On the detection of mesospheric meteoric smoke particles embedded in noctilucent cloud particles with rocket-borne dust probes

2015 ◽  
Vol 86 (3) ◽  
pp. 033305 ◽  
Author(s):  
T. Antonsen ◽  
O. Havnes
2012 ◽  
Vol 12 (1) ◽  
pp. 1553-1584
Author(s):  
R. W. Saunders ◽  
S. Dhomse ◽  
W. S. Tian ◽  
M. P. Chipperfield ◽  
J. M. C. Plane

Abstract. Nano-sized meteoric smoke particles (MSPs) with iron-magnesium silicate compositions, formed in the upper mesosphere as a result of meteoric ablation, may remove sulphuric acid from the gas-phase above 40 km and may also affect the composition and behaviour of supercooled H2SO4-H2O droplets in the global stratospheric aerosol (Junge) layer. This study describes a time-resolved spectroscopic analysis of the evolution of the ferric (Fe3+) ion originating from amorphous ferrous (Fe2+)-based silicate powders dissolved in varying Wt % sulphuric acid (30–75%) solutions over a temperature range of 223–295 K. Complete dissolution of the particles was observed under all conditions. The first-order rate coefficient for dissolution decreases at higher Wt % and lower temperature, which is consistent with the increased solution viscosity limiting diffusion of H2SO4 to the particle surfaces. Dissolution under stratospheric conditions should take less than a week, and is much faster than the dissolution of crystalline Fe2+ compounds. The chemistry climate model UMSLIMCAT (based on the UKMO Unified Model) was then used to study the transport of MSPs through the middle atmosphere. A series of model experiments were performed with different uptake coefficients. Setting the concentration of 1.5 nm radius MSPs at 80 km to 3000 cm−3 (based on rocket-borne charged particle measurements), the model matches the reported Wt % Fe values of 0.5–1.0 in Junge layer sulphate particles, and the MSP optical extinction between 40 and 75 km measured by a satellite-borne spectrometer, if the global meteoric input rate is about 20 t d−1. The model indicates that an uptake coefficient ≥0.01 is required to account for the observed two orders of magnitude depletion of H2SO4 vapour above 40 km.


Tellus ◽  
1964 ◽  
Vol 16 (1) ◽  
pp. 84-88 ◽  
Author(s):  
C. L. Hemenway ◽  
R. K. Soberman ◽  
G. Witt

2006 ◽  
Vol 6 (12) ◽  
pp. 4415-4426 ◽  
Author(s):  
L. Megner ◽  
M. Rapp ◽  
J. Gumbel

Abstract. Meteoroids entering the Earth's atmosphere experience strong deceleration and ablate, whereupon the resulting material is believed to re-condense to nanometre-size "smoke particles". These particles are thought to be of great importance for many middle atmosphere phenomena, such as noctilucent clouds, polar mesospheric summer echoes, metal layers, and heterogeneous chemistry. The properties and distribution of meteoric smoke depend on poorly known or highly variable factors such as the amount, composition and velocity of incoming meteoric material, the efficiency of coagulation, and the state and circulation of the atmosphere. This work uses a one-dimensional microphysical model to investigate the sensitivities of meteoric smoke properties to these poorly known or highly variable factors. The resulting uncertainty or variability of meteoric smoke quantities such as number density, mass density, and size distribution are determined. It is found that the two most important factors are the efficiency of the coagulation and background vertical wind. The seasonal variation of the vertical wind in the mesosphere implies strong global and temporal variations in the meteoric smoke distribution. This contrasts the simplistic picture of a homogeneous global meteoric smoke layer, which is currently assumed in many studies of middle atmospheric phenomena. In particular, our results suggest a very low number of nanometre-sized smoke particles at the summer mesopause where they are thought to serve as condensation nuclei for noctilucent clouds.


2017 ◽  
Vol 162 ◽  
pp. 178-191 ◽  
Author(s):  
Alexander D. James ◽  
Victoria L.F. Frankland ◽  
Josep M. Trigo-Rodríguez ◽  
Jacinto Alonso-Azcárate ◽  
Juan Carlos Gómez Martín ◽  
...  

