A Comparison of Convective and Stratiform Precipitation Microphysics of the Record-Breaking Typhoon In-Fa (2021)

In July 2021, Typhoon In-Fa attacked eastern China and broke many records for extreme precipitation over the last century. Such an unrivaled impact results from In-Fa’s slow moving speed and long residence time due to atmospheric circulations. With the supports of 66 networked surface disdrometers over eastern China and collaborative observations from the advanced GPM satellite, we are able to reveal the unique precipitation microphysical properties of the record-breaking Typhoon In-Fa (2021). After separating the typhoon precipitation into convective and stratiform types and comparing the drop size distribution (DSD) properties of Typhoon In-Fa with other typhoons from different climate regimes, it is found that typhoon precipitation shows significant internal differences as well as regional differences in terms of DSD-related parameters, such as mass-weighted mean diameter (Dm), normalized intercept parameter (Nw), radar reflectivity (Z), rain rate (R), and intercept, shape, and slope parameters (N0, µ, Λ). Comparing different rain types inside Typhoon In-Fa, convective rain (Nw ranging from 3.80 to 3.96 mm−1 m−3) shows higher raindrop concentration than stratiform rain (Nw ranging from 3.40 to 3.50 mm−1 m−3) due to more graupels melting into liquid water while falling. Large raindrops occupy most of the region below the melting layer in convective rain due to a dominant coalescence process of small raindrops (featured by larger ZKu, Dm, and smaller N0, µ, Λ), while small raindrops account for a considerable proportion in stratiform rain, reflecting a significant collisional breakup process of large raindrops (featured by smaller ZKu, Dm, and larger N0, µ, Λ). Compared with other typhoons in Hainan and Taiwan, the convective precipitation of Typhoon In-Fa shows a larger (smaller) raindrop concentration than that of Taiwan (Hainan), while smaller raindrop diameter than both Hainan and Taiwan. Moreover, the typhoon convective precipitation measured in In-Fa is more maritime-like than precipitation in Taiwan. Based on a great number of surface disdrometer observational data, the GPM precipitation products were further validated for both rain types, and a series of native quantitative precipitation estimation relations, such as Z–R and R–Dm relations were derived to improve the typhoon rainfall retrieval for both ground-based radar and spaceborne radar.

The influence of multiple groups of biological ice nucleating particles on microphysical properties of mixed-phase clouds observed during MC3E

A new empirical parameterization (EP) for multiple groups of primary biological aerosol particles (PBAPs) is implemented in the aerosol cloud model (AC) to investigate their roles as ice-nucleating particles (INPs). The EP describes the heterogeneous ice nucleation by (1) fungal spores, (2) bacteria, (3) pollen, (4) detritus of plants, animals, and viruses, and (5) algae. Each group includes fragments from the originally emitted particles. A high-resolution simulation of a midlatitude mesoscale squall line by AC is validated against airborne and ground observations. Sensitivity tests are carried out by varying the initial vertical profiles of the loadings of individual PBAP groups. The resulting changes in warm and ice microphysical parameters are investigated. Overall, PBAPs have little effect on the ice phase, especially in the convective region. In the stratiform region, increasing the initial PBAP loadings by a factor of 100 resulted in less than 60 % change in ice number concentrations. The total ice concentration is mostly controlled by various mechanisms of secondary ice production (SIP). However, when SIP is artificially prohibited in sensitivity tests, increasing the PBAP loading by a factor of 100 has no significant effect on the ice phase. Further sensitivity tests revealed that PBAPs have little effect on surface precipitation as well as on shortwave and longwave flux.

Vertical Distributions of Aerosol and Cloud Microphysical Properties and the Aerosol Impact on a Continental Cumulus Cloud Based on Aircraft Measurements From the Loess Plateau of China

