical determination.


Author(s):  
Masashi Nashimoto ◽  
Makoto Hattori ◽  
Ricardo Génova-Santos ◽  
Frédérick Poidevin

Abstract Complete studies of the radiative processes of thermal emission from the amorphous dust from microwave through far-infrared wavebands are presented by taking into account, self-consistently for the first time, the standard two-level systems (TLS) model of amorphous materials. The observed spectral energy distributions (SEDs) for the Perseus molecular cloud (MC) and W 43 from microwave through far-infrared are fitted with the SEDs calculated with the TLS model of amorphous silicate. We have found that the model SEDs reproduce the observed properties of the anomalous microwave emission (AME) well. The present result suggests an alternative interpretation for the AME being carried by the resonance emission of the TLS of amorphous materials without introducing new species. Simultaneous fitting of the intensity and polarization SEDs for the Perseus MC and W 43 are also performed. The amorphous model reproduces the overall observed feature of the intensity and polarization SEDs of the Perseus MC and W 43. However, the model’s predicted polarization fraction of the AME is slightly higher than the QUIJOTE upper limits in several frequency bands. A possible improvement of our model to resolve this problem is proposed. Our model predicts that interstellar dust is amorphous materials with very different physical characteristics compared with terrestrial amorphous materials.


1969 ◽  
Vol 13 ◽  
pp. 632-638 ◽  
Author(s):  
P. Lublin ◽  
P. Cukor ◽  
R. J. Jaworowski

For quantitative electron probe analysis, the raw intensity ratios must be corrected to take into account deviations due to absorption, fluoresecnce and electron beam penetration. The major correction is usually the absorption correction, so that for best results, accurate mass absorption coefficients are required. Many tables of absorption coefficients are calculated by interpolation or extrapolation from available measured values, and therefore new measurements are required for increased reliability. The region which requires the most attention for present-day probe analysis is the 2 to 10 Å range.Thin foils of the lighter metals are available for mass absorption coefficient measurements, but heavy metal foils, which must be extremely thin, are not obtainable, A method has been developed to prepare thin films of heavy metals on a suitable substrate by pyrolytic decomposition of metal organic compounds.


1990 ◽  
Vol 34 ◽  
pp. 325-335 ◽  
Author(s):  
Steve J. Chipera ◽  
David L. Bish

AbstractThe mass absorption coefficient is a useful parameter for quantitative characterization of materials. If the chemical composition of a sample is known, the mass absorption coefficient can be calculated directly. However, the mass absorption coefficient must be determined empirically if the chemical composition is unknown. Traditional methods for determining the mass absorption coefficient involve measuring the transmission of monochromatic X-rays through a sample of known thickness and density. Reynolds (1963,1967), however, proposed a method for determining the mass absorption coefficient by measuring the Compton or inelastic X-ray scattering from a sample using Mo radiation on an X-ray fluorescence spectrometer (XRF). With the recent advances in solid-state detectors/electronics for use with conventional powder diffractometers, it is now possible to readily determine mass absorption coefficients during routine X-ray diffraction (XRD) analyses.Using Cu Kα radiation and Reynolds’ method on a Siemens D-500 diffractometer fitted with a Kevex Si(Li) solid-state detector, we have measured the mass absorption coefficients of a suite of minerals and pure chemical compounds ranging in μ/ρ from graphite to Fe-metal (μ/ρ = 4.6-308 using Cu Kα radiation) to ±4.0% (lσ). The relationship between the known mass absorption coefficient and the inverse count rate is linear with a correlation coefficient of 0.997. Using mass absorption coefficients, phase abundances can be determined during quantitative XRD analysis without requiring the use of an internal standard, even when an amorphous component is present.


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