2021 ◽  
Vol 39 (6) ◽  
pp. 1055-1068
Author(s):  
Margaretha Myrvang ◽  
Carsten Baumann ◽  
Ingrid Mann

Abstract. We investigate if the presence of meteoric smoke particles (MSPs) influences the electron temperature during artificial heating in the D-region. By transferring the energy of powerful high-frequency radio waves into thermal energy of electrons, artificial heating increases the electron temperature. Artificial heating depends on the height variation of electron density. The presence of MSPs can influence the electron density through charging of MSPs by electrons, which can reduce the number of free electrons and even result in height regions with strongly reduced electron density, so-called electron bite-outs. We simulate the influence of the artificial heating by calculating the intensity of the upward-propagating radio wave. The electron temperature at each height is derived from the balance of radio wave absorption and cooling through elastic and inelastic collisions with neutral species. The influence of MSPs is investigated by including results from a one-dimensional height-dependent ionospheric model that includes electrons, positively and negatively charged ions, neutral MSPs, singly positively and singly negatively charged MSPs, and photochemistry such as photoionization and photodetachment. We apply typical ionospheric conditions and find that MSPs can influence both the magnitude and the height profile of the heated electron temperature above 80 km; however, this depends on ionospheric conditions. During night, the presence of MSPs leads to more efficient heating and thus a higher electron temperature above altitudes of 80 km. We found differences of up to 1000 K in electron temperature for calculations with and without MSPs. When MSPs are present, the heated electron temperature decreases more slowly. The presence of MSPs does not much affect the heating below 80 km for night conditions. For day conditions, the difference between the heated electron temperature with MSPs and without MSPs is less than 25 K. We also investigate model runs using MSP number density profiles for autumn, summer and winter. The night-time electron temperature is expected to be 280 K hotter in autumn than during winter conditions, while the sunlit D-region is 8 K cooler for autumn MSP conditions than for the summer case, depending on altitude. Finally, an investigation of the electron attachment efficiency to MSPs shows a significant impact on the amount of chargeable dust and consequently on the electron temperature.


2021 ◽  
Author(s):  
Margaretha Myrvang ◽  
Carsten Baumann ◽  
Ingrid Mann

<p>Artificial heating increases the electron temperature by transferring the energy of powerful high frequency radio waves into thermal energy of electrons. Current models most likely overestimate the effect of artificial heating in the D-region compared to observations [1, 2]. We investigate if the presence of meteoric smoke particles can explain the discrepancy between observations and model. The ionospheric D-region varies in altitude range from about 50 km to 100 km. In the D-region, the electron density is low, the neutral density is relatively high and it is here that meteors ablate. The ablated meteoric material is believed to recondense to form meteoric smoke particles (MSP). The presence of MSP in the D-region can influence plasma densities through charging of dust by electrons and ions, depending on different ionospheric conditions. Charging of dust influence the electron density mainly through electron attachment to the dust, which results in height regions with less electron density. The heating effect varies with electron density height profile [3], since the reduction in radio wave energy is due to absorption by electrons. We study artificial heating of the D-region and consider MSP by using a one-dimensional ionospheric model [4], which also includes photochemistry. In the ionospheric model, we assume that artificial heating only influences the chemical reactions that depend on electron temperature. We model the electron temperature increase during artificial heating with an electron density calculated from the ionospheric model, where we will do the modelling with and without the MSP and compare day and night condition. Our results show a difference in electron temperature increase with the MSP compared to without the MSP and between day and night condition.</p><p>References:</p><ul><li>[1] Senior, A., M. T. Rietveld, M. J. Kosch and W. Singer (2010): «Diagnosing radio plasma heating in the polar summer mesosphere using cross modulation: Theory and observations». Journal of geophysical research, Vol. 115, A09318.</li> <li>[2] Kero, A., C.-F Enell, Th. Ulich, E. Turunen, M. T. Rietveld and F. H. Honary (2007): «Statistical signature of active D-region HF heating in IRIS riometer data from 1994-2004». Ann. Geophys., 25, 407-415.</li> <li>[3] Kassa, M., O. Havnes and E. Belova (2005): «The effect of electron bite-outs on artificial electron heating and the PMSE overshoot». Annales Geophysicae, 23, 3633-3643.</li> <li>[4] Baumann, C., M. Rapp, A. Kero and C.-F. Enell (2013): «Meteor smoke influence on the D-region charge balance –review of recent in situ measurements and one-dimensional model results». Ann. Geophys., 31, 2049-2062.</li> </ul>


Tellus ◽  
1964 ◽  
Vol 16 (1) ◽  
pp. 89-95 ◽  
Author(s):  
R. K. Soberman ◽  
S. A. Chrest ◽  
J. J. Manning ◽  
L. Rey ◽  
T. G. Ryan ◽  
...  

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