Based on aircraft measurements of aerosols and continental cumulus clouds made over the Loess Plateau of China (Xinzhou, Shanxi Province) on 30 July 2020, this study focuses on the vertical profiles of microphysical properties of aerosols and cumulus clouds, and use them to study aerosol-cloud interactions. During the study period, the boundary layer was stable with a height ∼1,500 m above sea level. Aerosols in the boundary layer mainly came from local emissions, while aerosols above this layer were mostly dust aerosols transported over long distances. Vertical profiles of aerosols and cloud condensation nuclei were obtained, and aerosol activation ratios at different supersaturation (SS) levels ranged from 0.16 to 0.32 at 0.2% SS and 0.70 to 0.85 at 0.8% SS. A thick cumulus cloud in the development stage was observed from the bottom to the top with the horizontal dimension of 10 km by 7 km, the cloud-base height of 2,450 m (15.8°C), and the cloud-top height of 5,400 m (−3°C). The maximum updraft velocity near the cloud top was 13.45 m s−1, and the maximum downdraft velocity occuring in the upper-middle part of the cloud was 4.44 ms−1. The temperature inside the cloud was higher than the outside, with their difference being positively correlated with the cloud water content. The temperature lapse rate inside the cloud was about −6.5°C km−1. The liquid water content and droplet effective radius (Re) increased with increasing height. The cloud droplet number concentration (Nc) increased first then decreased, peaking in the middle and lower part of the cloud, the average values of Nc and Re were 767.9 cm−3 and 5.17 μm, respectively. The cloud droplet spectrum had a multi-peak distribution, with the first appearing at ∼4.5 μm. SS in the cloud first increased then decreased with height. The maximum SS is ∼0.7% appearing at ∼3,800 m. The conversion rate of intra-cloud aerosols to cloud droplets was between 0.2 and 0.54, with the ratio increasing gradually with increasing height. The cloud droplet spectral dispersion and Nc were positively correlated. The aerosol indirect effect (AIE) was estimated to be 0.245 and 0.16, based on Nc and Re, respectively. The cloud droplet dispersion mainly attenuated the AIE, up to ∼34.7%.

EUREC⁴A observations from the SAFIRE ATR42 aircraft

As part of the EUREC4A (Elucidating the role of cloud-circulation coupling in climate) field campaign, which took place in January and February 2020 over the western tropical Atlantic near Barbados, the French SAFIRE ATR42 research aircraft conducted 19 flights in the lower troposphere. Each flight followed a common flight pattern that sampled the atmosphere around the cloud-base level, at different heights of the subcloud layer, near the sea surface and in the lower free troposphere. The aircraft's payload included a backscatter lidar and a Doppler cloud radar that were both horizontally oriented, a Doppler cloud radar looking upward, microphysical probes, a cavity ring-down spectrometer for water isotopes, a multiwavelength radiometer, a visible camera and multiple meteorological sensors, including fast rate sensors for turbulence measurements. With this instrumentation, the ATR characterized the macrophysical and microphysical properties of trade-wind clouds together with their thermodynamical, turbulent and radiative environment. This paper presents the airborne operations, the flight segmentation, the instrumentation, the data processing and the EUREC4A datasets produced from the ATR measurements. It shows that the ATR measurements of humidity, wind and cloud-base cloud fraction measured with different techniques and samplings are internally consistent, that meteorological measurements are consistent with estimates from dropsondes launched from an overflying aircraft (HALO), and that water isotopic measurements are well correlated with data from the Barbados Cloud Observatory. This consistency demonstrates the robustness of the ATR measurements of humidity, wind, cloud-base cloud fraction and water isotopic composition during EUREC4A. It also confirms that through their repeated flight patterns, the ATR and HALO measurements provided a statistically consistent sampling of trade-wind clouds and of their environment. The ATR datasets are freely available at the locations specified in Table 11.

Comparison of Macro- and Microphysical Properties in Precipitating and Non-Precipitating Clouds over Central-Eastern China during Warm Season

The macro- and microphysical properties of clouds can reflect their vertical physical structure and evolution and are important indications of the formation and development of precipitation. We used four-year merged CloudSat-CALIPSO-MODIS products to distinguish the macro- and microphysical properties of precipitating and non-precipitating clouds over central-eastern China during the warm season (May–September). Our results showed that the clouds were dominated by single- and double-layer forms with occurrence frequencies > 85%. Clouds with a low probability of precipitation (POP) were usually geometrically thin. The POP showed an increasing trend with increases in the cloud optical depth, liquid water path, and ice water path, reaching maxima of 50%, 60%, and 75%, respectively. However, as cloud effective radius (CER) increased, the POP changed from an increasing to a decreasing trend for a CER > 22 μm, in contrast with our perception that large particles fall more easily against updrafts, but this shift can be attributed to the transition of the cloud phase from mixed clouds to ice clouds. A high POP > 60% usually occurred in mixed clouds with vigorous ice-phase processes. There were clear differences in the microphysical properties of non-precipitating and precipitating clouds. In contrast with the vertical evolution of non-precipitating clouds with weaker reflectivity, precipitating clouds were present above 0 dBZ with a significant downward increase in reflectivity, suggesting inherent differences in cloud dynamical and microphysical processes. Our findings highlight the differences in the POP of warm and mixed clouds, suggesting that the low frequency of precipitation from water clouds should be the focus of future studies.

