The impact of CO2on the electrical properties of water bearing porous media - laboratory experiments with respect to carbon capture and storage

2012 ◽  
Vol 61 ◽  
pp. 446-460 ◽  
Author(s):  
Jana H. Börner ◽  
Volker Herdegen ◽  
Jens-Uwe Repke ◽  
Klaus Spitzer
2019 ◽  
Vol 6 (6) ◽  
pp. 181902 ◽  
Author(s):  
Junchen Lv ◽  
Yuan Chi ◽  
Changzhong Zhao ◽  
Yi Zhang ◽  
Hailin Mu

Reliable measurement of the CO 2 diffusion coefficient in consolidated oil-saturated porous media is critical for the design and performance of CO 2 -enhanced oil recovery (EOR) and carbon capture and storage (CCS) projects. A thorough experimental investigation of the supercritical CO 2 diffusion in n -decane-saturated Berea cores with permeabilities of 50 and 100 mD was conducted in this study at elevated pressure (10–25 MPa) and temperature (333.15–373.15 K), which simulated actual reservoir conditions. The supercritical CO 2 diffusion coefficients in the Berea cores were calculated by a model appropriate for diffusion in porous media based on Fick's Law. The results show that the supercritical CO 2 diffusion coefficient increases as the pressure, temperature and permeability increase. The supercritical CO 2 diffusion coefficient first increases slowly at 10 MPa and then grows significantly with increasing pressure. The impact of the pressure decreases at elevated temperature. The effect of permeability remains steady despite the temperature change during the experiments. The effect of gas state and porous media on the supercritical CO 2 diffusion coefficient was further discussed by comparing the results of this study with previous study. Based on the experimental results, an empirical correlation for supercritical CO 2 diffusion coefficient in n -decane-saturated porous media was developed. The experimental results contribute to the study of supercritical CO 2 diffusion in compact porous media.


2021 ◽  
pp. 0734242X2110481
Author(s):  
V. Bisinella ◽  
J. Nedenskov ◽  
Christian Riber ◽  
Tore Hulgaard ◽  
Thomas H. Christensen

Amending municipal solid waste incineration with carbon capture and storage (CCS) is a new approach that can reduce the climate change impacts of waste incineration. This study provides a detailed analysis of the consequences of amending the new Amager Bakke incinerator in Copenhagen (capacity: 600,000 tonnes waste per year) with CCS as a post-combustion technology. Emphasis is on the changes in the energy flows and outputs as well as the environmental performance of the plant; the latter is assessed by life cycle assessment. Amending Amager Bakke with CCS of the chosen configuration reduces the electricity output by 50% due to steam use by the capture unit, but introducing post-capture flue gas condensation increases the heat output utilized in the Copenhagen district heating system by 20%. Thus, the overall net energy efficiency is not affected. The CCS amendment reduces the fossil CO2 emissions to 40 kg CO2 per tonne of incinerated waste and stores 530 kg biogenic CO2 per tonne of incinerated waste. Potential developments in the composition of the residual waste incinerated or in the energy systems that Amager Bakke interacts with, do not question the benefits of the CCS amendment. In terms of climate change impacts, considering different waste composition and energy system scenarios, introducing CCS reduces in average the impact of Amager Bakke by 850 kg CO2-equivalents per tonne of incinerated waste. CCS increases the environmental impacts in other categories, but not in the same order of magnitude as the savings introduced within climate change.


Author(s):  
Ralph F. Keeling ◽  
Andrew C. Manning ◽  
Manvendra K. Dubey

Compared with other industrial processes, carbon capture and storage (CCS) will have an unusual impact on atmospheric composition by reducing the CO 2 released from fossil-fuel combustion plants, but not reducing the associated O 2 loss. CO 2 that leaks into the air from below-ground CCS sites will also be unusual in lacking the O 2 deficit normally associated with typical land CO 2 sources, such as from combustion or ecosystem exchanges. CCS may also produce distinct isotopic changes in atmospheric CO 2 . Using simple models and calculations, we estimate the impact of CCS or leakage on regional atmospheric composition. We also estimate the possible impact on global atmospheric composition, assuming that the technology is widely adopted. Because of its unique signature, CCS may be especially amenable to monitoring, both regionally and globally, using atmospheric observing systems. Measurements of the O 2 /N 2 ratio and the CO 2 concentration in the proximity of a CCS site may allow detection of point leaks of the order of 1000 ton CO 2 yr −1 from a CCS reservoir up to 1 km from the source. Measurements of O 2 /N 2 and CO 2 in background air from a global network may allow quantification of global and hemispheric capture rates from CCS to the order of ±0.4 Pg C yr −1 .


Author(s):  
Patricia N. Seevam ◽  
Julia M. Race ◽  
Martin J. Downie ◽  
Phil Hopkins

Climate change has been attributed to greenhouse gases with carbon dioxide (CO2) being the major contributor. Most of these CO2 emissions originate from the burning of fossil fuels (e.g. power plants). Governments and industry worldwide are now proposing to capture CO2 from their power plants and either store it in depleted reservoirs or saline aquifers (‘Carbon Capture and Storage’, CCS), or use it for ‘Enhanced Oil Recovery’ (EOR) in depleting oil and gas fields. The capture of this anthropogenic (man made sources of CO2) CO2 will mitigate global warming, and possibly reduce the impact of climate change. The United States has over 30 years experience with the transportation of carbon dioxide by pipeline, mainly from naturally occurring, relatively pure CO2 sources for onshore EOR. CCS projects differ significantly from this past experience as they will be focusing on anthropogenic sources from major polluters such as fossil fuel power plants, and the necessary CO2 transport infrastructure will involve both long distance onshore and offshore pipelines. Also, the fossil fuel power plants will produce CO2 with varying combinations of impurities depending on the capture technology used. CO2 pipelines have never been designed for these differing conditions; therefore, CCS will introduce a new generation of CO2 for transport. Application of current design procedures to the new generation pipelines is likely to yield an over-designed pipeline facility, with excessive investment and operating cost. In particular, the presence of impurities has a significant impact on the physical properties of the transported CO2 which affects: pipeline design; compressor/pump power; repressurisation distance; pipeline capacity. These impurities could also have implications in the fracture control of the pipeline. All these effects have direct implications for both the technical and economic feasibility of developing a carbon dioxide transport infrastructure onshore and offshore. This paper compares and contrasts the current experience of transporting CO2 onshore with the proposed transport onshore and offshore for CCS. It covers studies on the effect of physical and transport properties (hydraulics) on key technical aspects of pipeline transportation, and the implications for designing and operating a pipeline for CO2 containing impurities. The studies reported in the paper have significant implications for future CO2 transportation, and highlight a number of knowledge gaps that will have to be filled to allow for the efficient and economic design of pipelines for this ‘next’ generation of anthropogenic CO2.


2010 ◽  
Vol 21 (8) ◽  
pp. 925-936 ◽  
Author(s):  
Edward H Owens ◽  
Samuel Chapman ◽  
Paul Allan

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