scholarly journals Practical limitations of aerosol separation by a tandem differential mobility analyzer–aerosol particle mass analyzer

2016 ◽  
Vol 50 (2) ◽  
pp. 160-172 ◽  
Author(s):  
James G. Radney ◽  
Christopher D. Zangmeister
2016 ◽  
Author(s):  
Sergey S. Vlasenko ◽  
Hang Su ◽  
Ulrich Pöschl ◽  
Meinrat O. Andreae ◽  
Eugene F. Mikhailov

Abstract. A tandem arrangement of Differential Mobility Analyzer and Humidified Centrifugal Particle Mass Analyzer (DMA-HCPMA) was developed to measure the deliquescence and efflorescence thresholds and the water uptake of submicron particles over the relative humidity (RH) range from 10 % to 95 %. The hygroscopic growth curves obtained for Ammonium sulfate and sodium chloride test aerosols are consistent with thermodynamic model predictions and literature data. The DMA-HCPMA system was applied to measure the hygroscopic properties of urban aerosol particles, and the kappa mass interaction model (KIM) was used to characterize and parameterize the concentration-dependent water uptake observed in the 50–95 % RH range. For DMA-selected 160 nm dry particles (mass of 3.5 fg), we obtained a volume-based hygroscopicity parameter κv ≈ 0.2, which is consistent with literature data for freshly emitted urban aerosols. Overall, our results show that the DMA-HCPMA system can be used to measure size-resolved mass growth factors of atmospheric aerosol particles upon hydration and dehydration up to 95 % RH. The direct measurements of humidified particle mass allow avoiding complications that occur in the commonly used mobility-diameter-based HTDMA technique due to poorly defined particle morphology and density.


2011 ◽  
Vol 45 (2) ◽  
pp. 196-214 ◽  
Author(s):  
Naoko Tajima ◽  
Nobuhiko Fukushima ◽  
Kensei Ehara ◽  
Hiromu Sakurai

2009 ◽  
Vol 43 (7) ◽  
pp. 673-678 ◽  
Author(s):  
Quentin G. J. Malloy ◽  
Shunsuke Nakao ◽  
Li Qi ◽  
Rebecca Austin ◽  
Clayton Stothers ◽  
...  

2017 ◽  
Vol 52 (1) ◽  
pp. 19-29 ◽  
Author(s):  
Bo-Xi Liao ◽  
Neng-Chun Tseng ◽  
Chuen-Jinn Tsai

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