The Effect of Using a New Parameterization of Nucleation in the WRF-Chem Model on New Particle Formation in a Passive Volcanic Plume

We investigated the role of the passive volcanic plume of Mount Etna (Italy) in the formation of new particles in the size range of 2.5–10 nm through the gas-to-particle nucleation of sulfuric acid (H2SO4) precursors, formed from the oxidation of SO2, and their evolution to particles with diameters larger than 100 nm. Two simulations were performed using the Weather Research and Forecasting Model coupled with chemistry (WRF-Chem) under the same configuration, except for the nucleation parameterization implemented in the model: the activation nucleation parameterization (JS1 = 2.0 × 10−6 × (H2SO4)) in the first simulation (S1) and a new parameterization for nucleation (NPN) (JS2 = 1.844 × 10−8 × (H2SO4)1.12) in the second simulation (S2). The comparison of the numerical results with the observations shows that, on average, NPN improves the performance of the model in the prediction of the H2SO4 concentrations, newly-formed particles (~2.5–10 nm), and their growth into larger particles (10–100 nm) by decreasing the rates of H2SO4 consumption and nucleation relative to S1. In addition, particles formed in the plume do not grow into cloud condensation nuclei (CCN) sizes (100–215 nm) within a few hours of the vent (tens of km). However, tracking the size evolution of simulated particles along the passive plume indicates the downwind formation of particles larger than 100 nm more than 100 km far from the vent with relatively high concentrations relative to the background (more than 1500 cm−3) in S2. These particles, originating in the volcanic source, could affect the chemical and microphysical properties of clouds and exert regional climatic effects over time.

Mass of different snow crystal shapes derived from fall speed measurements

Meteorological forecast and climate models require good knowledge of the microphysical properties of hydrometeors and the atmospheric snow and ice crystals in clouds, for instance, their size, cross-sectional area, shape, mass, and fall speed. Especially shape is an important parameter in that it strongly affects the scattering properties of ice particles and consequently their response to remote sensing techniques. The fall speed and mass of ice particles are other important parameters for both numerical forecast models and the representation of snow and ice clouds in climate models. In the case of fall speed, it is responsible for the rate of removal of ice from these models. The particle mass is a key quantity that connects the cloud microphysical properties to radiative properties. Using an empirical relationship between the dimensionless Reynolds and Best numbers, fall speed and mass can be derived from each other if particle size and cross-sectional area are also known. In this study, ground-based in situ measurements of snow particle microphysical properties are used to analyse mass as a function of shape and the other properties particle size, cross-sectional area, and fall speed. The measurements for this study were done in Kiruna, Sweden, during snowfall seasons of 2014 to 2019 and using the ground-based in situ Dual Ice Crystal Imager (D-ICI) instrument, which takes high-resolution side- and top-view images of natural hydrometeors. From these images, particle size (maximum dimension), cross-sectional area, and fall speed of individual particles are determined. The particles are shape-classified according to the scheme presented in our previous study, in which particles sort into 15 different shape groups depending on their shape and morphology. Particle masses of individual ice particles are estimated from measured particle size, cross-sectional area, and fall speed. The selected dataset covers sizes from about 0.1 to 3.2 mm, fall speeds from 0.1 to 1.6 m s−1, and masses from 0.2 to 450 µg. In our previous study, the fall speed relationships between particle size and cross-sectional area were studied. In this study, the same dataset is used to determine the particle mass, and consequently, the mass relationships between particle size, cross-sectional area, and fall speed are studied for these 15 shape groups. Furthermore, the mass relationships presented in this study are compared with the previous studies. For certain crystal habits, in particular columnar shapes, the maximum dimension is unsuitable for determining Reynolds number. Using a selection of columns, for which the simple geometry allows the verification of an empirical Best-number-to-Reynolds-number relationship, we show that Reynolds number and fall speed are more closely related to the diameter of the basal facet than the maximum dimension. The agreement with the empirical relationship is further improved using a modified Best number, a function of an area ratio based on the falling particle seen in the vertical direction.

The Leipzig Aerosol and Cloud Remote Observations System LACROS – a mobile infrastructure for aerosol-cloud-interaction observations at hot spots of atmospheric research

<p>The large number of unsolved questions concerning the interaction between aerosol particles and clouds and corresponding indirect effects on precipitation and radiative transfer demand new measurement strategies and systems to resolve the atmospheric processes involved. Obtaining synergistic information about cloud and aerosol properties from multi–instrument and hence multi–sensor observations is a key approach to overcome the current lack of knowledge. Motivated by these needs, the mobile multi–instrument platform Leipzig Aerosol and Cloud Remote Observations System LACROS was set-up in 2011 by Leibniz Institute for Tropospheric Research (TROPOS). LACROS nowadays is the central component of a sophisticated framework of synergistic state-of-the-art measurement techniques and methodologies, embedded into an environment of comprehensive data management.</p> <p>The current setup of LACROS comprises a set of state-of-the-art remote-sensing instruments such as a 35-GHz scanning polarimetric cloud radar, multi-wavelength polarization Raman lidars, Doppler lidar, micro rain radar, microwave radiometer, laser disdrometer, as well as sensors for direct and diffuse downwelling solar and terrestrial radiation. All instruments are installed within customized sea-freight containers. This ensures a highest-possible mobility of the whole set of instruments. LACROS is a central mobile exploratory platform of the European Union Aerosol, Clouds, and Trace Gases Research Infrastructure (ACTRIS, http://www.actris.net). A variety of ways for physical, remote, and virtual access to the LACROS capabilities are provided via the European Union project ATMO-ACCESS (https://www.atmo-access.eu).</p> <p>LACROS measurements focus on three main tasks: (1) Investigation of mixed-phase cloud processes by exploiting co‐located remote-sensing observations of microphysical properties and radiative effects of aerosols and clouds and their interactions. (2) Instrument validation and development of algorithms and new measurement techniques for cloud and aerosol microphysics retrievals such as, i.e., dual‐field‐of‐view lidar to derive cloud droplet size information, or retrievals of aerosol microphysical properties from combined lidar and Sun photometer measurements. (3) Field deployments in key regions of atmospheric research, where the processes under investigation are already naturally constrained and observations can ideally be combined with in-situ observations or model simulations.</p> <p> </p> <p>This contribution will present the current setup of LACROS and its recent deployments in Leipzig, the Netherlands, Cyprus and southern Chile, results of aerosol-cloud-interaction studies by means of both, case studies and multi-site long-term statistics, as well as an overview on the current and future involvement of LACROS in cal/val activities of new methods and satellite missions. </p>

Arctic low-level clouds and their importance for radiative transfer simulations

<p>The observation of low-level stratocumulus cloud decks in the Arctic poses challenges to ground-based remote sensing. These clouds frequently occur during summer below the lowest range gate of common zenith-pointing cloud radar instruments, like the KAZR and the Mira-35. In addition, the optical thickness of these low-level clouds often do cause a complete attenuation of the lidar beam. For remote-sensing instrument synergy retrievals, as Cloudnet (Illingworth, 2007) or ARSCL (Active Remote Sensing of Clouds, Shupe, 2007), liquid-water detection in clouds is usually based on lidar backscatter. Thus, a complete attenuation can cause misclassification of mixed-phase clouds as pure-ice clouds. Moreover, the missing cloud radar information makes it difficult to derive the cloud microphysical properties, as most common retrievals are based on cloud radar reflectivity.</p> <p>A new low-level stratus detection mask (Griesche, 2020) was used to detect these clouds. The liquid-water cloud microphysical properties were derived by a simple but effective analysis of the liquid-water path. This approach was applied to remote-sensing data from a shipborne expedition performed in the Arctic summer 2017. The values calculated by applying the adjusted method improve the results of radiative transfer simulations yielding the determination of radiative closure.</p> <p> </p> <p> </p> <p>Illingworth et al. (2007). “Cloudnet”. BAMS.</p> <p>Shupe (2007). “A ground-based multisensor cloud phase classifier”. GRL.</p> <p>Griesche et al. (2020). “Application of the shipborne remote sensing supersite OCEANET for profiling of Arctic aerosols and clouds during Polarstern cruise PS106”. AMT.</p>